Abstract
The tin isotope
100
Sn is of singular interest for nuclear structure due to its closed-shell proton and neutron configurations. It is also the heaviest nucleus comprising protons and ...neutrons in equal numbers—a feature that enhances the contribution of the short-range proton–neutron pairing interaction and strongly influences its decay via the weak interaction. Decay studies in the region of
100
Sn have attempted to prove its doubly magic character
1
but few have studied it from an ab initio theoretical perspective
2,3
, and none of these has addressed the odd-proton neighbours, which are inherently more difficult to describe but crucial for a complete test of nuclear forces. Here we present direct mass measurements of the exotic odd-proton nuclide
100
In, the beta-decay daughter of
100
Sn, and of
99
In, with one proton less than
100
Sn. We use advanced mass spectrometry techniques to measure
99
In, which is produced at a rate of only a few ions per second, and to resolve the ground and isomeric states in
101
In. The experimental results are compared with ab initio many-body calculations. The 100-fold improvement in precision of the
100
In mass value highlights a discrepancy in the atomic-mass values of
100
Sn deduced from recent beta-decay results
4,5
.
The recently confirmed neutron-shell closure at N=32 has been investigated for the first time below the magic proton number Z=20 with mass measurements of the exotic isotopes (52,53)K, the latter ...being the shortest-lived nuclide investigated at the online mass spectrometer ISOLTRAP. The resulting two-neutron separation energies reveal a 3 MeV shell gap at N=32, slightly lower than for 52Ca, highlighting the doubly magic nature of this nuclide. Skyrme-Hartree-Fock-Bogoliubov and ab initio Gorkov-Green function calculations are challenged by the new measurements but reproduce qualitatively the observed shell effect.
Masses adjacent to the classical waiting-point nuclide Cd130 have been measured by using the Penning-trap spectrometer ISOLTRAP at ISOLDE/CERN. We find a significant deviation of over 400 keV from ...earlier values evaluated by using nuclear beta-decay data. The new measurements show the reduction of the N=82 shell gap below the doubly magic Sn132. The nucleosynthesis associated with the ejected wind from type-II supernovae as well as from compact object binary mergers is studied, by using state-of-the-art hydrodynamic simulations. We find a consistent and direct impact of the newly measured masses on the calculated abundances in the A=128-132 region and a reduction of the uncertainties from the precision mass input data.
Precision mass measurements of 104Y, 106Zr, 104,104m,109Nb, and 111,112Mo have been performed with the JYFLTRAP double Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line ...facility. The order of the long-lived states in 104Nb was unambiguously established. The trend in two-neutron separation energies around the N=66 neutron midshell appeared to be steeper with respect to the Atomic Mass Evaluation 2020 extrapolations for the 39Y and 40Zr isotopic chains and less steep for the 41Nb chain, indicating a possible gap opening around Z=40. The experimental results were compared to the BSkG2 model calculations performed with and without vibrational and rotational corrections. All of them predict two low-lying minima for 106Zr. While the unaltered BSkG2 model fails to predict the trend in two-neutron separation energies, selecting the more deformed minima in calculations and removing the vibrational correction, the calculations are more in line with experimental data. The same is also true for the 21+ excitation energies and differences in charge radii in the Zr isotopes. The results stress the importance of improved treatment of collective corrections in large-scale models and further development of beyond-mean-field techniques.
Isomers close to the doubly magic nucleus 78Ni (Z=28, N=50) provide essential information on the shell evolution and shape coexistence far from stability. The existence of a long-lived isomeric state ...in 76Cu has been debated for a long time. We have performed high-precision mass measurements of 76Cu with the JYFLTRAP double Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line facility and confirm the existence of such an isomeric state with an excitation energy Ex=64.8(25) keV. Based on the ratio of detected ground- and isomeric-state ions as a function of time, we show that the isomer is the shorter-living state previously considered as the ground state of 76Cu. The result can potentially change the conclusions made in previous works related to the spin-parity and charge radius of the 76Cu ground state. Additionally, the new 76Cu(n,γ) reaction Q-value has an impact on the astrophysical rapid neutron-capture process.
Abstract
Proton radioactivity was discovered exactly 50 years ago. First, this nuclear decay mode sets the limit of existence on the nuclear landscape on the neutron-deficient side. Second, it ...comprises fundamental aspects of both quantum tunnelling as well as the coupling of (quasi)bound quantum states with the continuum in mesoscopic systems such as the atomic nucleus. Theoretical approaches can start either from bound-state nuclear shell-model theory or from resonance scattering. Thus, proton-radioactivity guides merging these types of theoretical approaches, which is of broader relevance for any few-body quantum system. Here, we report experimental measurements of proton-emission branches from an isomeric state in
54m
Ni, which were visualized in four dimensions in a newly developed detector. We show that these decays, which carry an unusually high angular momentum, ℓ = 5 and ℓ = 7, respectively, can be approximated theoretically with a potential model for the proton barrier penetration and a shell-model calculation for the overlap of the initial and final wave functions.
Isomers close to doubly magic _{28}^{78}Ni_{50} provide essential information on the shell evolution and shape coexistence near the Z=28 and N=50 double shell closure. We report the excitation energy ...measurement of the 1/2^{+} isomer in _{30}^{79}Zn_{49} through independent high-precision mass measurements with the JYFLTRAP double Penning trap and with the ISOLTRAP multi-reflection time-of-flight mass spectrometer. We unambiguously place the 1/2^{+} isomer at 942(10) keV, slightly below the 5/2^{+} state at 983(3) keV. With the use of state-of-the-art shell-model diagonalizations, complemented with discrete nonorthogonal shell-model calculations which are used here for the first time to interpret shape coexistence, we find low-lying deformed intruder states, similar to other N=49 isotones. The 1/2^{+} isomer is interpreted as the bandhead of a low-lying deformed structure akin to a predicted low-lying deformed band in ^{80}Zn, and points to shape coexistence in ^{79,80}Zn similar to the one observed in ^{78}Ni. The results make a strong case for confirming the claim of shape coexistence in this key region of the nuclear chart.
The article describes the commissioning and technical development of the Weak Interaction Studies with 32Ar Decay (WISArD) experiment, installed at the radioactive ion-beam facility ISOLDE/CERN. The ...experiment aims to extend the present limits on scalar and tensor currents in the weak interaction and hence search for physics beyond the Standard Model. The evaluation of these limits relies on measuring the proton energy in beta-delayed proton emission, sensitive to both the beta-neutrino angular correlation coefficient aβν and the Fierz interference term b. The method tries to improve previous studies by considering the positron-proton coincidences when determining the kinematic shift in the energy of the emitted protons. Using this coincidence technique, the aβν and b coefficients will be measured at the per mil level. Simulations were employed to optimize the ion beam transport efficiency and validate proof-of-principle results obtained in November 2018 (Nov2018). Upgrades are ongoing, and we are looking into improvements to the overall performance of the setup.
We report the first high-precision mass measurements of the neutron-rich nuclei 74,75Ni and the clearly identified ground state of 76Cu, along with a more precise mass-excess value of 78Cu, performed ...with the double Penning trap JYFLTRAP at the Ion Guide Isotope Separator On-Line (IGISOL) facility. These new results lead to a quantitative estimation of the quenching for the N=50 neutron shell gap. The impact of this shell quenching on core-collapse supernova dynamics is specifically tested using a dedicated statistical equilibrium approach that allows a variation of the mass model independent of the other microphysical inputs. We conclude that the impact of nuclear masses is strong when implemented using a fixed trajectory as in the previous studies, but the effect is substantially reduced when implemented self-consistently in the simulation.
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