Abstract
Unipolar pulses have a nonzero electric pulse area (integral of the electric field strength with respect of time in a given point of space). Due to unidirectional action on charges they can ...be an efficient tool for ultrafast control of wave packet dynamics in matter, charges acceleration and so one. In this paper, we briefly revise recent advances (including the results obtained by the authors) in optics of extremely-short unipolar half-cycle pulses.
We study theoretically a possibility of creation and ultrafast control (erasing, spatial frequency multiplication) of population density gratings in a multi-level resonant medium having a resonance ...transition frequency in the THz range. These gratings are produced by subcycle THz pulses coherently interacting with a nonlinear medium, without any need for pulses to overlap, thereby utilizing an indirect pulse interaction via an induced coherent polarization grating. High values of dipole moments of the transitions in the THz range facilitate low field strength of the needed THz excitation. Our results clearly show this possibility in multi-level resonant media. Our theoretical approach is based on an approximate analytical solution of time-dependent Schrödinger equation (TDSE) using perturbation theory. Remarkably, as we show here, quasi-unipolar subcycle pulses allow more efficient excitation of higher quantum levels, leading to gratings with a stronger modulation depth. Numerical simulations, performed for THz resonances of the Formula: see text molecule using Bloch equations for density matrix elements, are in agreement with analytical results in the perturbative regime. In the strong-field non-perturbative regime, the spatial shape of the gratings becomes non-harmonic. A possibility of THz radiation control using such gratings is discussed. The predicted phenomena open novel avenues in THz spectroscopy of molecules with unipolar and quasi-unipolar THz light bursts and allow for better control of ultra-short THz pulses.
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IZUM, KILJ, NUK, PILJ, PNG, SAZU, UL, UM, UPUK
Terahertz (THz) radiation produced by the filamentation of two-color pulses over long distances in argon is numerically investigated using a comprehensive model in full space-time-resolved geometry. ...We show that the dominant physical mechanism for THz generation in the filamentation regime at clamping intensity is based on quasi-dc plasma currents. The calculated THz spectra for different pump pulse energies and pulse durations are in agreement with previously reported experimental observations. For the same pulse parameters, near-infrared pump pulses at 2 μm are shown to generate a more than 1 order of magnitude greater THz yield than pumps centered at 800 nm.
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In the field of high-order harmonic generation from solids, the electron motion typically exceeds the edge of the first Brillouin zone. In conventional nonlinear optics, on the other hand, the ...excursion of band electrons is negligible. Here, we investigate the transition from conventional nonlinear optics to the regime where the crystal electrons begin to explore the first Brillouin zone. It is found that the nonlinear optical response changes abruptly already before intraband currents due to ionization become dominant. This is observed by an interference structure in the third-order harmonic generation of few-cycle pulses in a non-collinear geometry. Although approaching Keldysh parameter γ = 1, this is not a strong-field effect in the original sense, because the iterative series still converges and reproduces the interference structure. The change of the nonlinear interband response is attributed to Bloch motion of the reversible (or transient or virtual) population, similar to the Bloch motion of the irreversible (or real) population which affects the intraband currents that have been observed in high-order harmonic generation.
Abstract
Here we consider coherent mode-locking (CML) regimes in single-section cavity lasers, taking place for pulse durations less than atomic population and phase relaxation times, which arise due ...to coherent Rabi oscillations of the atomic inversion. Typically, CML is introduced for lasers with two sections, the gain and absorber ones. Here we show that, for certain combination of the cavity length and relaxation parameters, a very stable CML in a laser, containing only gain section, may arise. The mode-locking is unconditionally self-starting and appears due to balance of intra-pulse de-excitation and slow interpulse-scale pump-induced relaxation processes. We also discuss the scaling of the system to shorter pulse durations, showing a possibility of mode-locking for few-cycle pulses.
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Recent measurements of time delays during tunnelling of cold atoms through an optically created potential barrier have fuelled an ongoing debate about possible time delays during light-induced ...tunnelling of an electron from an atom. Yet, such a delay—whether it is present or not—is only one quantity characterizing the tunnelling wavepacket, whilst the underlying dynamics are richer. Here we show how to complement photo-electron detection in laser-induced tunnelling by measuring the light emitted by the tunnelling electron—the so-called Brunel radiation. Using a combination of single- and two-colour driving fields, we identify the all-optical signatures of the reshaping of the tunnelling wavepacket as it emerges from the tunnelling barrier and moves away from the core. This reshaping includes not only an effective time delay but also the time-reversal asymmetry of the ionization process, which we describe theoretically and observe experimentally. We show how both delay and reshaping are mapped onto the polarization properties of the Brunel radiation, with different harmonics behaving as different hands of a clock moving at different speeds. The all-optical detection may also allow time-resolved measurements of optical tunnelling in condensed matter systems on the attosecond time scale.Whether or not an electron wavepacket accumulates a time delay when tunnelling out of an atom is still under debate. Improved all-optical characterization of the tunnelling dynamics by combining one- and two-colour driving fields may shed light on this question.
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EMUNI, FIS, FZAB, GEOZS, GIS, IJS, IMTLJ, KILJ, KISLJ, MFDPS, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, SBMB, SBNM, UKNU, UL, UM, UPUK, VKSCE, ZAGLJ
The optical properties of metallic nanoparticles are most often considered in terms of plasmons, the coupled states of light and quasifree electrons. Confinement of electrons inside the nanostructure ...leads to another, very different type of resonances. We demonstrate that these confinement-induced resonances typically join into a single composite “super-resonance,” located at significantly lower frequencies than the plasmonic resonance. This super-resonance influences the optical properties in the low-frequency range, in particular, producing giant nonlinearities. We show that such nonlinearities can be used for efficient down-conversion from optical to terahertz and midinfrared frequencies on the submicrometer propagation distances in nanocomposites. We discuss the interaction of the quantum-confinement-induced super-resonance with the conventional plasmonic ones, as well as the unusual quantum level statistics, adapting here the paradigms of the quantum billiard theory and showing the possibility to control the resonance position and width using the geometry of the nanostructures.
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The spectrum of terahertz (THz) emission in gases via ionizing two-color femtosecond pulses is analyzed by means of a semi-analytic model and numerical simulations in 1D, 2D and 3D geometries taking ...into account propagation effects of both pump and THz fields. We show that produced THz signals interact with free electron trajectories and thus significantly influence further THz generation upon propagation, i.e., make the process inherently nonlocal. This self-action contributes to the observed strong spectral broadening of the generated THz field. We show that diffraction of the generated THz radiation is the limiting factor for the co-propagating low frequency amplitudes and thus for the self-action mechanism in 2D and 3D geometries.
Efficient all-optical switching is a challenging task as photons are bosons and cannot immediately interact with each other. Consequently, one has to resort to nonlinear optical interactions, with ...the Kerr gate being the classical example. However, the latter requires strong pulses to switch weaker ones. Numerous approaches have been investigated to overcome the resulting lack of fan-out capability of all-optical switches, most of which relied on types of resonant enhancement of light-matter interaction. Here we experimentally demonstrate a novel approach that utilizes switching between different portions of soliton fission induced supercontinua, exploiting an optical event horizon. This concept enables a high switching efficiency and contrast in a dissipation free setting. Our approach enables fan-out, does not require critical biasing, and is at least partially cascadable. Controlling complex soliton dynamics paves the way towards building all-optical logic gates with advanced functionalities.Fan-out capability, permitting one photon to switch many others, is a crucial ingredient of practical all-optical switching schemes. Exploiting an optical event horizon, high contrast switching is experimentally and theoretically demonstrated with above-unity fan-out.
Group-velocity matched cross-phase modulation between a fundamental soliton and a dispersive wave packet has been previously suggested for optical switching applications similar to an optical ...transistor. Moreover, the nonlinear interaction in the resulting group-velocity horizon can be exploited for adiabatic compression of the soliton down into the few-cycle regime. Here, we study the delicate phase- and frequency-matching mechanism of soliton/dispersive wave interaction by controlling the input chirp of the dispersive wave. We demonstrate that such a modification of the dispersive wave can significantly alter the soliton dynamics. In particular, we show that it allows a decrease of the fiber length needed for the best compression and, to some extent, control of the trajectory of the soliton. The mechanism of such an influence is related to the modification of the phase-matching condition between the soliton and dispersive wave.
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