This study describes a novel sample preparation and assay method developed, primarily in support of the Majorana Demonstrator neutrinoless double-beta decay experiment, for the determination of ...extremely low levels of Th and U in copper and lead shielding components. Meticulously clean sample preparation methods combined with anion exchange separations for analyte pre-concentration and matrix removal were developed. Quantification was performed by isotope dilution inductively coupled plasma mass spectrometry. Detection limits of 0.0084 pg 232Th/g (0.034µBq 232Th/kg) and 0.0106 pg 238U/g (0.131µBq 238U/kg) were determined for copper, while detection limits of 0.23 pg 232Th/g (0.94µBq 232Th/kg) and 0.46 pg 238U/g (5.7µBq 238U/kg) were achieved for lead. These methods allow the Majorana Collaboration to accurately assay detector components and ensure that the experiment׳s stringent radiopurity requirements are met.
New data are reported from a second run of the 2-liter PICO-2L C sub(3) F sub(8) bubble chamber with a total exposure of 129 kg-days at a thermodynamic threshold energy of 3.3 keV. These data show ...that measures taken to control particulate contamination in the superheated fluid resulted in the absence of the anomalous background events observed in the first run of this bubble chamber. One single nuclear-recoil event was observed in the data, consistent both with the predicted background rate from neutrons and with the observed rate of unambiguous multiple-bubble neutron scattering events. The chamber exhibits the same excellent electron-recoil and alpha decay rejection as was previously reported. These data provide the most stringent direct detection constraints on weakly interacting massive particle (WIMP)-proton spin-dependent scattering to date for WIMP masses <50GeV/c super(2).
The performance of LSC cocktails in ultra-sensitive applications was evaluated. Backgrounds from radioactive contaminations in commercially available and in-house developed liquid scintillation ...cocktails were measured and compared to the predicted background levels of the ultra-low background liquid scintillation counter. Through the ICP-MS assay of the cocktails and their constituents, potassium impurities in the surfactant component were identified as a significant source of background, potentially limiting the use of LSC counting in ultra-sensitive applications. This work lays the groundwork for future research towards ultrapure LSC cocktails for ultrasensitive LSC counting.
Intrinsic
40
K radioactive backgrounds from impurities of natural K in liquid scintillation cocktails have previously been demonstrated to limit their use in ultra-sensitive applications. This work ...explores two methodologies in parallel for the reduction of
40
K backgrounds in the cocktails, and lays the groundwork for use in ultra-sensitive applications. In one method, alternative low-K liquid scintillation matrix constituents were identified and in the other, a simple purification method for single components and finished cocktails was developed. Both methods were verified via ICP-MS analysis. Liquid scintillation counting of selected purified cocktails demonstrated background reduction, improved stability, and enhanced performance. The best performing purified cocktail was also counted on a custom-built ultra-low background liquid scintillation counter, with results below the detector background.
Radioactive contaminants on the surfaces of detector components can be a problematic source of background events for physics experiments searching for rare processes. Exposure to radon is a specific ...concern because it can result in the relatively long-lived 210Pb (and progeny) being implanted to significant subsurface depths such that removal is challenging. In this article we present results from a broad exploration of cleaning treatments to remove implanted 210Pb and 210Po contamination from silicon, which is a material frequently used in rare-events searches. We demonstrate for the first time that heat treatments (“baking”) can effectively mitigate such surface contamination, with a 1200 °C bake resulting in a 97−3+2% reduction. We also report results using wet-chemistry and plasma-based methods, which show that etching can be highly effective provided the etch depth is sufficiently aggressive. Our survey of cleaning methods suggests consideration of multiple approaches during the different phases of detector construction to enable greater flexibility for efficient removal of 210Pb and 210Po surface contamination.
Many compelling models predict dark matter coupling to the electromagnetic current through higher multipole interactions, while remaining electrically neutral. Different multipole couplings have been ...studied, among them anapole moment, electric and magnetic dipole moments, and millicharge. This study sets limits on the couplings for these photon-mediated interactions using nonrelativistic contact operators in an effective field theory framework. Using data from the PICO-60 bubble chamber leading limits for dark matter masses between 2.7 and 24 GeV/c2 and above 265 GeV/c2 (anapole moment), 2.7 and 11.7 GeV/c2 (electric moment), 3 and 9.5 GeV/c2 (magnetic moment), and 2.7 and 12 GeV/c2 (millicharged) are reported for the coupling of these photon-mediated dark matter-nucleus interactions. The detector was filled with 52 kg of C3F8 operating at thermodynamic thresholds of 2.45 keV and 3.29 keV, reaching exposures of 1404 kg-day and 1167 kg-day, respectively.
The bubble nucleation efficiency of low-energy nuclear recoils in superheated liquids plays a crucial role in interpreting results from direct searches for weakly interacting massive particle (WIMP) ...dark matter. Here, the PICO collaboration presents the results of the efficiencies for bubble nucleation from carbon and fluorine recoils in superheated C3F8 from calibration data taken with five distinct neutron spectra at various thermodynamic thresholds ranging from 2.1 to 3.9 keV. Instead of assuming any particular functional forms for the nuclear recoil efficiency, a generalized piecewise linear model is proposed with systematic errors included as nuisance parameters to minimize model-introduced uncertainties. A Markov chain Monte Carlo routine is applied to sample the nuclear recoil efficiency for fluorine and carbon at 2.45 and 3.29 keV thermodynamic thresholds simultaneously. The nucleation efficiency for fluorine was found to be ≥ 50% for nuclear recoils of 3.3 keV (3.7 keV) at a thermodynamic Seitz threshold of 2.45 keV (3.29 keV), and for carbon the efficiency was found to be ≥ 50% for recoils of 10.6 keV (11.1 keV) at a threshold of 2.45 keV (3.29 keV). Simulated datasets are used to calculate a p value for the fit, confirming that the model used is compatible with the data. The fit paradigm is also assessed for potential systematic biases, which although small, are corrected for. Additional steps are performed to calculate the expected interaction rates of WIMPs in the PICO-60 detector, a requirement for calculating WIMP exclusion limits.
Ultra-pure NaI(Tl) crystals are the key element for a model-independent verification of the long standing DAMA result and a powerful means to search for the annual modulation signature of dark matter ...interactions. The SABRE collaboration has been developing cutting-edge techniques for the reduction of intrinsic backgrounds over several years. In this paper we report the first characterization of a 3.4 kg crystal, named NaI-33, performed in an underground passive shielding setup at LNGS. NaI-33 has a record low
39
K contamination of 4.3 ± 0.2 ppb as determined by mass spectrometry. We measured a light yield of 11.1 ± 0.2 photoelectrons/keV and an energy resolution of 13.2% (FWHM/E) at 59.5 keV. We evaluated the activities of
226
Ra and
228
Th inside the crystal to be
5.9
±
0.6
μ
Bq/kg and
1.6
±
0.3
μ
Bq/kg, respectively, which would indicate a contamination from
238
U and
232
Th at part-per-trillion level. We measured an activity of 0.51 ± 0.02 mBq/kg due to
210
Pb out of equilibrium and a
α
quenching factor of 0.63 ± 0.01 at 5304 keV. We illustrate the analyses techniques developed to reject electronic noise in the lower part of the energy spectrum. A cut-based strategy and a multivariate approach indicated a rate, attributed to the intrinsic radioactivity of the crystal, of
∼
1 count/day/kg/keV in the 5–20 keV region.
Celotno besedilo
Dostopno za:
DOBA, IZUM, KILJ, NUK, PILJ, PNG, SAZU, SIK, UILJ, UKNU, UL, UM, UPUK
Dust particulate fallout on materials in use for rare-event searches is a concerning source of radioactive backgrounds due to the presence of the naturally occurring radionuclides 40K, 232Th, 238U, ...and their progeny in dust. Much effort is dedicated to inform radioactive backgrounds from dust and evaluate the efficacy of mitigation procedures. A great portion of such effort relies on fallout models and assumed dust composition. In this work, an ICP-MS based methodology was employed for a direct determination of fallout rates of radionuclides and stable isotopes of interest from dust particulate at the SNOLAB facility. Hosted in an active mine, the SNOLAB underground laboratory strives to maintain experimental areas at class 2000 cleanroom level. This work validates the mitigation procedures in place at SNOLAB and informs dust backgrounds during laboratory activities. Fallout rates of major constituents of the local rock were measured two to three orders of magnitude lower in the clean experimental areas compared to non-clean transition areas from the mine to the laboratory. An increase of approximately two orders of magnitude in the fallout rate of stable Pb isotopes was determined in an experimental area during activities involving handling of Pb bricks. Increased 40K, 232Th, and 238U fallout rates were measured in clean experimental areas during activities generating particulate.
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