A newly assembled multi-reflection time-of-flight mass spectrograph (MRTOF-MS) at RIKEN’s RIBF facility became operational for the first time in spring 2020; further modifications and performance ...tests using stable ions were completed in early 2021. By using a pulsed-drift-tube technique to modify the ions’ kinetic energy in a wide range, we directly characterize the dispersion function of the system for use in a new procedure for optimizing the voltages applied to the electrostatic mirrors. Thus far, a mass resolving power of Rm>1000000 is reached within a total time-of-flight of only 12.5ms, making the spectrometer capable of studying short-lived nuclei possessing low-lying isomers. Detailed information about the setup and measurement procedure is reported, and an alternative in-MRTOF ion selection scheme to remove molecular contaminants in the absence of a dedicated deflection device is introduced. The setup underwent an initial on-line commissioning at the BigRIPS facility at the end of 2020, where more than 70 nuclear masses have been measured. A summary of the commissioning experiments and results from a test of mass accuracy will be presented.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
The Rare-RI Ring (R3) is a recently commissioned cyclotronlike storage ring mass spectrometer dedicated to mass measurements of exotic nuclei far from stability at Radioactive Isotope Beam Factory ...(RIBF) in RIKEN. The first application of mass measurement using the R3 mass spectrometer at RIBF is reported. Rare isotopes produced at RIBF-^{127}Sn, ^{126}In, ^{125}Cd, ^{124}Ag, ^{123}Pd-were injected in R3. Masses of ^{126}In, ^{125}Cd, and ^{123}Pd were measured whereby the mass uncertainty of ^{123}Pd was improved. This is the first reported measurement with a new storage ring mass spectrometry technique realized at a heavy-ion cyclotron and employing individual injection of the preidentified rare nuclei. The latter is essential for the future mass measurements of the rarest isotopes produced at RIBF. The impact of the new ^{123}Pd result on the solar r-process abundances in a neutron star merger event is investigated by performing reaction network calculations of 20 trajectories with varying electron fraction Y_{e}. It is found that the neutron capture cross section on ^{123}Pd increases by a factor of 2.2 and β-delayed neutron emission probability, P_{1 n}, of ^{123}Rh increases by 14%. The neutron capture cross section on ^{122}Pd decreases by a factor of 2.6 leading to pileup of material at A=122, thus reproducing the trend of the solar r-process abundances. The trend of the two-neutron separation energies (S_{2n}) was investigated for the Pd isotopic chain. The new mass measurement with improved uncertainty excludes large changes of the S_{2n} value at N=77. Such large increase of the S_{2n} values before N=82 was proposed as an alternative to the quenching of the N=82 shell gap to reproduce r-process abundances in the mass region of A=112-124.
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We performed the first direct mass measurements of neutron-rich scandium, titanium, and vanadium isotopes around the neutron number 40 at the RIKEN RI Beam Factory using the time-of-flight ...magnetic-rigidity technique. The atomic mass excesses of 58−60Sc, 60−62Ti, and 62−64V were measured for the first time. The experimental results show that the two-neutron separation energies in the vicinity of 62Ti increase compared to neighboring nuclei. This shows that the masses of Ti isotopes near N = 40 are affected by the Jahn-Teller effect. Therefore, a development of Jahn-Teller stabilization appears below the Cr isotopes, and the systematics in Sc, Ti, and V isotopes suggest that 62Ti is located close to the peak of the Jahn-Teller effect.
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The atomic masses of ^{55}Sc, ^{56,58}Ti, and ^{56-59}V have been determined using the high-precision multireflection time-of-flight technique. The radioisotopes have been produced at RIKEN's ...Radioactive Isotope Beam Factory (RIBF) and delivered to the novel designed gas cell and multireflection system, which has been recently commissioned downstream of the ZeroDegree spectrometer following the BigRIPS separator. For ^{56,58}Ti and ^{56-59}V, the mass uncertainties have been reduced down to the order of 10 keV, shedding new light on the N=34 shell effect in Ti and V isotopes by the first high-precision mass measurements of the critical species ^{58}Ti and ^{59}V. With the new precision achieved, we reveal the nonexistence of the N=34 empirical two-neutron shell gaps for Ti and V, and the enhanced energy gap above the occupied νp_{3/2} orbit is identified as a feature unique to Ca. We perform new Monte Carlo shell model calculations including the νd_{5/2} and νg_{9/2} orbits and compare the results with conventional shell model calculations, which exclude the νg_{9/2} and the νd_{5/2} orbits. The comparison indicates that the shell gap reduction in Ti is related to a partial occupation of the higher orbitals for the outer two valence neutrons at N=34.
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γ emission probabilities from unbound states in 78,80Se, populated by a neutron-transfer reaction (d,p) on 77,79Se nuclei in inverse kinematics, were measured by directly detecting reaction residues. ...Assuming the spin distribution at the respective excitation energy of the unbound state, the cross-sections of the 79Se(n,γ)80Se reaction were evaluated using the γ emission probabilities. The surrogate-ratio method with the experimental γ emission probabilities of 78,80Se was also employed to deduce the cross-sections of 79Se(n,γ) reaction by incorporating the theoretical evaluations of the neutron-capture reaction on the isomeric state in 77Se. Our two cross-sections are in good agreement with existing nuclear data compilations for the neutron-capture reaction on 79Se. The presented method contributes to the body of existing knowledge by providing approaches for determining the neutron capture cross-sections of radioactive nuclei at various neutron energies.
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GEOZS, IJS, IMTLJ, KILJ, KISLJ, NLZOH, NUK, OILJ, PNG, SAZU, SBCE, SBJE, UILJ, UL, UM, UPCLJ, UPUK, ZAGLJ, ZRSKP
We perform the first direct mass measurements of neutron-rich calcium isotopes beyond neutron number 34 at the RIKEN Radioactive Isotope Beam Factory by using the time-of-flight magnetic-rigidity ...technique. The atomic mass excesses of 55–57Ca are determined for the first time to be −18650(160), −13510(250), and −7370(990) keV, respectively. We examine the emergence of neutron magicity at N = 34 based on the new atomic masses. The new masses provide experimental evidence for the appearance of a sizable energy gap between the neutron 2p1/2 and 1f5/2 orbitals in 54 Ca , comparable to the gap between the neutron 2p3/2 and 2p1/2 orbitals in 52Ca. For the 56Ca nucleus, an open-shell property in neutrons is suggested.
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Neutron-rich Pm (Z=61) isotopes were studied by delayed γ-ray spectroscopy at RIBF, RIKEN Nishina Center using the in-flight fission of a 345 MeV/nucleon 238U beam. A cluster-type Ge detector array, ...EURICA, was used to measure the delayed γ rays from stopped ions. Isomeric γ decays were observed in 159Pm and 161Pm with half-lives of 4.97(12) μs and 0.79(4) μs, respectively. Level schemes for 159Pm and 161Pm were constructed in this study. The isomeric states of 159Pm and 161Pm could be interpreted as two quasiparticle excitations of neutrons with the configurations of ν(7/2633⊗5/2523) and ν(7/2633⊗1/2521), respectively. They are analogous to the isomers that have been observed systematically in other even-mass N=98 and N=100 isotones in this region. A projected shell model calculation was performed and it reproduced the order of three-quasiparticle states only if new Nilsson parameters with an N-dependent spin-orbit interaction were used. This work demonstrates that the strength of spin-orbit interactions in standard Nilsson parameters needs to be modified to study the properties of neutron-rich rare-earth nuclei around A=165, and provides new evidence supporting the existence of the deformed N=98 subshell gap in odd-mass nuclei for the first time.
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