This study explores the variability in concentrations of dissolved CH4 and annual flux estimates in the pelagic zone in a statistically defined sample of 207 lakes in Finland. The lakes were situated ...in the boreal zone, in an area where the mean annual air temperature ranges from −2.8 to 5.9°C. We examined how lake CH4 dynamics related to regional lake types assessed according to the EU water framework directive. Ten lake types were defined on the basis of water chemistry, color, and size. Lakes were sampled for dissolved CH4 concentrations four times per year, at four different depths at the deepest point of each lake. We found that CH4 concentrations and fluxes to the atmosphere tended to be high in nutrient rich calcareous lakes, and that the shallow lakes had the greatest surface water concentrations. Methane concentration in the hypolimnion was related to oxygen and nutrient concentrations, and to lake depth or lake area. The surface water CH4 concentration was related to the depth or area of lake. Methane concentration close to the bottom can be viewed as proxy of lake status in terms of frequency of anoxia and nutrient levels. The mean pelagic CH4 release from randomly selected lakes was 49 mmol m−2 a−1. The sum CH4 flux (storage and diffusion) correlated with lake depth, area and nutrient content, and CH4 release was greatest from the shallow nutrient rich and humic lakes. Our results support earlier lake studies regarding the regulating factors and also the magnitude of global emission estimate. These results propose that in boreal region small lakes have higher CH4 fluxes per unit area than larger lakes, and that the small lakes have a disproportionate significance regarding to the CH4 release.
We present the first experimental evidence of the scissors mode in the superheavy nucleus 254No produced in the 208Pb(48Ca, 2nγ))254No reaction. The spectrum of γ rays emitted by the excited 254No ...nuclei shows an enhanced γ-ray yield for transition energies of ≈2.5 MeV. By measuring the linear polarization properties of the emitted γ rays, we confirm that the transitions in the enhancement region are predominantly of magnetic-dipole character, characteristic for the scissors mode. To further characterize the enhanced γ-ray yield, simulations of the electromagnetic decay of 254No were performed. The observed enhancement is reproduced by including an M1 component in the γ strength function with total strength B(M1↑)=11.8(19)μN2. This is in good agreement with the integrated M1 strength from sum-rule estimates and new calculations within the quasi-particle random-phase approximation presented here. Our results provide a stringent test of phenomenological formulae for the scissors mode currently used in stellar nucleosynthesis calculations. We find that those formulae are not satisfactory, and we recommend using sum-rule estimates assuming a rigid-body moment of inertia instead for describing the scissors mode in superheavy nuclei.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
The electromagnetic character of the ΔI=1 transitions connecting the 1- to 0-phonon and the 2- to 1-phonon wobbling bands should be dominated by an E2 component, due to the collective motion of the ...entire nuclear charge. In the present work it is shown, based on combined angular correlation and linear polarization measurements, that the mixing ratios of all analyzed connecting transitions between low-lying bands in 135Pr interpreted as 0-, 1-, and 2-phonon wobbling bands, have absolute values smaller than one. This indicates predominant M1 magnetic character, which is incompatible with the proposed wobbling nature. All experimental observables are instead in good agreement with quasiparticle-plus-triaxial-rotor model calculations, which describe the bands as resulting from a rapid re-alignment of the total angular momentum from the short to the intermediate nuclear axis.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
Abstract
The electromagnetic transition probabilities of the yrast
$$2^+$$
2
+
states in the midshell Te isotopes, two protons above the closed shell at Sn, are of great importance for the ...understanding of nuclear collectivity in these isotopes and the role played by the neutron-proton interactions and cross-shell excitations. However, the large uncertainty of the experimental data for the midshell nucleus
118
Te and the missing data for
116
Te make it difficult to pin down the general trend of the evolution of transition probabilities as a function of the neutron number. In this work, the lifetime of the yrast
$$2^+$$
2
+
state in
118
Te was measured, with the aim of reducing the uncertainty of the previous measurement. The result is
$$\tau _{2+}=7.46(19)$$
τ
2
+
=
7.46
(
19
)
ps. In addition, the lifetime of the
$$4^+$$
4
+
state was measured to be
$$\tau _{4+} = 4.25(23)$$
τ
4
+
=
4.25
(
23
)
ps. The experimental transition rates are extracted from the measured lifetimes and compared with systematic large-scale shell-model calculations. The trend of the
$$B(\textrm{E2};0^+\rightarrow 2^+)$$
B
(
E2
;
0
+
→
2
+
)
values in the midshell area is in good agreement with the calculations and the calculated
$$B_{4/2}$$
B
4
/
2
ratio provide evidence for
118
Te as a near perfect harmonic vibrator.
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EMUNI, FIS, FZAB, GEOZS, GIS, IJS, IMTLJ, KILJ, KISLJ, MFDPS, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, SBMB, SBNM, UKNU, UL, UM, UPUK, VKSCE, ZAGLJ
Lifetimes of low-lying excited states in the νi13/2+ bands of the neutron-deficient osmium isotopes 169,171,173Os have been measured for the first time using the recoil-distance Doppler shift and ...recoil-isomer tagging techniques. An unusually low value is observed for the ratio B(E2;21/2+→17/2+)/B(E2;17/2+→13/2+) in 169Os, similar to the “anomalously” low values of the ratio B(E2;41+→21+)/B(E2;21+→0gs+) previously observed in several transitional rare-earth nuclides with even numbers of neutrons and protons, including the neighbouring 168,170Os. Furthermore, the evolution of B(E2;21/2+→17/2+)/B(E2;17/2+→13/2+) with increasing neutron number in the odd-mass isotopic chain 169,171,173Os is observed to follow the same trend as observed previously in the even-even Os isotopes. These findings indicate that the possible quantum phase transition from a seniority conserving structure to a collective regime as a function of neutron number suggested for the even-even systems is maintained in these odd-mass osmium nuclei, with the odd valence neutron merely acting as a “spectator”. As for the even-even nuclei, the phenomenon is highly unexpected for nuclei that are not situated near closed shells.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
Nitrogen (N) pollution of peatlands alters their carbon (C) balances, yet long-term effects and controls are poorly understood. We applied the model PEATBOG to explore impacts of long-term nitrogen ...(N) fertilization on C cycling in an ombrotrophic bog. Simulations of summer gross ecosystem production (GEP), ecosystem respiration (ER) and net ecosystem exchange (NEE) were evaluated against 8 years of observations and extrapolated for 80 years to identify potential effects of N fertilization and factors influencing model behaviour. The model successfully simulated moss decline and raised GEP, ER and NEE on fertilized plots. GEP was systematically overestimated in the model compared to the field data due to factors that can be related to differences in vegetation distribution (e.g. shrubs vs. graminoid vegetation) and to high tolerance of vascular plants to N deposition in the model. Model performance regarding the 8-year response of GEP and NEE to N input was improved by introducing an N content threshold shifting the response of photosynthetic capacity (GEPmax) to N content in shrubs and graminoids from positive to negative at high N contents. Such changes also eliminated the competitive advantages of vascular species and led to resilience of mosses in the long-term. Regardless of the large changes of C fluxes over the short-term, the simulated GEP, ER and NEE after 80 years depended on whether a graminoid- or shrub-dominated system evolved. When the peatland remained shrub-Sphagnum-dominated, it shifted to a C source after only 10 years of fertilization at 6.4 g N m-2 yr-1, whereas this was not the case when it became graminoid-dominated. The modelling results thus highlight the importance of ecosystem adaptation and reaction of plant functional types to N deposition, when predicting the future C balance of N-polluted cool temperate bogs.
Prolate-oblate shape coexistence close to the ground state in the strongly-deformed proton-rich A≈120 nuclei is reported for the first time. One of the four reported bands in 119Cs, built on a 11/2− ...state at 670 keV, consists of nearly degenerate signature partners, and has properties which unequivocally indicate the strongly-coupled πh11/250511/2− configuration associated with oblate shape. Together with the decoupled πh11/25413/2− band built on the 11/2− prolate state at 110 keV, for which a half-life of T1/2=55(5)μs has been measured, the new bands bring evidence of shape coexistence at low spin in the proton-rich strongly deformed A≈120 nuclei, a phenomenon predicted since long time, but not yet observed. Calculations using the particle-number conserving cranked shell model and two dimensional tilted axis cranking covariant density functional theory support and well reproduce the observed oblate and prolate coexisting low-energy states in 119Cs.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
In-beam $$\gamma $$-ray spectroscopy of $$^{94}$$Ag Pereira-López, X.; Bentley, M. A.; Wadsworth, R. ...
The European physical journal. A, Hadrons and nuclei,
03/2023, Volume:
59, Issue:
3
Journal Article
Peer reviewed
Open access
Abstract
A recoil-beta-tagging experiment has been performed to study the excited
$$T=0$$
T
=
0
and
$$T=1$$
T
=
1
states in the odd–odd
$$N=Z$$
N
=
Z
nucleus
$$^{94}$$
94
Ag, populated via the
...$$^{40}$$
40
Ca(
$$^{58}$$
58
Ni,1p3n)
$$^{94}$$
94
Ag reaction. The experiment was conducted using the MARA recoil separator and JUROGAM3 array at the Accelerator Laboratory of the University of Jyväskylä. Through correlating fast, high-energy beta decays at the MARA focal plane with prompt
$$\gamma $$
γ
rays emitted at the reaction target, a number of transitions between excited states in
$$^{94}$$
94
Ag have been identified. The timing characteristics of these transitions confirm that they fall within decay sequences that feed the short-lived
$$T=1$$
T
=
1
ground state of
$$^{94}$$
94
Ag. The transitions are proposed to proceed within and between the sets of states with
$$T=0$$
T
=
0
and
$$T=1$$
T
=
1
. Possible correspondence between some of these transitions from analog states in
$$^{94}$$
94
Pd has been discussed, and shell-model calculations including multipole and monopole electromagnetic effects have been presented, in order to enable predictions of the decay patterns between the
$$T=0$$
T
=
0
and
$$T=1$$
T
=
1
states and to allow a theoretical set of Coulomb energy differences to be calculated for the
$$A = 94$$
A
=
94
$$T=1$$
T
=
1
analog states.
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EMUNI, FIS, FZAB, GEOZS, GIS, IJS, IMTLJ, KILJ, KISLJ, MFDPS, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, SBMB, SBNM, UKNU, UL, UM, UPUK, VKSCE, ZAGLJ
The electromagnetic transition probabilities of the yrast 2+ states in the midshell Te isotopes, two protons above the closed shell at Sn, are of great importance for the understanding of nuclear ...collectivity in these isotopes and the role played by the neutron-proton interactions and cross-shell excitations. However, the large uncertainty of the experimental data for the midshell nucleus 118Te and the missing data for 116Te make it difficult to pin down the general trend of the evolution of transition probabilities as a function of the neutron number. In this work, the lifetime of the yrast 2+ state in 118Te was measured, with the aim of reducing the uncertainty of the previous measurement. The result is τ2+ = 7.46(19) ps. In addition, the lifetime of the 4+ state was measured to be τ4+ = 4.25(23) ps. The experimental transition rates are extracted from the measured lifetimes and compared with systematic large-scale shell-model calculations. The trend of the B(E2; 0+ → 2+) values in the midshell area is in good agreement with the calculations and the calculated B4/2 ratio provide evidence for 118Te as a near perfect harmonic vibrator.
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DOBA, EMUNI, FIS, FZAB, GEOZS, GIS, IJS, IMTLJ, IZUM, KILJ, KISLJ, MFDPS, NLZOH, NUK, OILJ, PILJ, PNG, SAZU, SBCE, SBJE, SBMB, SBNM, SIK, UILJ, UKNU, UL, UM, UPUK, VKSCE, ZAGLJ
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