One of the most important atomic properties governing an element's chemical behavior is the energy required to remove its least-bound electron, referred to as the first ionization potential. For the ...heaviest elements, this fundamental quantity is strongly influenced by relativistic effects which lead to unique chemical properties. Laser spectroscopy on an atom-at-a-time scale was developed and applied to probe the optical spectrum of neutral nobelium near the ionization threshold. The first ionization potential of nobelium is determined here with a very high precision from the convergence of measured Rydberg series to be 6.626 21±0.000 05 eV. This work provides a stringent benchmark for state-of-the-art many-body atomic modeling that considers relativistic and quantum electrodynamic effects and paves the way for high-precision measurements of atomic properties of elements only available from heavy-ion accelerator facilities.
The cascading 3.21 and 4.44 MeV electric quadrupole transitions have been observed from the Hoyle state at 7.65 MeV excitation energy in C12, excited by the C12(p,p′) reaction at 10.7 MeV proton ...energy. From the proton-γ−γ triple coincidence data, a value of Γrad/Γ=6.2(6)×10−4 was obtained for the radiative branching ratio. Using our results, together with ΓπE0/Γ from Eriksen et al. Phys. Rev. C 102, 024320 (2020) and the currently adopted Γπ(E0) values, the radiative width of the Hoyle state is determined as Γrad=5.1(6)×10−3 eV. This value is about 34% higher than the currently adopted value and will impact models of stellar evolution and nucleosynthesis.
Until recently, ground-state nuclear moments of the heaviest nuclei could only be inferred from nuclear spectroscopy, where model assumptions are required. Laser spectroscopy in combination with ...modern atomic structure calculations is now able to probe these moments directly, in a comprehensive and nuclear-model-independent way. Here we report on unique access to the differential mean-square charge radii of ^{252,253,254}No, and therefore to changes in nuclear size and shape. State-of-the-art nuclear density functional calculations describe well the changes in nuclear charge radii in the region of the heavy actinides, indicating an appreciable central depression in the deformed proton density distribution in ^{252,254}No isotopes. Finally, the hyperfine splitting of ^{253}No was evaluated, enabling a complementary measure of its (quadrupole) deformation, as well as an insight into the neutron single-particle wave function via the nuclear spin and magnetic moment.
A nuclear spectroscopy experiment was conducted to study α-decay chains stemming from isotopes of flerovium (element Z=114). An upgraded TASISpec decay station was placed behind the gas-filled ...separator TASCA at the GSI Helmholtzzentrum für Schwerionenforschung in Darmstadt, Germany. The fusion-evaporation reactions ^{48}Ca+^{242}Pu and ^{48}Ca+^{244}Pu provided a total of 32 flerovium-candidate decay chains, of which two and eleven were firmly assigned to ^{286}Fl and ^{288}Fl, respectively. A prompt coincidence between a 9.60(1)-MeV α particle event and a 0.36(1)-MeV conversion electron marked the first observation of an excited state in an even-even isotope of the heaviest man-made elements, namely ^{282}Cn. Spectroscopy of ^{288}Fl decay chains fixed Q_{α}=10.06(1) MeV. In one case, a Q_{α}=9.46(1)-MeV decay from ^{284}Cn into ^{280}Ds was observed, with ^{280}Ds fissioning after only 518 μs. The impact of these findings, aggregated with existing data on decay chains of ^{286,288}Fl, on the size of an anticipated shell gap at proton number Z=114 is discussed in light of predictions from two beyond-mean-field calculations, which take into account triaxial deformation.
Nuclear fragmentation measurements are necessary when using heavy-ion beams in hadrontherapy to predict the effects of the ion nuclear interactions within the human body. Moreover, they are also ...fundamental to validate and improve the Monte Carlo codes for their use in planning tumor treatments. Nowadays, a very limited set of carbon fragmentation cross sections are being measured, and in particular, to our knowledge, no double-differential fragmentation cross sections at intermediate energies are available in the literature. In this work, we have measured the double-differential cross sections and the angular distributions of the secondary fragments produced in the 12C fragmentation at 62 A MeV on a thin carbon target. The experimental data have been used to benchmark the prediction capability of the Geant4 Monte Carlo code at intermediate energies, where it was never tested before. In particular, we have compared the experimental data with the predictions of two Geant4 nuclear reaction models: the Binary Light Ions Cascade and the Quantum Molecular Dynamic. From the comparison, it has been observed that the Binary Light Ions Cascade approximates the angular distributions of the fragment production cross sections better than the Quantum Molecular Dynamic model. However, the discrepancies observed between the experimental data and the Monte Carlo simulations lead to the conclusion that the prediction capability of both models needs to be improved at intermediate energies.
Alpha-gamma decay studies of 247Md Heßberger, F. P.; Antalic, S.; Giacoppo, F. ...
The European physical journal. A, Hadrons and nuclei,
2022/1, Letnik:
58, Številka:
1
Journal Article
Recenzirano
Odprti dostop
Alpha decay and spontaneous fission of the ground-state and the isomeric state of
247
Md were investigated with specific emphasis to identify the ground-state of the daughter nucleus
243
Es. The ...decay studies were accompanied by measuring
α
-
γ
coincidences. On the basis of the measured data an improved decay scheme of
247
Md is proposed. Spontaneous fission half-lives of
247
g
Md and
247
m
Md were determined and the fission hindrance of the high spin ground-state (7/2
-
) relative to the low spin isomeric state (1/2
-
) was estimated.
Direct high-precision mass spectrometry of the heaviest elements with SHIPTRAP, at GSI in Darmstadt, Germany, requires high efficiency to deal with the low production rates of such exotic nuclides. A ...second-generation gas stopping cell, operating at cryogenic temperatures, was developed and recently integrated into the relocated system to boost the overall efficiency. Offline measurements using 223Ra and 225Ac recoil-ion sources placed inside the gas volume were performed to characterize the gas stopping cell with respect to purity and extraction efficiency. In addition, a first online test using the fusion-evaporation residue 254No was performed, resulting in a combined stopping and extraction efficiency of 33(5)%. An extraction time of 55(44)ms was achieved. The overall efficiency of SHIPTRAP for fusion-evaporation reaction products was increased by an order of magnitude to 6(1)%. This will pave the way for direct mass spectrometry of heavier and more exotic nuclei, eventually in the region of superheavy elements with proton numbers Z⩾104.
Twenty-one two-proton knockout (p , 3p) cross sections were measured from neutron-rich nuclei at ∼ 250 MeV /nucleon in inverse kinematics. The angular distribution of the three emitted protons was ...determined for the first time, demonstrating that the (p, 3p) kinematics are consistent with two sequential proton-proton collisions within the projectile nucleus. Ratios of (p , 3p) over (p, 2p) inclusive cross sections follow the trend of other many-nucleon removal reactions, further reinforcing the sequential nature of (p, 3p) in neutron-rich nuclei.
Fifty-five inclusive single nucleon-removal cross sections from medium mass neutron-rich nuclei impinging on a hydrogen target at ∼250 MeV/nucleon are measured at the RIKEN Radioactive Isotope Beam ...Factory. Systematically higher cross sections are found for proton removal from nuclei with an even number of protons as compared to odd-proton number projectiles for a given neutron separation energy. Neutron removal cross sections display no even-odd splitting, contrary to nuclear cascade model predictions. Both effects are understood through simple considerations of neutron separation energies and bound state level densities originating in pairing correlations in the daughter nuclei. These conclusions are supported by comparison with semimicroscopic model predictions, highlighting the enhanced role of low-lying level densities in nucleon-removal cross sections from loosely bound nuclei.
Prompt and delayed γ-ray spectroscopy of the neutron-deficient, semi-magic isotope 187Pb has been performed using the recoil-decay and isomer-decay tagging techniques at the Argonne Gas-Filled ...Analyzer. A new 5.15(15)-μs isomeric state at only 308 keV above the spherical 3/2− ground state is identified and classified as a shape isomer. A strongly-coupled band is observed on top of the isomer, which is nearly identical to the one built on the prolate 7/2−514 Nilsson state in the isotone 185Hg. Based on this similarity and on the result of the potential-energy surface calculations, the new isomer in 187Pb is proposed to originate from the same configuration. The retarded character of the 308-keV (7/2−)→3/2gs− transition with a deduced B(E2)=5.6(2)×10−4 W.u. can be well explained by the significant difference between the prolate parent and spherical daughter configurations, leading to the shape isomerism. The excitation energy of the isomer is surprisingly low, being roughly half of the excitation energies of the known 0+ intruder bandheads in the neighboring 186,188Pb isotopes. The combined results of the present work and the previous α-decay and laser spectroscopy studies present evidence for triple shape coexistence at low energy in the negative-parity configurations of 187Pb, which is well reproduced by the potential-energy surface calculations.
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