We have solved the long-standing problem of the mechanism of terahertz (THz) generation by a two-color filament in air and found that both neutrals and plasma contribute to the radiation. We reveal ...that the contribution from neutrals by four-wave mixing is much weaker and higher in frequency than the distinctive plasma lower-frequency contribution. The former is in the forward direction while the latter is in a cone and reveals an abrupt down-shift to the plasma frequency. Ring-shaped spatial distributions of the THz radiation are shown to be of universal nature and they occur in both collimated and focusing propagation geometries. Experimental measurements of the frequency-angular spectrum generated by 130-fs laser pulses agree with numerical simulations based on a unidirectional pulse propagation model.
Terahertz pulse generation by ultraintense two-color laser fields ionizing gases with near- to far-infrared carrier wavelength is studied from particle-in-cell simulations. For a long pump wavelength ...(10.6 μm) promoting a large ratio of electron density over critical, photoionization is shown to catastrophically enhance the plasma wakefield, causing a net downshift in the optical spectrum and exciting THz fields with tens of GV/m amplitude in the laser direction. This emission is accompanied by coherent transition radiation (CTR) of comparable amplitude due to wakefield-driven electron acceleration. We analytically evaluate the fraction of CTR energy up to 30% of the total radiated emission including the particle self-field and numerically calibrate the efficiency of the matched blowout regime for electron densities varied over three orders of magnitude.
We study the influence of the polarization states of ionizing femtosecond two-color pulses on the emitted terahertz radiation in gases. A local-current model and plane-wave evaluations justify the ...previously-reported impact on the THz energy yield and a (almost) linearly-polarized THz field when using circularly-polarized laser harmonics. For such pump pulses, the THz yield is independent of the relative phase between the two colors. When the pump pulses have same helicity, the increase in the THz yield is associated with longer ionization sequences and higher electron transverse momenta acquired in the driving field. Reversely, for two color pulses with opposite helicity, the dramatic loss of THz power comes from destructive interferences driven by the highly symmetric response of the photocurrents lined up on the third harmonic of the fundamental pulse. While our experiments confirm an increased THz yield for circularly-polarized pumps of same helicity, surprisingly, the emitted THz radiation is not linearly-polarized. This effect is explained by means of comprehensive 3D numerical simulations highlighting the role of the spatial alignment and non-collinear propagation of the two colors.
Terahertz to far-infrared emission by two-color, ultrashort optical pulses interacting with underdense helium gases at ultrahigh intensities (>10^{19} W/cm^{2}) is investigated by means of 3D ...particle-in-cell simulations. The terahertz field is shown to be produced by two mechanisms occurring sequentially, namely, photoionization-induced radiation (PIR) by the two-color pulse, and coherent transition radiation (CTR) by the wakefield-accelerated electrons escaping the plasma. We exhibit laser-plasma parameters for which CTR proves to be the dominant process, providing terahertz bursts with field strength as high as 100 GV/m and energy in excess of 10 mJ. Analytical models are developed for both the PIR and CTR processes, which correctly reproduce the simulation data.
Beyond a critical disorder, two-dimensional (2D) superconductors become insulating. In this Superconductor-Insulator Transition (SIT), the nature of the insulator is still controversial. Here, we ...present an extensive experimental study on insulating Nb
Si
close to the SIT, as well as corresponding numerical simulations of the electrical conductivity. At low temperatures, we show that electronic transport is activated and dominated by charging energies. The sample thickness variation results in a large spread of activation temperatures, fine-tuned via disorder. We show numerically and experimentally that this originates from the localization length varying exponentially with thickness. At the lowest temperatures, there is an increase in activation energy related to the temperature at which this overactivated regime is observed. This relation, observed in many 2D systems shows that conduction is dominated by single charges that have to overcome the gap when entering superconducting grains.
We numerically study the influence of chirping and delaying several ionizing two-color light pulses in order to engineer terahertz (THz) wave generation in air. By means of comprehensive 3D ...simulations, it is shown that two chirped pulses can increase the THz yield when they are separated by a suitable time delay for the same laser energy in focused propagation geometry. To interpret these results, the local current theory is revisited and we propose an easy, accessible all-optical criterion that predicts the laser-to-THz conversion efficiencies given any input laser spectrum. In the filamentation regime, numerical simulations display evidence that a chirped pulse is able to produce more THz radiation due to propagation effects, which maintain the two colors of the laser field more efficiently coupled over long distances. A large delay between two pulses promotes multi-peaked THz spectra as well as conversion efficiencies above 10−4.
We develop a one-dimensional model of THz emissions induced by laser-driven, time-asymmetric ionization and current oscillations in a hydrogen gas. Our model highlights complex scalings of the THz ...fields with respect to the laser and gas parameters, in particular, a non-monotonic behavior against the laser parameters. Analytical expressions of the transmitted and reflected fields are presented, explaining the THz spectra observed in particle-in-cell and forward-pulse propagation codes. The backward-propagating THz wave is mainly driven by the electron current oscillations at the plasma frequency, and its resulting spectrum operates below the plasma frequency. The transmitted THz wave is emitted from both plasma current oscillations and photo-ionization. Their respective signal presents a contribution below and around the plasma frequency, plus a contribution at higher frequencies associated to the photo-induced current. The interplay between these two mechanisms relies on the ratio between the propagation length and the plasma skin depth.
We theoretically and numerically study the influence of both instantaneous and Raman-delayed Kerr nonlinearities as well as a long-wavelength pump in the terahertz (THz) emissions produced by ...two-color femtosecond filaments in air. Although the Raman-delayed nonlinearity induced by air molecules weakens THz generation, four-wave mixing is found to impact the THz spectra accumulated upon propagation via self-, cross-phase modulations and self-steepening. Besides, using the local current theory, we show that the scaling of laser-to-THz conversion efficiency with the fundamental laser wavelength strongly depends on the relative phase between the two colors, the pulse duration and shape, rendering a universal scaling law impossible. Scaling laws in powers of the pump wavelength may only provide a rough estimate of the increase in the THz yield. We confront these results with comprehensive numerical simulations of strongly focused pulses and of filaments propagating over meter-range distances.
Relativistic interactions between ultraintense (>10^{18} W cm^{-2}) laser pulses and magnetized underdense plasmas are known to produce few-cycle Cerenkov wake radiation in the terahertz (THz) ...domain. Using multidimensional particle-in-cell simulations, we demonstrate the possibility of generating high-field (>100 GV m^{-1}) THz bursts from helium gas plasmas embedded in strong (>100 T) magnetic fields perpendicular to the laser path. We show that two criteria must be satisfied for efficient THz generation. First, the plasma density should be adjusted to the laser pulse duration for a strong resonant excitation of the electromagnetic plasma wake. Second, in order to mitigate the damping of the transverse wake component across the density gradients at the plasma exit, the ratio of the relativistic electron cyclotron and plasma frequencies must be chosen slightly above unity, but not too large, lest the wake be degraded. Such conditions lead the outgoing THz wave to surpass in amplitude the electrostatic wakefield induced in a similar, yet unmagnetized plasma.
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