The volume aerosol size distribution (V-ASD) obtained from the AERONET (AErosol RObotic NETwork) and SKYNET network for the years 2006–2019 at five monitoring sites in Thailand was investigated. The ...relationship between V-ASD and climate variables was determined. Fine-mode aerosols showed clear domination at all sites except at Nakhon Pathom and Phimai stations. Aerosol type can be classified into anthropogenic pollution, biomass-burning smoke and mineral dust. The results also revealed that mean temperature (
T
mean
) is directly related to both fine and coarse modes, while rainfall (R) is more effective in removing both aerosol modes, particularly smaller fine and larger coarse modes. In addition, small aerosol particles remain longer in the atmosphere at high
T
mean
with low R and low relative humidity (RH).
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DOBA, EMUNI, FIS, FZAB, GEOZS, GIS, IJS, IMTLJ, IZUM, KILJ, KISLJ, MFDPS, NLZOH, NUK, OBVAL, OILJ, PILJ, PNG, SAZU, SBCE, SBJE, SBMB, SBNM, UILJ, UKNU, UL, UM, UPUK, VKSCE, ZAGLJ
This paper presents characterization of aerosols over the Indochina peninsular regions of Southeast Asia during pre-monsoon season from satellite and ground-based radiometric observations. Our ...analysis focuses on the seasonal peak period in aerosol loading and biomass burning, prior to the onset of the Asian summer monsoon, as observed in the inter-annual variations of Aerosol Optical Depth (AOD) and fire count data from MODIS. Multi-year (2007–2011) analysis of spaceborne lidar measurements, from CALIOP, indicates presence of aerosols mostly within boundary layer, however extending to elevated altitudes to ∼4 km over northern regions of Indochina, encompassing Myanmar, northern Thailand and southern China. In addition, a strong gradient in aerosol loading and vertical distribution is observed from the relatively clean equatorial conditions to heavy smoke-laden northern regions (greater aerosol extinction and smaller depolarization ratio). Based on column-integrated ground-based measurements from four AERONET locations distributed over Thailand, the regional aerosol loading is found to be significantly absorbing with spectral single scattering albedo (SSA) below 0.91 ± 0.02 in the 440–1020 nm range, with lowest seasonal mean SSA (most absorbing aerosol) over the northern location of Chiang Mai (SSA ∼ 0.85) during pre-monsoon season. The smoke-laden aerosol loading is found to exhibit a significant diurnal pattern with higher AOD departures during early morning observations relative to late afternoon conditions (peak difference of more than 15% amplitude). Finally, satellite-based aerosol radiative impact is assessed using CERES shortwave Top-of-Atmosphere flux, in conjunction with MODIS AOD. Overall, a consistency in the aerosol-induced solar absorption characteristic is found among selected regions from ground-based sunphotometer-derived spectral SSA retrievals and satellite-based radiative forcing analysis.
► Characterization of aerosols over Indochina from satellite and surface observations. ► Multi-year analysis of aerosol vertical distribution is presented from CALIOP data. ► Regional aerosol loading is found to be significantly absorbing from AERONET data. ► The smoke-laden aerosol loading is found to exhibit a significant diurnal pattern. ► Satellite-based aerosol radiative impact is assessed using CERES data.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UL, UM, UPCLJ, UPUK
This paper presents a sky luminance model for the tropics. The model is mathematically expressed as a multiplication of two functions. These are φ, which is a function of the zenith angle of a sky ...element and solar zenith angle, and f, which is a function of the angle between the sky element and the sun. To obtain the analytical forms of these functions, the sky luminance data collected at Nakhon Pathom (13.82°N, 100.04°E), Thailand, during a four-year period were analyzed. Additionally, satellite-derived cloud index at the position of the sky luminance measurements during the same period was estimated. Based on values of the cloud index, the skies were classified into 10 types, from clear to overcast skies. By using appropriate grouping and mathematical operation of the sky luminance data, the values of the two functions were obtained and then fitted with empirical equations. The multiplication of these equations gives the final form of the sky luminance model. To validate the model, it was used to calculate the relative sky luminance at other three sites in the tropics. It was found that values of relative sky luminance calculated from the model and those obtained from the measurements were in reasonable agreement.
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FZAB, GIS, IJS, IZUM, KILJ, NLZOH, NUK, OILJ, PILJ, PNG, SAZU, SBCE, SBMB, UL, UM, UPUK
Southeast Asia (SEA) hosts one of the most complex aerosol systems in the world, with convoluted meteorological scales, sharp geographic and socioeconomic features, high biological productivity, ...mixtures of a wide range of atmospheric pollutants, and likely a significant susceptibility to global climate change. This physical complexity of SEA is coupled with one of the world's most challenging environments for both in situ and remote sensing observation. The 7-Southeast Asian Studies (7SEAS) program was formed to facilitate interdisciplinary research into the integrated SEA aerosol environment via grass roots style collaboration. In support of the early 7SEAS program and the affiliated Southeast Asia Composition, Cloud, Climate Coupling Regional Study (SEAC4RS), this review was created to outline the network of connections linking aerosol particles in SEA with meteorology, climate and the total earth system. In this review, we focus on and repeatedly link back to our primary data source: satellite aerosol remote sensing and associated observability issues. We begin with a brief rationale for the program, outlining key aerosol impacts and, comparing their magnitudes to the relative uncertainty of observations. We then discuss aspects of SEA's physical, socio-economic and biological geography relevant to meteorology and observability issues associated with clouds and precipitation. We show that not only does SEA pose significant observability challenges for aerosol particles, but for clouds and precipitation as well. With the fundamentals of the environment outlined, we explore SEA's most studied aerosol issue: biomass burning. We summarize research on bulk aerosol properties for SEA, including a short synopsis of recent AERONET observations. We describe long range transport patterns. Finally, considerable attention is paid to satellite aerosol observability issues, with a face value comparison of common aerosol products in the region including passive and active aerosol products as well as fluxes. We show that satellite data products diverge greatly due to a host of known artifacts. These artifacts have important implications for how research is conducted, and care must be taken when using satellite products to study aerosol problems. The paper ends with a discussion of how the community can approach this complex and important environment.
► The complex relationships between Southeast Asia’s geographic, meteorological and aerosol systems are reviewed. ► There are few aerosol measurements in Southeast Asia, and those that do exist suggest significant regional variability. ► Southeast Asia hosts one of the world’s most challenging aerosol observing environments. ► Satellite derived products for clouds, precipitation, fire and aerosol diverge significantly in Southeast Asia. ► If used properly, satellite products can provide significant insight into the regional aerosol environment.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UL, UM, UPCLJ, UPUK
The direct aerosol radiative effects of biomass-burning (BB) aerosols over northern Indochina were estimated by using aerosol properties (physical, chemical, and optical) along with the vertical ...profile measurements from ground-based measurements with integration of an optical and a radiative transfer model during the Seven South East Asian Studies Biomass-Burning Aerosols Stratocumulus Environment: Lifecycles Interactions Experiment (7-SEASBASELInE) conducted in spring 2013. Cluster analysis of backward trajectories showed the air masses arriving at mountainous background site (Doi Ang Khang; 19.93degN, 99.05degE, 1536 m above mean sea level) in northern Indochina, mainly from near-source inland BB activities and being confined in the planetary boundary layer. The PM(sub10) and black carbon (BC)mass were 87 +/- 28 and 7 +/- 2 micrograms m(exp -3), respectively. The aerosol optical depth (AOD (sub 500) was found to be 0.26--1.13 (0.71 +/- 0.24). Finer (fine mode fraction is approximately or equal to 0.95, angstrom-exponent at 440-870 nm is approximately or equal to 1.77) and significantly absorbing aerosols(single scattering albedo is approximately or equal to 0.89, asymmetry-parameter is approximately or equal to 0.67, and absorption AOD 0.1 at 440 nm) dominated over this region. BB aerosols (water soluble and BC) were the main contributor to the aerosol radiative forcing (ARF), while others (water insoluble, sea salt and mineral dust) were negligible mainly due to their low extinction efficiency. BC contributed only 6 to the surface aerosol mass but its contribution to AOD was 12 (2 times higher). The overall mean ARF was 8.0 and -31.4 W m(exp -2) at top-of-atmosphere (TOA) and at the surface (SFC), respectively. Likely, ARF due to BC was +10.7 and -18.1 W m(exp -2) at TOA and SFC, respectively. BC imposed the heating rate of +1.4 K d(exp -1) within the atmosphere and highlighting its pivotal role in modifying the radiation budget. We propose that to upgrade our knowledge on BB aerosol radiative effects in BB source region, the long-term and extensive field measurements are needed.
The performance of 14 models for estimating hourly diffuse irradiation on inclined surfaces was investigated. In order to obtain solar radiation data for this investigation, equipment for measuring ...solar radiation on inclined surfaces facing to the north, south, east and the west at different tilted angles to the horizontal surface (30°, 60° and 90°) were constructed and installed at two tropical sites in Thailand, namely Nakhon Pathom (13.82 °N, 100.04 °E) and Ubon Ratchathani (15.25 °N, 104.87 °E). Radiation data encompassing different periods of 1–4 years were used in this work. Diffuse irradiance measurements at different tilted angles were compared with various model algorithms. Results show that the Muneer and Gueymard models have comparable performance in terms of root mean square difference (RMSD) and these models give the lowest RMSD, as compared to that of the other models.
•Performance of 14 tilted surface diffuse radiation models was tested at two sites.•The results from the two sites are mostly similar.•The Muneer and Gueymard models have comparable performance and give best results.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UL, UM, UPCLJ, UPUK, ZRSKP
The objectives of 7-SEASBASELInE (Seven SouthEast Asian Studies Biomass-burning Aerosols and Stratocumulus Environment: Lifecycles and Interactions Experiment) campaigns in spring 2013-2015 were to ...synergize measurements from uniquely distributed ground-based networks (e.g., AERONET (AErosol RObotic NETwork)), MPLNET ( NASA Micro-Pulse Lidar Network)) and sophisticated platforms (e.g.,SMARTLabs (Surface-based Mobile Atmospheric Research and Testbed Laboratories), regional contributing instruments), along with satellite observations retrievals and regional atmospheric transport chemical models to establish a critically needed database, and to advance our understanding of biomass-burning aerosols and trace gases in Southeast Asia (SEA). We present a satellite-surface perspective of 7-SEASBASELInE and highlight scientific findings concerning: (1) regional meteorology of moisture fields conducive to the production and maintenance of low-level stratiform clouds over land; (2) atmospheric composition in a biomass-burning environment, particularly tracers-markers to serve as important indicators for assessing the state and evolution of atmospheric constituents; (3) applications of remote sensing to air quality and impact on radiative energetics, examining the effect of diurnal variability of boundary-layer height on aerosol loading; (4) aerosol hygroscopicity and ground-based cloud radar measurements in aerosol-cloud processes by advanced cloud ensemble models; and (5) implications of air quality, in terms of toxicity of nanoparticles and trace gases, to human health. This volume is the third 7-SEAS special issue (after Atmospheric Research, vol. 122, 2013; and Atmospheric Environment, vol. 78, 2013) and includes 27 papers published, with emphasis on air quality and aerosol-cloud effects on the environment. BASELInE observations of stratiform clouds over SEA are unique, such clouds are embedded in a heavy aerosol-laden environment and feature characteristically greater stability over land than over ocean, with minimal radar surface clutter at a high vertical spatial resolution. To facilitate an improved understanding of regional aerosol-cloud effects, we envision that future BASELInE-like measurement modeling needs fall into two categories: (1) efficient yet critical in-situ profiling of the boundary layer for validating remote-sensing retrievals and for initializing regional transport chemical and cloud ensemble models; and (2) fully utilizing the high observing frequencies of geostationary satellites for resolving the diurnal cycle of the boundary layerheight as it affects the loading of biomass-burning aerosols, air quality and radiative energetics.
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