Mesoscale simulations of the shock-compression response of nickel and aluminum powder mixtures have been performed to investigate the influence of particle configuration (size, shape and ...distribution) on the micromechanical processes of deformation, mass flow and mixing. Real microstructures were constructed from scanning electron microscopy montages of the starting mixtures pre-pressed at various densities Eakins D, Thadhani NN, J Appl Phys, 2007;101:043508. The travel of the high-pressure disturbance was used to determine the equation-of-state of the mixture material, and compared to the results of real-time experiments for validation. Observations of particle-level processes were used to formulate an understanding of the wide range of macroscopic behaviors exhibited as a function of particle morphology and distribution, porosity, and dissimilarities in properties of the two constituents. The results reveal the effects of particle heterogeneity on the physical, chemical and micromechanical response of shock-compressed Ni
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Al powder mixtures, and their role in the initiation of shock-induced chemical reactions.
The shock compression of reactive powder mixtures can yield varied chemical behaviour with occurrence of mechanochemical reactions in the timescale of the high pressure state, or thermochemical ...reactions in the timescale of temperature equilibration, or simply the creation of dense packed highly reactive state of material. The principal challenge has been to understand the processes that distinguish between mechanochemical (shock induced) and thermochemical (shock assisted) reactions, which has broad implications for the synthesis of novel metastable or non-equilibrium materials, or the design of highly configurable next generation energetic materials. In this paper, the process of shock compression in reactive powder mixtures and the associated role of various intrinsic and extrinsic characteristics of reactants in the triggering of ultrafast shock induced chemical reactions are discussed. Experimental techniques employing time resolved diagnostics and results which identify the occurrence of shock induced reactions are reviewed. Conceptual and numerical models used to describe the heterogeneous nature of such reactions through mesoscopic details of shock compression are presented. Finally, a discussion of the application of recent results for the design of reactive material systems with controlled reaction initiation and energy release characteristics is provided.
Betatron radiation from laser wakefield accelerators is an ultrashort pulsed source of hard, synchrotron-like x-ray radiation. It emanates from a centimetre scale plasma accelerator producing GeV ...level electron beams. In recent years betatron radiation has been developed as a unique source capable of producing high resolution x-ray images in compact geometries. However, until now, the short pulse nature of this radiation has not been exploited. This report details the first experiment to utilize betatron radiation to image a rapidly evolving phenomenon by using it to radiograph a laser driven shock wave in a silicon target. The spatial resolution of the image is comparable to what has been achieved in similar experiments at conventional synchrotron light sources. The intrinsic temporal resolution of betatron radiation is below 100 fs, indicating that significantly faster processes could be probed in future without compromising spatial resolution. Quantitative measurements of the shock velocity and material density were made from the radiographs recorded during shock compression and were consistent with the established shock response of silicon, as determined with traditional velocimetry approaches. This suggests that future compact betatron imaging beamlines could be useful in the imaging and diagnosis of high-energy-density physics experiments.
Extraordinary states of highly localised pressure and temperature can be generated upon the collapse of impulsively driven cavities. Direct observation of this phenomenon in solids has proved ...challenging, but recent advances in high-speed synchrotron radiography now permit the study of highly transient, subsurface events in real time. We present a study on the shock-induced collapse of spherical cavities in a solid polymethyl methacrylate medium, driven to shock states between 0.49 and 16.60 GPa. Utilising multi-MHz phase contrast radiography, extended sequences of the collapse process have been captured, revealing new details of interface motion, material failure and jet instability formation. Results reveal a rich array of collapse characteristics dominated by strength effects at low shock pressures and leading to a hydrodynamic response at the highest loading conditions.
This article offers a comprehensive experimental and theoretical study of the causes of thermal hardening in FCC Al and BCC Fe at high strain rates, with the aim to shed light on important mechanisms ...governing deformation and failures in materials subjected to shocks and impacts at very high strain rates. Experimental evidence regarding the temperature dependence of the dynamic yield point of FCC Al and BCC Fe shock loaded at 107 s−1 is provided. The dynamic yield point of Al increases with temperature in the range 125K–795K; for the same loading and temperate range, the dynamic yield point of BCC Fe remains largely insensitive. A Multiscale Discrete Dislocation Plasticity (MDDP) model of both Fe and Al is developed, leading to good agreement with experiments. The importance of the Peierls barrier in Fe is highlighted, showing it is largely responsible for the temperature insensitivity in BCC metals. The relevance of the mobility of edge components in determining the plastic response of both FCC Al and BCC Fe at different temperatures is discussed, which leads to developing a mechanistic explanation of the underlying mechanisms leading to the experimental behaviour using Dynamic Discrete Dislocation Plasticity (D3P). It is shown that the main contributing factor to temperature evolution of the dynamic yield point is not the mobility of dislocations, but the temperature variation of the shear modulus, the decrease of which is correlated to the experimental behaviour observed for both FCC Al and BCC Fe.
The effect of grain orientation distribution on the dynamic strength of highly textured magnesium alloy AZ31B has been studied in a series of plate-impact experiments. Specimens with thicknesses ...between 0.45 mm and 2 mm were cut parallel and perpendicular to the material extrusion direction and shock loaded to impact stresses between 1.4 GPa and 3.4 GPa. The dynamic strength is found to be highly dependent on the loading direction, with loading along the extrusion direction exhibiting significantly higher Hugoniot elastic limits than the transverse direction, including a much slower precursor decay rate. Application of an orientation-based analysis framework shows that the yield point of the polycrystalline material can be predicted reasonably well from its grain orientation distribution, predicated upon the use of dynamic critical resolved shear stress values from single-crystal data modified by a fitted strengthening factor. It is shown that the strong dependence on loading orientation in Mg AZ31 is caused by the relative differences in slip system activity and the slip anisotropies inherent to the hexagonal close packed crystal structure.