The diagnosis of the key components of rotating machinery systems is essential for the production efficiency and quality of manufacturing processes. The performance of the traditional diagnosis ...method depends heavily on feature extraction, which relies on the degree of individual's expertise or prior knowledge. Recently, a deep learning (DL) method is applied to automate feature extraction. However, training in the DL method requires a massive amount of sensor data, which is time consuming and poses a challenge for its applications in engineering. In this paper, a new data-driven fault diagnosis method based on compressed sensing (CS) and improved multiscale network (IMSN) is proposed to recognize and classify the faults in rotating machinery. CS is used to reduce the amount of raw data, from which the fault information is discovered. At the same time, it can be used to generate sufficient training samples for the subsequent learning. The one-dimensional compressed signal is converted to two-dimensional image for further learning. An IMSN is established for learning and obtaining deep features. It improves the diagnosis performance of the DL process. The faults of the key components are identified from a softmax model. Experimental analysis is performed to verify effectiveness of the proposed data-driven fault diagnosis method.
The intelligent recognition of epileptic electro-encephalogram (EEG) signals is a valuable tool for the epileptic seizure detection. Recent deep learning models fail to fully consider both spectral ...and temporal domain representations simultaneously, which may lead to omitting the nonstationary or nonlinear property in epileptic EEGs and further produce a suboptimal recognition performance consequently. In this paper, an end-to-end EEG seizure detection framework is proposed by using a novel channel-embedding spectral-temporal squeeze-and-excitation network (CE-stSENet) with a maximum mean discrepancy-based information maximizing loss. Specifically, the CE-stSENet firstly integrates both multi-level spectral and multi-scale temporal analysis simultaneously. Hierarchical multi-domain representations are then captured in a unified manner with a variant of squeeze-and-excitation block. The classification net is finally implemented for epileptic EEG recognition based on features extracted in previous subnetworks. Particularly, to address the fact that the scarcity of seizure events results in finite data distribution and the severe overfitting problem in seizure detection, the CE-stSENet is coordinated with a maximum mean discrepancy-based information maximizing loss for mitigating the overfitting problem. Competitive experimental results on three EEG datasets against the state-of-the-art methods demonstrate the effectiveness of the proposed framework in recognizing epileptic EEGs, indicating its powerful capability in the automatic seizure detection.
Although municipal solid waste (MSW) has a potential risk for human health and ecological environment, it is gradually considered as one of the most renewable resources. To maximize resource ...utilization of MSW and its elimination, numerous efforts have been devoted worldwide to develop a systematic MSW management coupled with technologies in treatment and resource utilization (TTRU). This paper mainly focuses on MSW in eight eastern coastal regions in China on the aspects of background information (MSW generation, population, gross domestic product (GDP)/gross regional product (GRP)), related laws (acts, regulations), MSW characteristics (composition, separation, collection, transport) and TTRU. Besides, emerging technologies in MSW resource utilization for waste-to-energy (WtE) and waste-to-material (WtM) are reviewed for the first time. Finally, a comparison based on above information is conducted between China and selected developed regions, namely Berlin, Tokyo, and Singapore. The findings for China are summarized as follows: (1) MSW generation keeps a strong increasing trend especially in Guangdong, Jiangsu, Shandong, Zhejiang, and Fujian provinces, while MSW generation shows spatiotemporal variation in eastern coastal cities, provinces, and special zones; (2) MSW composition characteristics is complicated with a >50% moisture content and is dominated by 52.8–65.3% kitchen waste, 3.5–11.9% paper, and 9.9–19.1% rubber & plastics; (3) MSW management system needs to be optimized in China; (4) The MSW is treated by 52% landfill, 45% incineration and 3% composting technologies and utilization efficiency in China is much lower than that of developed countries; (5) Advanced and emerging technologies for MSW resource utilization are required and several potential WtE and WtM technologies are listed. Eventually, (6) Recommendations for developing an optimal system integrating MSW management with enhanced TTRU are presented, and technology transfer potentials from Berlin, Tokyo, and Singapore are noted.
Schematic diagram showing the MSW generation in China’s eastern coastal provinces and their provincial capital cities (or special zones) in 2018 associated with their spatial distribution, composition and characteristics. Display omitted
•Municipal solid waste (MSW) characteristics and related laws are discussed.•Emerging technologies in waste-to-energy and waste-to-material are reviewed.•A comparison is conducted between Chinese provinces and selected developed regions.•Integrated MSW management and treatment and utilization technologies are suggested.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
A succinct strategy was demonstrated for constructing a hydroxyl group and imidazolium-bifunctionalized ionic network via a one-pot quaternization. Key to success lies in the rational design of ...multi-imidazole precursor and hydroxyl-containing counterpart. Unique properties of the resultant ionic network render its high catalytic efficiency toward CO2 fixation under ambient conditions.
Grazing by livestock greatly affects the soil carbon (C) cycle in grassland ecosystems. However, the effects of grazing at different intensities and durations on the dynamics of soil C in its subsoil ...layers are not clearly understood. Here, we compiled data from 78 sites (in total 122 published studies) to examine the effects of varying grazing intensities and durations on soil C content at different depths for grasslands in China. Our meta‐analysis revealed that grazing led to an overall decrease in soil C content and productivity of above‐ground vegetation (e.g., above‐ground biomass and litter) but an increase in below‐ground biomass. Specifically, the effects of grazing on soil C content became less negative or even positive with increasing soil depths. An increase of soil C content was consequently found under light grazing (LG), although soil C content still decreased under moderate and heavy grazing. The increase in soil C content under LG could be largely attributed to the increase of soil C content in subsoil layers (>20 cm), despite that soil C content in surface soil layer (0–20 cm) decreased. Moreover, the magnitude of increase in soil C content under LG in subsoil layers increased with grazing duration. A possible reason of the increase in soil C content in the subsoil layers was due to the increases in below‐ground biomass. Our study highlights that LG may modify the allocation of C input and promote its accumulation in subsoil layers, thus offsetting the negative impact of grazing on surface soil C content, a finding that has significant implications for C sequestration in grasslands.
Light grazing (LG) increased the soil C content (SCC) owing to its positive effect on SCC in subsoil layers (>20 cm), although its effect in the surface soil layer (0–20 cm) was negative. A possible reason is that LG may promote the below‐ground biomass (BGB) in subsoil layers (>20 cm), offsetting the negative impact on above‐ground biomass (AGB) and litter. Blue downward pointing arrows represent decrease and red upward pointing arrows represent increase in the variables. SWC: soil water content.
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BFBNIB, FZAB, GIS, IJS, KILJ, NLZOH, NUK, OILJ, SBCE, SBMB, UL, UM, UPUK
Superlubricity of graphite and graphene has aroused increasing interest in recent years. Yet how to obtain a long-lasting superlubricity between graphene layers, under high applied normal load in ...ambient atmosphere still remains a challenge but is highly desirable. Here, we report a direct measurement of sliding friction between graphene and graphene, and graphene and hexagonal boron nitride (h-BN) under high contact pressures by employing graphene-coated microsphere (GMS) probe prepared by metal-catalyst-free chemical vapour deposition. The exceptionally low and robust friction coefficient of 0.003 is accomplished under local asperity contact pressure up to 1 GPa, at arbitrary relative surface rotation angles, which is insensitive to relative humidity up to 51% RH. This ultralow friction is attributed to the sustainable overall incommensurability due to the multi-asperity contact covered with randomly oriented graphene nanograins. This realization of microscale superlubricity can be extended to the sliding between a variety of two-dimensional (2D) layers.
Embedding metal species into zeolite frameworks can create framework-bond metal sites in a confined microenvironment. The metals sitting in the specific T sites of zeolites and their crystalline ...surroundings are both committed to the interaction with the reactant, participation in the activation, and transient state achievement during the whole catalytic process. Herein, we construct isolated Co-motifs into purely siliceous MFI zeolite frameworks (Co-MFI) and reveal the location and microenvironment of the isolated Co active center in the MFI zeolite framework particularly beneficial for propane dehydrogenation (PDH). The isolated Co-motif with the distorted tetrahedral structure ({(SiO)2Co(HO–Si)2}, two Co–O–Si bonds, and two pseudobridging hydroxyls (Co···OH–Si) is located at T1(7) and T3(9) sites of the MFI zeolite. DFT calculations and deuterium-labeling reactions verify that the isolated Co-motif together with the MFI microenvironment collectively promotes the PDH reaction by providing an exclusive microenvironment to preactivate C3H8, polarizing the oxygen in Co–O–Si bonds to accept H* ({(SiO)CoHδ− (Hδ+O–Si)3}), and a scaffold structure to stabilize the C3H7* intermediate. The Co-motif active center in Co-MFI goes through the dynamic evolutions and restoration in electronic states and coordination states in a continuous and repetitive way, which meets the requirements from the series of elementary steps in the PDH catalytic cycle and fulfills the successful catalysis like enzyme catalysis.
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IJS, KILJ, NUK, PNG, UL, UM
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Sulfonamides as the major antibiotic have become emerging contaminants worldwide in aquatic environments. Herein, a heterogeneous Fenton-like oxidation driven by a novel BF-PMCs ...bismuth ferrites reported firstly for efficient degradation of sulfamethoxazole (SMX) in which the possible degradation pathways are thoroughly analyzed through identifying some of key intermediates (i.e., C8H11N3O4S, C4H4NO2, etc.) using liquid chromatography-mass spectrum (LC-MS), monitoring organic acids (i.e., acetic acid, pyruvic acid) and inorganic anions (i.e., sulfate, nitrate) using ion chromatography (IC), and detecting radical species (i.e., HO) using both chemical quenchers and fluorescence technique, simultaneously. The optimal operations in BF-PMCs/H2O2 system for SMX degradation are recommended at the conditions of initial pH ~4.5, 1.5 mg L−1 SMX, 70 mM H2O2, and BF-PMCs loading of 0.2 g L−1. The degradation rates (kinetic value of kapp) for SMX, azoxystrobin, bisphenol A, and 2,4-dichlorophenol are 9.5 × 10−3, 13.6 × 10−3, 7.3 × 10−3, and 5.9 × 10−3 min−1, respectively. Meanwhile, the degradation rates in BF-PMCs/H2O2 system for SMX degradation are slightly slower in the presence of inorganic anions (e.g., Cl−, NO3−) and NOM (e.g., humic acid). Based on an overall consideration, the BF-PMCs/H2O2 system has great potential for degradation of emerging organic pollutants (EOPs) in natural water systems.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
Chromatin dynamics regulated by epigenetic modification is crucial in genome stability and gene expression. Various epigenetic mechanisms have been identified in the pathogenesis of human diseases. ...Here, we examined the effects of ten epigenetic agents on pseudorabies virus (PRV) infection by using GFP-reporter assays. Inhibitors of bromodomain protein 4 (BRD4), which receives much more attention in cancer than viral infection, was found to exhibit substantial anti-viral activity against PRV as well as a range of DNA and RNA viruses. We further demonstrated that BRD4 inhibition boosted a robust innate immune response. BRD4 inhibition also de-compacted chromatin structure and induced the DNA damage response, thereby triggering the activation of cGAS-mediated innate immunity and increasing host resistance to viral infection both in vitro and in vivo. Mechanistically, the inhibitory effect of BRD4 inhibition on viral infection was mainly attributed to the attenuation of viral attachment. Our findings reveal a unique mechanism through which BRD4 inhibition restrains viral infection and points to its potent therapeutic value for viral infectious diseases.
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DOBA, IZUM, KILJ, NUK, PILJ, PNG, SAZU, SIK, UILJ, UKNU, UL, UM, UPUK
The Newtonian gravitational constant, G, is one of the most fundamental constants of nature, but we still do not have an accurate value for it. Despite two centuries of experimental effort, the value ...of G remains the least precisely known of the fundamental constants. A discrepancy of up to 0.05 per cent in recent determinations of G suggests that there may be undiscovered systematic errors in the various existing methods. One way to resolve this issue is to measure G using a number of methods that are unlikely to involve the same systematic effects. Here we report two independent determinations of G using torsion pendulum experiments with the time-of-swing method and the angular-acceleration-feedback method. We obtain G values of 6.674184 × 10
and 6.674484 × 10
cubic metres per kilogram per second squared, with relative standard uncertainties of 11.64 and 11.61 parts per million, respectively. These values have the smallest uncertainties reported until now, and both agree with the latest recommended value within two standard deviations.
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KISLJ, NUK, SBMB, UL, UM, UPUK