The title compound crystallizes in the monoclinic space group P21/n with a = 8.706(1), b = 9.192(1), c = 15.261(2) Å, β = 94.740(3)°, V = 1217.0(3) Å3, Z = 4, Dcalc = 2.278 g cm–3. The ...tris(imidazolyl)borate ligand bridges between three thallium atoms. The structure consists of one‐dimensional twisted ladder‐like strands.
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