Total Synthesis of Polyene Natural Product Dihydroxerulin by Mild Organocatalyzed Dehydrogenation of Alcohols

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Total Synthesis of Polyene Natural Product Dihydroxerulin by Mild Organocatalyzed Dehydrogenation of Alcohols

Xie, Hexin; Zhang, Shilei; Li, Hao; Zhang, Xinshuai; Zhao, Sihan; Xu, Zian; Song, Xixi; Yu, Xinhong; Wang, Wei

Chemistry : a European journal, February 20, 2012, Volume: 18, Issue: 8

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Polyene synthesis: An efficient approach to the total synthesis of polyene natural product dihydroxrulin (1) is described. A novel, mild, direct organocatalytic IBX‐mediated dehydrogenation process of simple alcohols to enals has been developed, which serves as a key step in the synthesis (see scheme).

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