We report a study of the impact of cold crystallization on the structure of nanocomposites comprising poly(vinylidene fluoride) (PVDF) and Lucentite STN™ organically modified silicate (OMS). ...Nanocomposites were prepared from solution over a very wide composition range, from 0.01 to 20% OMS by weight. Thermal preparation involved cold crystallization at 145°C of quenched, compression-molded plaques. Static and real-time wide and small angle X-ray scattering (WAXS, SAXS), Fourier transform infrared spectroscopy (FTIR), and differential scanning calorimetry (DSC) were used to investigate the crystalline phase of PVDF. For OMS content greater than 0.50wt%, WAXS studies show that that the silicate gallery spacing increases modestly in the nanocomposites compared to neat OMS film, indicating a level of polymer intercalation.
Using Gaussian peak fitting of WAXS profiles, we determine that the composition range can be divided into three parts. First, for OMS greater than 0.5wt%, alpha phase fraction, ϕalpha, is insignificant (ϕalpha∼0–0.01). Second, at the intermediate range, for OMS between 0.5wt% down to 0.025wt%, beta phase dominates and the beta fraction, ϕbeta, is related to alpha by ϕbeta>ϕalpha. Third, below 0.025wt% OMS, alpha dominates and ϕalpha>ϕbeta. The ability of small amounts of OMS (≥0.025wt%) to cause beta crystal domination is remarkable. Overall, crystallinity index (from the ratio of WAXS crystal peak area to total area) ranges from about 0.36 to 0.51 after cold crystallization. Real-time WAXS studies during heating of initially cold crystallized nanocomposites show that there is no inter-conversion between the alpha and beta phase PVDF crystals, where these crystals coexist at room temperature. While all samples showed a strong SAXS Bragg peak, indicating existence of two-phase lamellar stacks, the sample containing predominantly beta phase had poorly correlated lamellar stacks, compared to samples containing predominantly alpha phase.
The charge-conjugation and parity-reversal (CP) symmetry of fundamental particles is a symmetry between matter and antimatter. Violation of this CP symmetry was first observed in 1964
, and CP ...violation in the weak interactions of quarks was soon established
. Sakharov proposed
that CP violation is necessary to explain the observed imbalance of matter and antimatter abundance in the Universe. However, CP violation in quarks is too small to support this explanation. So far, CP violation has not been observed in non-quark elementary particle systems. It has been shown that CP violation in leptons could generate the matter-antimatter disparity through a process called leptogenesis
. Leptonic mixing, which appears in the standard model's charged current interactions
, provides a potential source of CP violation through a complex phase δ
, which is required by some theoretical models of leptogenesis
. This CP violation can be measured in muon neutrino to electron neutrino oscillations and the corresponding antineutrino oscillations, which are experimentally accessible using accelerator-produced beams as established by the Tokai-to-Kamioka (T2K) and NOvA experiments
. Until now, the value of δ
has not been substantially constrained by neutrino oscillation experiments. Here we report a measurement using long-baseline neutrino and antineutrino oscillations observed by the T2K experiment that shows a large increase in the neutrino oscillation probability, excluding values of δ
that result in a large increase in the observed antineutrino oscillation probability at three standard deviations (3σ). The 3σ confidence interval for δ
, which is cyclic and repeats every 2π, is -3.41, -0.03 for the so-called normal mass ordering and -2.54, -0.32 for the inverted mass ordering. Our results indicate CP violation in leptons and our method enables sensitive searches for matter-antimatter asymmetry in neutrino oscillations using accelerator-produced neutrino beams. Future measurements with larger datasets will test whether leptonic CP violation is larger than the CP violation in quarks.
The T2K experiment reports updated measurements of neutrino and antineutrino oscillations using both appearance and disappearance channels. This result comes from an exposure of 14.9 (16.4) × 1020 ...protons on target in neutrino (antineutrino) mode. Significant improvements have been made to the neutrino interaction model and far detector reconstruction. An extensive set of simulated data studies have also been performed to quantify the effect interaction model uncertainties have on the T2K oscillation parameter sensitivity. T2K performs multiple oscillation analyses that present both frequentist and Bayesian intervals for the Pontecorvo-Maki-Nakagawa-Sakata parameters. For fits including a constraint on sin 2θ13 from reactor data and assuming normal mass ordering T2K measures sin 2θ23 = 0.53 +0.03 −0.04 and Δm232 = (2.45 ± 0.07) × 10−3 eV2 c−4. The Bayesian analyses show a weak preference for normal mass ordering (89% posterior probability) and the upper sin 2θ23 octant (80% posterior probability), with a uniform prior probability assumed in both cases. The T2K data exclude CP conservation in neutrino oscillations at the 2σ level.
T2K reports its first results in the search for CP violation in neutrino oscillations using appearance and disappearance channels for neutrino- and antineutrino-mode beams. The data include all runs ...from January 2010 to May 2016 and comprise 7.482×10^{20} protons on target in neutrino mode, which yielded in the far detector 32 e-like and 135 μ-like events, and 7.471×10^{20} protons on target in antineutrino mode, which yielded 4 e-like and 66 μ-like events. Reactor measurements of sin^{2}2θ_{13} have been used as an additional constraint. The one-dimensional confidence interval at 90% for the phase δ_{CP} spans the range (-3.13, -0.39) for normal mass ordering. The CP conservation hypothesis (δ_{CP}=0, π) is excluded at 90% C.L.
This paper reports on the search for heavy neutrinos with masses in the range 140<MN<493 MeV/c2 using the off-axis near detector ND280 of the T2K experiment. These particles can be produced from kaon ...decays in the standard neutrino beam and then subsequently decay in ND280. The decay modes under consideration are N→ℓα±π∓ and N→ℓα+ℓβ−ν(−)(α,β=e,μ). A search for such events has been made using the Time Projection Chambers of ND280, where the background has been reduced to less than two events in the current dataset in all channels. No excess has been observed in the signal region. A combined Bayesian statistical approach has been applied to extract upper limits on the mixing elements of heavy neutrinos to electron-, muon- and tau- flavored currents (Ue2, Uμ2, Uτ2) as a function of the heavy neutrino mass, e.g., Ue2<10−9 at 90% C.L. for a mass of 390 MeV/c2. These constraints are competitive with previous experiments.
The T2K experiment has observed electron neutrino appearance in a muon neutrino beam produced 295 km from the Super-Kamiokande detector with a peak energy of 0.6 GeV. A total of 28 electron neutrino ...events were detected with an energy distribution consistent with an appearance signal, corresponding to a significance of 7.3σ when compared to 4.92±0.55 expected background events. In the Pontecorvo-Maki-Nakagawa-Sakata mixing model, the electron neutrino appearance signal depends on several parameters including three mixing angles θ12, θ23, θ13, a mass difference Δm(32)(2) and a CP violating phase δ(CP). In this neutrino oscillation scenario, assuming |Δm(32)(2)|=2.4×10(-3) eV(2), sin(2)θ(23)=0.5, and Δm322>0 (Δm(32)(2)<0), a best-fit value of sin(2)2θ(13)=0.140(-0.032)(+0.038) (0.170(-0.037)(+0.045)) is obtained at δ(CP)=0. When combining the result with the current best knowledge of oscillation parameters including the world average value of θ(13) from reactor experiments, some values of δ(CP) are disfavored at the 90% C.L.
We report the results of a search for ν(e) appearance in a ν(μ) beam in the MINOS long-baseline neutrino experiment. With an improved analysis and an increased exposure of 8.2 × 10(20) protons on the ...NuMI target at Fermilab, we find that 2 sin(2) (θ(23))sin(2)(2θ(13))<0.12(0.20) at 90% confidence level for δ = 0 and the normal (inverted) neutrino mass hierarchy, with a best-fit of 2sin(2) (θ(23))sin(2)(2θ(13)) = 0.041(-0.031)(+0.047) (0.079(-0.053) (+0.071)). The θ(13) = 0 hypothesis is disfavored by the MINOS data at the 89% confidence level.
A set of comparisons among neutrino interaction experiments MiniBooNE, MINERvA, Tokai-to-Kamioka (T2K), and MicroBooNE is presented. This gives a broad view of the field of neutrino-nucleus ...interactions. The emphasis is on charged-current inclusive, quasielastic-like, and pion production experiments. Measurements are compared in new ways. Comparisons of recent data with available event generator codes are made more comprehensively than is regularly found in most previous publications. Generator studies show sensitivities for experimental model dependence. Efficiencies calculated with different generators are presented in a novel way. A comparison of different forward-folding techniques is also presented.
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