Cobalt(III)‐Catalyzed Aerobic Diamination of α‐Alkyl Styrenes with Anilines

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Cobalt(III)‐Catalyzed Aerobic Diamination of α‐Alkyl Styrenes with Anilines

Yang, Jinglei; Wu, Yun‐Dong; Pu, Maoping

Advanced synthesis & catalysis, July 18, 2023, Volume: 365, Issue: 14

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A commercially available cobalt complex Cp*CoIII(CO)I2 has been found to effectively catalyze the diamination of α‐alkyl styrenes with anilines under a mild reaction condition, using dioxygen as the oxidant. This reaction features a reasonably good substrate scope of amines and a good functional group tolerance. Preliminary mechanistic studies have shown that Cp*CoIII(CO)I2 alone can promote the diamination reaction.

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Yang, Jinglei | Wu, Yun‐Dong | Pu, Maoping

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