Abstract Pyrocumulonimbus (pyroCb) firestorm systems have been shown to inject significant amounts of black carbon (BC) to the stratosphere with a residence time of several months. Injected BC warms ...the local stratospheric air, consequently perturbing transport and hence spatial distributions of ozone and water vapor. A distinguishing feature of BC-containing particles residing within pyroCb smoke is their thick surface coatings made of condensed organic matter. When coated with non-refractory materials, BC’s absorption is enhanced, yet the absorption enhancement factor ( E abs ) for pyroCb BC is not well constrained. Here, we perform particle-scale measurements of BC mass, morphology, and coating thickness from inside a pyroCb cloud and quantify E abs using an established particle-resolved BC optics model. We find that the population-averaged E abs for BC asymptotes to 2.0 with increasing coating thickness. This value denotes the upper limit of E abs for thickly coated BC in the atmosphere. Our results provide observationally constrained parameterizations of BC absorption for improved radiative transfer calculations of pyroCb events.
Pyrocumulonimbus (pyroCb) are wildfire-generated convective clouds that can inject smoke directly into the stratosphere. PyroCb have been tracked for years, yet their apparent rarity and episodic ...nature lead to highly uncertain climate impacts. In situ measurements of pyroCb smoke reveal its distinctive and exceptionally stable aerosol properties and define the long-term influence of pyroCb activity on the stratospheric aerosol budget. Analysis of 13 years of airborne observations shows that pyroCb are responsible for 10 to 25% of the black carbon and organic aerosols in the "present-day" lower stratosphere, with similar impacts in both the North and South Hemispheres. These results suggest that, should pyroCb increase in frequency and/or magnitude in future climates, they could generate dominant trends in stratospheric aerosol.
Abstract
Anthropogenic iron oxide aerosols (FeO
x
) have been identified as a climatically significant atmospheric light absorber, and as a contributor of free iron to the oceans. Here we provide ...global-scale constraints on their atmospheric abundance with measurements over the remote Pacific and Atlantic Oceans from aircraft campaigns spanning 10 years. We find FeO
x
-like aerosols are transported far from source regions with similar efficiency as black carbon particles. Strong contrast in concentrations was observed between the Northern and Southern Hemisphere Pacific. We provide observational constraints in remote regions on the ambient ratios of FeO
x
relative to BC from fossil fuel burning. Comparison with a global aerosol model tuned to recent observations in East-Asian source regions confirm an upward revision of emissions based on model/observation comparison over the Pacific receptor region. We find that anthropogenic FeO
x
-like particles generate global-scale shortwave atmospheric heating 0.3–26% of that of black carbon in remote regions where concentrations of both aerosols are very low.
Due to the lack of free neutron targets, studies of the structure of the neutron are typically made by scattering electrons from either 2H or 3He targets. In order to extract useful neutron ...information from a 3He target, one must understand how the neutron in a 3He system differs from a free neutron by taking into account nuclear effects such as final state interactions and meson exchange currents. The target single spin asymmetry Ay0 is an ideal probe of such effects, as any deviation from zero indicates effects beyond plane wave impulse approximation. New measurements of the target single spin asymmetry Ay0 at Q2 of 0.46 and 0.96 (GeV/c)2 were made at Jefferson Lab using the quasi-elastic He↑3(e,e′n) reaction. Our measured asymmetry decreases rapidly, from >20% at Q2=0.46 (GeV/c)2 to nearly zero at Q2=0.96 (GeV/c)2, demonstrating the fall-off of the reaction mechanism effects as Q2 increases. We also observed a small ϵ-dependent increase in Ay0 compared to previous measurements, particularly at moderate Q2. This indicates that upcoming high Q2 measurements from the Jefferson Lab 12 GeV program can cleanly probe neutron structure from polarized 3He using plane wave impulse approximation.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
Accurate fire emissions inventories are crucial to predict the impacts of wildland fires on air quality and atmospheric composition. Two traditional approaches are widely used to calculate fire ...emissions: a satellite-based top-down approach and a fuels-based bottom-up approach. However, these methods often considerably disagree on the amount of particulate mass emitted from fires. Previously available observational datasets tended to be sparse, and lacked the statistics needed to resolve these methodological discrepancies. Here, we leverage the extensive and comprehensive airborne in situ and remote sensing measurements of smoke plumes from the recent Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) campaign to statistically assess the skill of the two traditional approaches. We use detailed campaign observations to calculate and compare emission rates at an exceptionally high-resolution using three separate approaches: top-down, bottom-up, and a novel approach based entirely on integrated airborne in situ measurements. We then compute the daily average of these high-resolution estimates and compare with estimates from lower resolution, global top-down and bottom-up inventories. We uncover strong, linear relationships between all of the high-resolution emission rate estimates in aggregate, however no single approach is capable of capturing the emission characteristics of every fire. Global inventory emission rate estimates exhibited weaker correlations with the high-resolution approaches and displayed evidence of systematic bias. The disparity between the low resolution global inventories and the high-resolution approaches is likely caused by high levels of uncertainty in essential variables used in bottom-up inventories and imperfect assumptions in top-down inventories.
Plain Language Summary
Smoke emitted by wildland fires is dangerous to human health and contributes to climate change.To predict and evaluate the impacts of fires, we need to know how much smoke is emitted into the atmosphere. There are two state-of-the-art methods used to estimate the mass of smoke emitted by fires, but they often disagree. In this study, we use unusually detailed measurements collected using an aircraft that flew within wildland fire smoke plumes to calculate the amount ofsmoke emitted from fires in the Western United States. We compare emission rates derived from the exceptionally high spatial and temporal resolution approach to the two traditional, lower resolution approaches to understand why they sometimes diverge
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BFBNIB, FZAB, GIS, IJS, KILJ, NLZOH, NUK, OILJ, SAZU, SBCE, SBMB, UL, UM, UPUK
We report the first measurement of the target-normal single-spin asymmetry in deep-inelastic scattering from the inclusive reaction super(3)Heuarr (e, e')X on a polarized super(3)He gas target. ...Assuming time-reversal invariance, this asymmetry is strictly zero in the Born approximation but can be nonzero if two-photon-exchange contributions are included. The experiment, conducted at Jefferson Lab using a 5.89 GeV electron beam, covers a range of 1.7 < W < 2.9 GeV, 1.0 < Q super(2) < 4.0 GeV super(2) and 0.16 < x < 0.65. Neutron asymmetries were extracted using the effective nucleon polarization and measured proton-to- super(3)He cross-section ratios. The measured neutron asymmetries are negative with an average value of (-1.09 + or - 0.38) x 10 super(-2) for invariant mass W > 2 GeV, which is nonzero at the 2.89sigma level. Our measured asymmetry agrees both in sign and magnitude with a two-photon-exchange model prediction that uses input from the Sivers transverse momentum distribution obtained from semiinclusive deepinelastic scattering.
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CMK, CTK, FMFMET, IJS, NUK, PNG, UM
We report a new, high-precision measurement of the proton elastic form factor ratio μpGE/GM for the four-momentum transfer squared Q2=0.3–0.7(GeV/c)2. The measurement was performed at Jefferson Lab ...(JLab) in Hall A using recoil polarimetry. With a total uncertainty of approximately 1%, the new data clearly show that the deviation of the ratio μpGE/GM from unity observed in previous polarization measurements at high Q2 continues down to the lowest Q2 value of this measurement. The updated global fit that includes the new results yields an electric (magnetic) form factor roughly 2% smaller (1% larger) than the previous global fit in this Q2 range. We obtain new extractions of the proton electric and magnetic radii, which are 〈rE2〉1/2=0.875±0.010 fm and 〈rM2〉1/2=0.867±0.020 fm. The charge radius is consistent with other recent extractions based on the electron–proton interaction, including the atomic hydrogen Lamb shift measurements, which suggests a missing correction in the comparison of measurements of the proton charge radius using electron probes and the recent extraction from the muonic hydrogen Lamb shift.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UL, UM, UPCLJ, UPUK
The SeaQuest spectrometer at Fermilab Aidala, C.A.; Arrington, J.R.; Ayuso, C. ...
Nuclear instruments & methods in physics research. Section A, Accelerators, spectrometers, detectors and associated equipment,
06/2019, Volume:
930, Issue:
C
Journal Article
Peer reviewed
Open access
The SeaQuest spectrometer at Fermilab was designed to detect oppositely-charged pairs of muons (dimuons) produced by interactions between a 120 GeV proton beam and liquid hydrogen, liquid deuterium ...and solid nuclear targets. The primary physics program uses the Drell–Yan process to probe antiquark distributions in the target nucleon. The spectrometer consists of a target system, two dipole magnets and four detector stations. The upstream magnet is a closed-aperture solid iron magnet which also serves as the beam dump, while the second magnet is an open aperture magnet. Each of the detector stations consists of scintillator hodoscopes and a high-resolution tracking device. The FPGA-based trigger compares the hodoscope signals to a set of pre-programmed roads to determine if the event contains oppositely-signed, high-mass muon pairs.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
We report on the results of the E06-014 experiment performed at Jefferson Lab in Hall A, where a precision measurement of the twist-3 matrix element d2 of the neutron (d2n) was conducted. The ...quantity d2n represents the average color Lorentz force a struck quark experiences in a deep inelastic electron scattering event off a neutron due to its interaction with the hadronizing remnants. This color force was determined from a linear combination of the third moments of the He3 spin structure functions, g1 and g2, after nuclear corrections had been applied to these moments. The structure functions were obtained from a measurement of the unpolarized cross section and of double-spin asymmetries in the scattering of a longitudinally polarized electron beam from a transversely and a longitudinally polarized He3 target. The measurement kinematics included two average Q2 bins of 3.2 GeV2 and 4.3 GeV2, and Bjorken-x 0.25≤x≤0.90 covering the deep inelastic and resonance regions. We have found that d2n is small and negative for ⟨Q2⟩=3.2 GeV2, and even smaller for ⟨Q2⟩=4.3 GeV2, consistent with the results of a lattice QCD calculation. The twist-4 matrix element f2n was extracted by combining our measured d2n with the world data on the first moment in x of g1n, Γ1n. We found f2n to be roughly an order of magnitude larger than d2n. Utilizing the extracted d2n and f2n data, we separated the Lorentz color force into its electric and magnetic components, FEy,n and FBy,n, and found them to be equal and opposite in magnitude, in agreement with the predictions from an instanton model but not with those from QCD sum rules. Furthermore, using the measured double-spin asymmetries, we have extracted the virtual photon-nucleon asymmetry on the neutron A1n, the structure function ratio g1n/F1n, and the quark ratios (Δu+Δu¯)/(u+u¯) and (Δd+Δd¯)/(d+d¯). These results were found to be consistent with deep-inelastic scattering world data and with the prediction of the constituent quark model but at odds with the perturbative quantum chromodynamics predictions at large x.
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CMK, CTK, FMFMET, IJS, NUK, PNG, UM
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