In the TRITIUM project, an on-site monitoring system is being developed to measure tritium (3H) levels in water near nuclear power plants. The quite low-energy betas emitted by 3H have a very short ...average path in water (5 μm as shown by simulations for 18 keV electrons). This path would be further reduced by impurities present in the water, resulting in a significant reduction of the detection efficiency. Therefore, one of the essential requirements of the project is the elimination of these impurities through a filtration process and the removal of salts in solution. This paper describes a water treatment system developed for the project that meets the following requirements: the water produced should be of near-pure water quality according to ISO 3696 grade 3 standard (conductivity < 10 μS/cm); the system should operate autonomously and be remotely monitored.
The Modane underground laboratory (LSM) is the deepest operating underground laboratory in Europe. It is located under the Fréjus peak in Savoie Alps in France, with average overburden of 4800 m w. ...e. (water equivalent), providing low-background environment for experiments in nuclear and particle physics, astrophysics and environmental physics. It is crucial to understand individual sources of background such as residual cosmic-ray flux of high-energy muons, muon-induced neutrons and contributions from radionuclides present in the environment. The identified dominant sources of background are radioactive contamination of construction materials of detectors and laboratory walls, radon contamination of the laboratory air, and neutrons produced in the laboratory. The largest neutron contribution has been identified from (α, n) reactions in low Z materials (10−7-10−4 n s−1 Bq−1) and from spontaneous fission of 238U (1.1× 10−6 n s−1 Bq−1).
•Individual background contributions in the Modane underground laboratory are discussed.•Natural radioactive contamination in the detector construction and laboratory environment is the dominant background source.•Neutrons coming from the (α, n) reactions and spontaneous fission have been identified as the dominant neutron background sources.•Muon induced neutrons contribute less than 1% to neutron flux.
The influence of the addition of copper on the resistance to pitting corrosion of stainless steels has been investigated using different experimental techniques––current transient analysis, ...polarization curves in acidic media, pitting and repassivation potential measurements, XPS and SEM observations––so that pit initiation, propagation and repassivation could be analysed separately. Copper addition is shown to act in three different ways on pitting corrosion. On the one hand, copper reduces steel dissolution rates in acidic chloride media and also pit propagation rates. On the other hand, copper addition in steel is shown to lower repassivation potentials in neutral chloride environments and also to delay pit repassivation. Lastly, when copper is injected into solution as CuCl
2 or when the steel is polarized at anodic potentials so that copper can dissolve from the steel into solution, pit initiation close to sulfide inclusions is prevented. A model is proposed for these three different actions of copper, showing that the role of this element is complex and that no relevant information can be drawn from only considering its effect on the pitting potential.
Simulation results of a real-time in water tritium monitor Azevedo, C.D.R.; Baeza, A.; Chauveau, E. ...
Nuclear instruments & methods in physics research. Section A, Accelerators, spectrometers, detectors and associated equipment,
12/2020, Letnik:
982
Journal Article
Recenzirano
In this work we present simulation results for a modular tritium in-water real-time monitor. The system allows for scalability in order to achieve the required sensitivity. The modules are composed ...by 340 uncladed scintillating fibers immersed in water and 2 photosensors in coincidence for light readout. Light yield and Birks’ coefficient uncertainties for low energy beta particles is discussed. A study of the detection efficiency according to the fiber length is presented. Discussion on the system requirements and background mitigation for a device with sensitivity of 100Bq/L, required to comply with the European directive 2013/51/Euratom, is presented. Due to the low energetic beta emission from tritium a detection efficiency close to 3.3% was calculated for a single 2 mm round fiber.
The possibility to probe new physics scenarios of light Majorana neutrino exchange and right-handed currents at the planned next generation neutrinoless double
β
decay experiment SuperNEMO is ...discussed. Its ability to study different isotopes and track the outgoing electrons provides the means to discriminate different underlying mechanisms for the neutrinoless double
β
decay by measuring the decay half-life and the electron angular and energy distributions.
Abstract
In this paper, we report the development and performance of
a detector module envisaging a tritium-in-water real-time activity
monitor. The monitor is based on modular detection units whose
...number can be chosen according to the required sensitivity. The full
system is being designed to achieve a
Minimum Detectable
Activity
(
MDA
) of 100 Bq/L of tritium-in-water activity
which is the limit established by the E.U. Council Directive
2013/51/Euratom for water intended for human consumption. The same
system can be used as a real-time pre-alert system for nuclear power
plant regarding tritium-in water environmental surveillance. The
first detector module was characterized, commissioned and installed
immediately after the discharge channel of the Arrocampo dam
(Almaraz nuclear power plant, Spain) on the Tagus river. Due to the
high sensitivity of the single detection modules, the system
requires radioactive background mitigation techniques through the
use of active and passive shielding. We have extrapolated a
MDA
of 3.6 kBq/L for a single module being this value
limited by the cosmic background. The obtained value for a single
module is already compatible with a real-time environmental
surveillance and pre-alert system. Further optimization of the
single-module sensitivity will imply the reduction of the number of
modules and the cost of the detector system.
Tritium is released abundantly to the environment by nuclear power plants (NPP), as a product of neutron capture by hydrogen and deuterium. In normal running conditions, released cooling waters may ...contain levels of tritium close to or even larger than the maximum authorised limit for human consumption (drinking and irrigation). The European Council Directive 2013/51/Euratom requires a maximum level of tritium in water for human consumption lower than 100 Bq=L. Current monitoring of tritium activity in water by liquid scintillating method takes about two days and can only be carried out in a dedicated laboratory. This system is not appropriate for real time monitoring. At present, there exists no available detector device with enough sensitivity to monitor waters for human consumption with high enough sensitivity. The goal of the TRITIUM project is to build a tritium monitor capable to measure tritium activities with detection limit close to 100Bq=L, using instrumentation technique developed in recent years for Nuclear and Particle Physics, such as scintillating fibres and silicon photomultipliers (SiPM). In this paper the current status of the TRITIUM project is presented and he results of first prototypes are discussed. A detector system based on scintillating fibers read out either photomultiplier tubes (PMTs) or silicon photomultiplier (SiPM) arrays is under development and will be installed in the vicinity of Almaraz nuclear power plant (Cáceres, Spain) by the fourth term of 2019.
A novel and simple method for the measurement of cloud point temperatures of solutions is presented. Cloud point determination, which is currently used to establish the phase diagrams of protein ...solutions, is indicative of proteins interactions and constitutes a useful tool for food products engineering. We describe a novel experimental setup that allows screening of a large number of physical-chemical conditions in one measurement and the determination of cloud point temperatures both above and below ambient temperature. We use a simple method to avoid solvent evaporation and condensation, so that the set-up can be used for solutions prepared with a volatile solvent. We present the operating parameter range and the precision of the measurement. The optical properties of the system are calibrated with solutions of known transmittance, and the determination of cloud point temperatures is validated on a standard non-ionic surfactant solution. Finally, we demonstrate the efficiency of the method by determining the phase diagram of a wheat protein extract, soluble in a water/ethanol mixture. Complemented with differential scanning calorimetry measurements, the liquid-liquid phase transition can be determined up to a protein concentration of 250 g/L, a range inaccessible with conventional methods for this protein extract.
Abstract
In 1956 Reines & Cowan discovered the neutrino using a liquid scintillator detector. The neutrinos interacted with the scintillator, producing light that propagated across transparent ...volumes to surrounding photo-sensors. This approach has remained one of the most widespread and successful neutrino detection technologies used since. This article introduces a concept that breaks with the conventional paradigm of transparency by confining and collecting light near its creation point with an opaque scintillator and a dense array of optical fibres. This technique, called LiquidO, can provide high-resolution imaging to enable efficient identification of individual particles event-by-event. A natural affinity for adding dopants at high concentrations is provided by the use of an opaque medium. With these and other capabilities, the potential of our detector concept to unlock opportunities in neutrino physics is presented here, alongside the results of the first experimental validation.