We report the best limit on coherent elastic scattering of electron antineutrinos emitted from a nuclear reactor off germanium nuclei. The measurement was performed with the CONUS detectors ...positioned at 17.1 m from the 3.9 GW_{th} reactor core of the nuclear power plant in Brokdorf, Germany. The antineutrino energies of less than 10 MeV assure interactions in the fully coherent regime. The analyzed dataset includes 248.7 kg d with the reactor turned on and background data of 58.8 kg d with the reactor off. With a quenching parameter of k=0.18 for germanium, we determined an upper limit on the number of neutrino events of 85 in the region of interest at 90% confidence level. This new CONUS dataset disfavors quenching parameters above k=0.27, under the assumption of standard-model-like coherent scattering of the reactor antineutrinos.
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CMK, CTK, FMFMET, IJS, NUK, PNG, UL, UM
Chromatin is organized in a highly ordered yet dynamic manner in the cell nucleus, but the principles governing this organization remain unclear. Similarly, it is unknown whether, and how, various ...proteins regulate chromatin motion and as a result influence nuclear organization. Here by studying the dynamics of different genomic regions in the nucleus of live cells, we show that the genome has highly constrained dynamics. Interestingly, depletion of lamin A strikingly alters genome dynamics, inducing a dramatic transition from slow anomalous diffusion to fast and normal diffusion. In contrast, depletion of LAP2α, a protein that interacts with lamin A and chromatin, has no such effect on genome dynamics. We speculate that chromosomal inter-chain interactions formed by lamin A throughout the nucleus contribute to chromatin dynamics, and suggest that the molecular regulation of chromatin diffusion by lamin A in the nuclear interior is critical for the maintenance of genome organization.
CONUS is a novel experiment aiming at detecting elastic neutrino–nucleus scattering in the almost fully coherent regime using high-purity germanium (Ge) detectors and a reactor as antineutrino ...source. The detector setup is installed at the commercial nuclear power plant in Brokdorf, Germany, at a short distance to the reactor core to guarantee a high antineutrino flux. A good understanding of neutron-induced backgrounds is required, as the neutron recoil signals can mimic the predicted neutrino interactions. Especially events correlated with the reactor thermal power are troublesome. On-site measurements revealed such a correlated, highly thermalized neutron field with a maximum fluence rate of
(
745
±
30
)
cm
-
2
day
-
1
. These neutrons, produced inside the reactor core, are reduced by a factor of
∼
10
20
on their way to the CONUS shield. With a high-purity Ge detector without shield the
γ
-ray background was examined including thermal power correlated
16
N
decay products and neutron capture
γ
-lines. Using the measured neutron spectrum as input, Monte Carlo simulations demonstrated that the thermal power correlated field is successfully mitigated by the CONUS shield. The reactor-induced background contribution in the region of interest is exceeded by the expected signal by at least one order of magnitude assuming a realistic ionization quenching factor.
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DOBA, IZUM, KILJ, NUK, PILJ, PNG, SAZU, SIK, UILJ, UKNU, UL, UM, UPUK
A
bstract
The measurements of coherent elastic neutrino-nucleus scattering (CE
ν
NS) experiments have opened up the possibility to constrain neutrino physics beyond the standard model of elementary ...particle physics. Furthermore, by considering neutrino-electron scattering in the keV-energy region, it is possible to set additional limits on new physics processes. Here, we present constraints that are derived from Conus germanium data on beyond the standard model (BSM) processes like tensor and vector non-standard interactions (NSIs) in the neutrino-quark sector, as well as light vector and scalar mediators. Thanks to the realized low background levels in the C
onus
experiment at ionization energies below 1 keV, we are able to set the world’s best limits on tensor NSIs from CE
ν
NS and constrain the scale of corresponding new physics to lie above 360 GeV. For vector NSIs, the derived limits strongly depend on the assumed ionization quenching factor within the detector material, since small quenching factors largely suppress potential signals for both, the expected standard model CE
ν
NS process and the vector NSIs. Furthermore, competitive limits on scalar and vector mediators are obtained from the CE
ν
NS channel at reactor-site which allow to probe coupling constants as low as 5 ∙ 10
−
5
of low mediator masses, assuming the currently favored quenching factor regime. The consideration of neutrino-electron scatterings allows to set even stronger constraints for mediator masses below ∼ 1 MeV and ∼ 10 MeV for scalar and vector mediators, respectively.
Functionalized enantiopure organosilanes are important building blocks with applications in various fields of chemistry; nevertheless, asymmetric synthetic methods for their preparation are rare. ...Here we report the first organocatalytic enantioselective synthesis of tertiary silyl ethers possessing “central chirality” on silicon. The reaction proceeds via a desymmetrizing carbon–carbon bond forming silicon–hydrogen exchange reaction of symmetrical bis(methallyl)silanes with phenols using newly developed imidodiphosphorimidate (IDPi) catalysts. A variety of enantiopure silyl ethers was obtained in high yields with good chemo- and enantioselectivities and could be readily derivatized to several useful chiral silicon compounds, leveraging the olefin functionality and the leaving group nature of the phenoxy substituent.
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IJS, KILJ, NUK, PNG, UL, UM
A
bstract
We study the impact of TeV-scale sterile neutrinos on electro-weak precision observables and lepton number and flavour violating decays in the framework of a type-I see-saw extension of the ...Standard Model. At tree level sterile neutrinos manifest themselves via non-unitarity of the PMNS matrix and at one-loop level they modify the oblique radiative corrections. We derive explicit formulae for the
S, T, U
parameters in terms of the neutrino masses and mixings and perform a numerical fit to the electro-weak observables. We find regions of parameter space with a sizable active-sterile mixing which provide a better over-all fit compared to the case where the mixing is negligible. Specifically we find improvements of the invisible
Z
-decay width, the charged-to-neutral-current ratio for neutrino scattering experiments and of the deviation of the
W
boson mass from the theoretical expectation.
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EMUNI, FIS, FZAB, GEOZS, GIS, IJS, IMTLJ, KILJ, KISLJ, MFDPS, NUK, OILJ, PNG, SAZU, SBCE, SBJE, SBMB, SBNM, UKNU, UL, UM, UPUK, VKSCE, ZAGLJ
This article reports the measurement of the ionization quenching factor in germanium for nuclear recoil energies in the keV range. Precise knowledge of this factor in this energy range is highly ...relevant for coherent elastic neutrino-nucleus scattering and low mass dark matter searches with germanium-based detectors. Nuclear recoils were produced in a thin high-purity germanium target with a very low energy threshold via irradiation using monoenergetic neutron beams. The energy dependence of the ionization quenching factor was directly measured via kinematically constrained coincidences with surrounding liquid scintillator based neutron detectors. The systematic uncertainties of the measurements are discussed in detail. With measured quenching factors between 0.16 and 0.23 in the 0.4 keV
nr
to 6.3 keV
nr
energy range, the data are compatible with the Lindhard theory with a parameter
k
of 0.162
±
0.004
(stat + sys).
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DOBA, IZUM, KILJ, NUK, PILJ, PNG, SAZU, SIK, UILJ, UKNU, UL, UM, UPUK
The synthesis of novel semiconducting donor–acceptor (D–A) diblock copolymers by means of nitroxide‐mediated polymerization (NMP) is reported. The copolymers contain functional moieties for hole ...transport, electron transport, and light absorption. The first block, representing the donor, is made up of either substituted triphenylamines (poly(bis(4‐methoxyphenyl)‐4′‐vinylphenylamine), PvDMTPA) or substituted tetraphenylbenzidines (poly(N,N′‐bis(4‐methoxyphenyl)‐N‐phenyl‐N′‐4‐vinylphenyl‐(1,1′‐biphenyl)‐4,4′‐diamine), PvDMTPD). The second block consists of perylene diimide side groups attached to a polyacrylate backbone (PPerAcr) via a flexible spacer. This block is responsible for absorption in the visible range and for electron‐transport properties. The electrochemical properties of these fully functionalized diblock copolymers, PvDMTPA‐b‐PPerAcr and PvDMTPD‐b‐PPerAcr, are investigated by cyclic voltammetry (CV), and their morphology is investigated by transmission electron microscopy (TEM). All diblock copolymers exhibit microphase‐separated domains in the form of either wire‐ or wormlike structures made of perylene diimide embedded in a hole‐conductor matrix. In single‐active‐layer organic solar cells, PvDMTPD‐b‐PPerAcr reveals a fourfold improvement in power conversion efficiency (η = 0.26 %, short‐circuit current (ISC) 1.21 mA cm–2), and PvDMTPA‐b‐PPerAcr a fivefold increased efficiency (η = 0.32 %, ISC = 1.14 mA cm–2) compared with its unsubstituted analogue PvTPA‐b‐PPerAcr (η = 0.065 %, ISC = 0.23 mA cm–2).
A series of novel semiconducting donor–acceptor block copolymers that contain substituted triphenylamines as donors and perylene diimide as the acceptor (see figure) are synthesized by means of nitroxide‐mediated polymerization, and the influence of morphology and the highest occupied molecular orbital (HOMO) level of the donor on block‐copolymer solar‐cell characteristics is studied.
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BFBNIB, FZAB, GIS, IJS, KILJ, NLZOH, NUK, OILJ, SAZU, SBCE, SBMB, UL, UM, UPUK
The spectral shape of reactor antineutrinos measured in recent experiments shows anomalies in comparison to neutrino reference spectra. New precision measurements of the reactor neutrino spectra as ...well as more complete input in nuclear data bases are needed to resolve the observed discrepancies between models and experimental results. This article proposes the combination of experiments at reactors which are highly enriched in U235 with commercial reactors with typically lower enrichment to gain new insights into the origin of the anomalous neutrino spectrum. The presented method clarifies, if the spectral anomaly is either solely or not at all related to the predicted U235 spectrum. Considering the current improvements of the energy scale uncertainty of present-day experiments, a significance of three sigma and above can be reached. As an example, we discuss the option of a direct comparison of the measured shape in the currently running Double Chooz near detector and the upcoming Stereo experiment. A quantitative feasibility study emphasizes that a precise understanding of the energy scale systematics is a crucial prerequisite in recent and next generation experiments investigating the spectral anomaly.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
On June 21st, a Mw6.2 earthquake struck the Afghan‐Pakistan‐border‐region, situated within the India‐Asia collision. Thousand thirty‐nine deaths were reported, making the earthquake the deadliest of ...2022. We investigate the event's rupture processes by combining seismological and geodetic observations, aiming to understand what made it that fatal. Our Interferometric Synthetic Aperture Radar‐constrained slip‐model and regional moment‐tensor inversion, confirmed through field observations, reveal a sinistral rupture with maximum slip of 1.8 m at 5 km depth on a N20°E striking, sub‐vertical fault. We suggest that not only external factors (event‐time, building stock) but fault‐specific factors made the event excessively destructive. Surface rupture was favored by the rock foliation, coinciding with the fault strike. The distribution of Peak‐Ground‐Velocity was governed by the sub‐vertical fault. Maximum slip was large compared to other events globally and might have resulted in peak‐frequencies coinciding with resonance‐frequencies of the local buildings and demonstrates the devastating impact of moderate‐size earthquakes.
Plain Language Summary
The June 2022 devastating M6.2 Afghanistan earthquake has caused a high depth toll, making it the deadliest earthquake of 2022. This is notable and partly intriguing as the earthquake size is much smaller than other events that happened in 2022. Therefore, we combine a range of geophysical, geodetic and geological methods to understand how exactly the subsurface ruptured during the earthquake. We suggest that it was a combination of the local circumstances (the event time, as it hit at night time, and the building stock) and the geometry of the rupture surface together with the local geology that made this event particularly deadly. More generally, this study shows the excessive hazard and impact caused by moderate‐size earthquakes.
Key Points
We combine Interferometric Synthetic Aperture Radar, moment tensor inversion, field mapping and Peak‐Ground‐Velocity (PGV) simulations to investigate the rupture processes
The event had a sinistral rupture with maximum slip of 1.8 m at 5 km depth on a N20°E striking, sub‐vertical fault
Coincidence of large slip, fault geometry and alignment of rock foliation with strike enhanced PGV and the destructiveness of the event
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FZAB, GIS, IJS, KILJ, NLZOH, NUK, OILJ, SAZU, SBCE, SBMB, UL, UM, UPUK