The interactions between aerosols, clouds, and precipitation remain among the largest sources of uncertainty in the Earth's energy budget. Biomass-burning aerosols are a key feature of the global ...aerosol system, with significant annually-repeating fires in several parts of the world, including Southeast Asia (SEA). SEA in particular provides a "natural laboratory" for these studies, as smoke travels from source regions downwind in which it is coupled to persistent stratocumulus decks. However, SEA has been under-exploited for these studies. This review summarizes previous related field campaigns in SEA, with a focus on the ongoing Seven South East Asian Studies (7-SEAS) and results from the most recent BASELInE deployment. Progress from remote sensing and modeling studies, along with the challenges faced for these studies, are also discussed. We suggest that improvements to our knowledge of these aerosol/cloud effects require the synergistic use of field measurements with remote sensing and modeling tools.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UL, UM, UPCLJ, UPUK
Nonuniform beam filling (NUBF) within an atmospheric radar sampling volume can cause significant Doppler velocity errors when the radar is located on a fast-moving platform. A case of strong NUBF ...errors was identified in ER-2 X-band Radar (EXRAD) data from the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) 2020 field campaign. A basic NUBF correction was employed using an estimate of the along-track radar reflectivity gradient. The relationship is verified empirically using colocated Doppler velocity measurements from the higher resolution cloud radar system (CRS).
Initial droplet spectra produced upon activation impact the ensuing chain of microphysical processes and therefore play a crucial role in cloud evolution. This work re-examines dependencies of newly ...formed cloud droplet size distribution (CDSD) characteristics on environmental and aerosol properties via parcel model simulations that serve as the basis for a multi-moment bulk microphysics droplet activation scheme suitable for a cloud-resolving model (CRM). It is found that applying a fixed size threshold to define activated droplets versus employing physical considerations can lead to erroneous activation and overly broad CDSDs for high aerosol concentration and weak updraft conditions. Aerosol distributions characterized by larger median sizes and/or increased solubility can result in greater activated droplet numbers, whereas impacts of these parameters on CDSD spectral width depend on both aerosol number concentration and updraft velocity. An expansion of the activation scheme to include CDSD spectral width is proposed to aid efforts to extend high-order moment prediction to cloud droplet categories in CRMs as well as better represent variability in the activation process on the cloud scale.
•Cloud droplet definition impacts newly activated droplet spectra characteristics.•Activated droplet spectra sensitivity to aerosol size depends on activation regime.•Spectral width of activated droplet spectrum attainable via look-up table approach.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UL, UM, UPCLJ, UPUK, ZRSKP
The objectives of 7-SEASBASELInE (Seven SouthEast Asian Studies Biomass-burning Aerosols and Stratocumulus Environment: Lifecycles and Interactions Experiment) campaigns in spring 2013-2015 were to ...synergize measurements from uniquely distributed ground-based networks (e.g., AERONET (AErosol RObotic NETwork)), MPLNET ( NASA Micro-Pulse Lidar Network)) and sophisticated platforms (e.g.,SMARTLabs (Surface-based Mobile Atmospheric Research and Testbed Laboratories), regional contributing instruments), along with satellite observations retrievals and regional atmospheric transport chemical models to establish a critically needed database, and to advance our understanding of biomass-burning aerosols and trace gases in Southeast Asia (SEA). We present a satellite-surface perspective of 7-SEASBASELInE and highlight scientific findings concerning: (1) regional meteorology of moisture fields conducive to the production and maintenance of low-level stratiform clouds over land; (2) atmospheric composition in a biomass-burning environment, particularly tracers-markers to serve as important indicators for assessing the state and evolution of atmospheric constituents; (3) applications of remote sensing to air quality and impact on radiative energetics, examining the effect of diurnal variability of boundary-layer height on aerosol loading; (4) aerosol hygroscopicity and ground-based cloud radar measurements in aerosol-cloud processes by advanced cloud ensemble models; and (5) implications of air quality, in terms of toxicity of nanoparticles and trace gases, to human health. This volume is the third 7-SEAS special issue (after Atmospheric Research, vol. 122, 2013; and Atmospheric Environment, vol. 78, 2013) and includes 27 papers published, with emphasis on air quality and aerosol-cloud effects on the environment. BASELInE observations of stratiform clouds over SEA are unique, such clouds are embedded in a heavy aerosol-laden environment and feature characteristically greater stability over land than over ocean, with minimal radar surface clutter at a high vertical spatial resolution. To facilitate an improved understanding of regional aerosol-cloud effects, we envision that future BASELInE-like measurement modeling needs fall into two categories: (1) efficient yet critical in-situ profiling of the boundary layer for validating remote-sensing retrievals and for initializing regional transport chemical and cloud ensemble models; and (2) fully utilizing the high observing frequencies of geostationary satellites for resolving the diurnal cycle of the boundary layerheight as it affects the loading of biomass-burning aerosols, air quality and radiative energetics.
The spring 2015 deployment of a suite of instrumentation at Doi Ang Khang (DAK) in northwestern Thailand enabled the characterization of air masses containing smoke aerosols from burning ...predominantly in Myanmar. Aerosol Robotic Network (AERONET) Sun photometer data were used to validate Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6 "Deep Blue" aerosol optical depth (AOD) retrievals; MODIS Terra and Aqua provided results of similar quality, with correlation coefficients of 0.93-0.94 and similar agreement within expected uncertainties to global-average performance. Scattering and absorption measurements were used to compare surface and total column aerosol single scatter albedo (SSA); while the two were well-correlated, and showed consistent positive relationships with moisture (increasing SSA through the season as surface relative humidity and total columnar water vapor increased), in situ surface-level SSA was nevertheless significantly lower by 0.12-0.17. This could be related to vertical heterogeneity and/or instrumental issues. DAK is at approximately 1,500 meters above sea level in heterogeneous terrain, and the resulting strong diurnal variability in planetary boundary layer depth above the site leads to high temporal variability in both surface and column measurements, and acts as a controlling factor to the ratio between surface particulate matter (PM) levels and column AOD. In contrast, while some hygroscopic effects were observed relating to aerosol particle size and Angstrom exponent, relative humidity variations appear to be less important for this ratio here. As part of the Seven South-East Asian Studies (7-SEAS) project, the Biomass-burning Aerosols & Stratocumulus Environment: Lifecycles and Interactions Experiment (BASELInE) was intended to probe physicochemical processes, interactions, and feedbacks related to biomass burning aerosols and clouds during the spring burning season (February-April) in southeast Asia (SEA).
The transport of aerosols relies primarily upon air flow for conveyance; however, the air flow pattern is dominated by large-scale circulation conditions. One mission of the 2013 7-SEAS/BASELInE ...(Seven SouthEast Asian Studies/Biomassburning Aerosols ＆ Stratocumulus Environment: Lifecycles and Interactions Experiment) was to capture/confirm the downwind effect on the surface air quality due to the long-range transport of Southeast Asia biomass-burning (SEA BB) pollutants. This phenomenon was first discovered during the 2010 Dongsha experiment and directly observed by a lidar system at Hengchun in southern Taiwan during 7-SEAS/BASELInE. Through three-dimensional structural analysis, it was found that the sinking motion behind the upper-level active short wave trough is the major mechanism that enhances subsidence along the cold surge leading edge. In turn, the enhanced subsidence could bring the long-range transport of the SEA BB pollutants down to the surface. Furthermore, the HYSPLIT backward air trajectories helped identify the SEA BB pollutants in the mid-troposphere, while the fine-resolution WRF model simulation combined with dual-polarization lidar observations demonstrated the evolution of the brought-down aerosols process. An additional significant finding of this study is that the upper-level ridge-trough short wave within 20°-35°N was very active during spring 2013, highlighting the inter-annual variability of the long-range transport of SEA BB pollutants.
Abstract
Two methods designed to parameterize mesoscale ascent in a three-dimensional numerical cloud model via near-surface momentum and heat fluxes are presented and compared to the commonly used ...technique of an initial perturbation placed within the model initial condition. The flux techniques use a continuously reinforced thermal or convergent low-level wind field to produce upward vertical motion on the order of 10 cm s−1, by which deep, moist convection can be initiated. The sensitivity of the convective response to the type, strength, and size of the forcing is evaluated using numerical simulations of a conditionally unstable environment with weak unidirectional shear. Precipitation-free cloud processes are used to further simplify the model response to the forcing. The three methods tested produce an initial convective response, but only the momentum and heat flux methods are able to produce sustained deep convection that approximately resembles isolated multicellular convection. Cell regeneration periods, defined as the elapsed time between subsequent vertical velocity maxima passing through a constant level in the updraft region above the source, vary from 8 to 25 min, depending on the forcing type, magnitude, and geometry.
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DOBA, IZUM, KILJ, NUK, PILJ, PNG, SAZU, UILJ, UKNU, UL, UM, UPUK
The 2013 7-SEASBASELInE campaign over northern Southeast Asia (SEA) provided, for the first time ever, comprehensive ground-based W-band radar measurements of the low-level stratocumulus (Sc) systems ...that often exist during the spring over northern Vietnam in the presence of biomass-burning aerosols. Although spatially limited, ground-based remote sensing observations are generally free of the surface contamination and signal attenuation effects that often hinder space-borne measurements of these low-level cloud systems. Such observations permit detailed measurements of structures and lifecycles of these clouds as part of a broader effort to study potential impacts of these coupled aerosol-cloud systems on local and regional weather and air quality. Introductory analyses of the W-band radar data show these Sc systems generally follow a diurnal cycle, with peak occurrences during the nighttime and early morning hours, often accompanied by light precipitation. Preliminary results from idealized simulations of Sc development over land based on the observations reveal the familiar response of increased numbers and smaller sizes of cloud droplets, along with suppressed drizzle formation, as aerosol concentrations increase. Slight reductions in simulated W-band reflectivity values also are seen with increasing aerosol concentrations and result primarily from decreased droplet sizes. As precipitation can play a large role in removing aerosol from the atmosphere, and thereby improving air quality locally, quantifying feedbacks between aerosols and cloud systems over this region are essential, particularly given the negative impacts of biomass burning on human health in SEA. Such an endeavor should involve improved modeling capabilities along with comprehensive measurements of time-dependent aerosol and cloud profiles.
Aerosol optical thickness (τaer) is a fundamental parameter for analyzing aerosol loading and associated radiative effects. The τaer can constrain many inversion algorithms using passive/active ...sensor measurements to retrieve other aerosol properties and/or the abundance of trace gases. In the next wave of spectroradiometric observations from geostationary platforms, we envision that a strategically distributed network of robust, well‐calibrated ground‐based spectroradiometers will comprehensively complement spaceborne measurements in spectral and temporal domains. Spectral τaer can be accurately obtained from direct‐Sun measurements based on the Langley calibration method, which allows for the analysis of distinct spectral features of the calibration results. In this study, we present a spectral τaer retrieval algorithm for an in‐house developed, field deployable spectroradiometer instrument covering wavelengths from ultraviolet to near‐infrared (UV‐Vis‐NIR). The spectral total optical thickness obtained from the Langley calibration method is partitioned into molecular and particulate components by utilizing a least squares method. The resulting high temporal‐resolution τaer and Ångström Exponent can be used effectively for cloud screening. The new algorithm was applied to month‐long measurements acquired from the rooftop at National Aeronautics and Space Administration Goddard Space Flight Center's Building 33. The retrieved τaer demonstrated excellent agreement with those from well‐calibrated Aerosol Robotic Network Sun photometers at all overlapping wavelengths (correlation coefficients higher than 0.98). In addition, empirical stray light corrections considerably improved τaer retrievals at short wavelengths in the UV. The continuous spectrum of τaer from UV‐Vis‐NIR spectroradiometers is expected to provide more informative constraints for retrieval of additional aerosol properties such as refractive indices, size, and bulk vertical distribution.
Key Points
Spectral aerosol optical thickness retrieval algorithm was developed based on the Langley calibration method
Developed empirical stray light correction method considerably improved aerosol optical thickness retrievals at ultraviolet wavelengths
Retrieved spectral aerosol optical thickness provides the key constraints for additional aerosol properties and trace gas retrievals
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BFBNIB, FZAB, GIS, IJS, KILJ, NLZOH, NUK, OILJ, SBCE, SBMB, UL, UM, UPUK
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