We compute the charge radii and ground-state energies of even-mass neon and magnesium isotopes from neutron number N=8 to the dripline. Our calculations are based on nucleon-nucleon and three-nucleon ...potentials from chiral effective field theory that include Δ isobars. These potentials yield an accurate saturation point and symmetry energy of nuclear matter. We use the coupled-cluster method and start from an axially symmetric reference state. Binding energies and two-neutron separation energies largely agree with data, and the dripline in neon is accurate. The computed charge radii are accurate for many isotopes where data exist. Finer details, such as isotope shifts, however, are not accurately reproduced. These chiral potentials indicate a subshell closure at N=14 for the radii (but not for two-neutron separation energies) and a decrease in charge radii at N=8 (observed in neon and predicted for magnesium). They yield a continued increase of charge radii as neutrons are added beyond N=14 yet underestimate the large increase at N=20 in magnesium.
In the past decade, coupled-cluster theory has seen a renaissance in nuclear physics, with computations of neutron-rich and medium-mass nuclei. The method is efficient for nuclei with product-state ...references, and it describes many aspects of weakly bound and unbound nuclei. This report reviews the technical and conceptual developments of this method in nuclear physics, and the results of coupled-cluster calculations for nucleonic matter, and for exotic isotopes of helium, oxygen, calcium, and some of their neighbors.
We employ interactions from chiral effective field theory and compute binding energies, excited states, and radii for isotopes of oxygen with the coupled-cluster method. Our calculation includes the ...effects of three-nucleon forces and of the particle continuum, both of which are important for the description of neutron-rich isotopes in the vicinity of the nucleus 24O. Our main results are the placement of the neutron drip line at 24O, the assignment of spins, parities and resonance widths for several low-lying states of the drip line nucleus, and an efficient approximation that incorporates the effects of three-body interactions.
We employ interactions from chiral effective field theory and compute the binding energies and low-lying excitations of calcium isotopes with the coupled-cluster method. Effects of three-nucleon ...forces are included phenomenologically as in-medium two-nucleon interactions, and the coupling to the particle continuum is taken into account using a Berggren basis. The computed ground-state energies and the low-lying J(π) = 2+ states for the isotopes (42,48,50,52)Ca are in good agreement with data, and we predict the excitation energy of the first J(π) = 2+ state in (54)Ca at 1.9 MeV, displaying only a weak subshell closure. In the odd-mass nuclei (53,55,61)Ca we find that the positive parity states deviate strongly from the naive shell model.
We optimize the nucleon-nucleon interaction from chiral effective field theory at next-to-next-to-leading order (NNLO). The resulting new chiral force NNLO(opt) yields χ(2)≈1 per degree of freedom ...for laboratory energies below approximately 125 MeV. In the A=3, 4 nucleon systems, the contributions of three-nucleon forces are smaller than for previous parametrizations of chiral interactions. We use NNLO(opt) to study properties of key nuclei and neutron matter, and we demonstrate that many aspects of nuclear structure can be understood in terms of this nucleon-nucleon interaction, without explicitly invoking three-nucleon forces.
Despite being a complex many-body system, the atomic nucleus exhibits simple structures for certain 'magic' numbers of protons and neutrons. The calcium chain in particular is both unique and ...puzzling: evidence of doubly magic features are known in 40,48Ca, and recently suggested in two radioactive isotopes, 52,54Ca. Although many properties of experimentally known calcium isotopes have been successfully described by nuclear theory, it is still a challenge to predict the evolution of their charge radii. Here we present the first measurements of the charge radii of 49,51,52Ca, obtained from laser spectroscopy experiments at ISOLDE, CERN. The experimental results are complemented by state-of-the-art theoretical calculations. The large and unexpected increase of the size of the neutron-rich calcium isotopes beyond N = 28 challenges the doubly magic nature of 52Ca and opens new intriguing questions on the evolution of nuclear sizes away from stability, which are of importance for our understanding of neutron-rich atomic nuclei.
Nanocrystalline oxide powders of the type IrxSn1−xO2 (0.2≤x≤1) have been produced and characterised. These oxides have been developed primarily as oxygen evolution electrocatalysts for proton ...exchange membrane (PEM) water electrolysers. Two methods were used to produce the oxide materials: the modified polyol method and the Adams fusion method. X-ray diffraction analysis suggests that an iridium–tin oxide solid solution with a rutile structure can be produced using the modified polyol method, with a linear relationship between the lattice parameters and composition. The crystal size of the solid solution phase is below 15 nm for all compositions. The Adams fusion method results in at least two separate oxide phases, namely a tin rich oxide and an iridium rich oxide. X-ray photoelectron spectroscopy (XPS) analysis revealed no significant difference between the bulk and surface compositions, and that the iridium was present in at least two valent states. The electrical resistivity of the powders was compared, and an exponential increase in resistivity with tin addition was found. Overall the resistivity measurements suggest that the limit for tin addition is around 50–60 mol% due to the high ohmic losses expected at higher tin contents in a PEM water electrolyser.
Structure of the Lightest Tin Isotopes Morris, T D; Simonis, J; Stroberg, S R ...
Physical review letters,
2018-Apr-13, Letnik:
120, Številka:
15
Journal Article
Recenzirano
Odprti dostop
We link the structure of nuclei around ^{100}Sn, the heaviest doubly magic nucleus with equal neutron and proton numbers (N=Z=50), to nucleon-nucleon (NN) and three-nucleon (NNN) forces constrained ...by data of few-nucleon systems. Our results indicate that ^{100}Sn is doubly magic, and we predict its quadrupole collectivity. We present precise computations of ^{101}Sn based on three-particle-two-hole excitations of ^{100}Sn, and we find that one interaction accurately reproduces the small splitting between the lowest J^{π}=7/2^{+} and 5/2^{+} states.
The dominant decay mode of atomic nuclei is beta decay (β-decay), a process that changes a neutron into a proton (and vice versa). This decay offers a window to physics beyond the standard model, and ...is at the heart of microphysical processes in stellar explosions and element synthesis in the Universe1–3. However, observed β-decay rates in nuclei have been found to be systematically smaller than for free neutrons: this 50-year-old puzzle about the apparent quenching of the fundamental coupling constant by a factor of about 0.75 (ref. 4) is without a first-principles theoretical explanation. Here, we demonstrate that this quenching arises to a large extent from the coupling of the weak force to two nucleons as well as from strong correlations in the nucleus. We present state-of-the-art computations of β-decays from light- and medium-mass nuclei to 100Sn by combining effective field theories of the strong and weak forces5 with powerful quantum many-body techniques6–8. Our results are consistent with experimental data and have implications for heavy element synthesis in neutron star mergers9–11 and predictions for the neutrino-less double-β-decay3, where an analogous quenching puzzle is a source of uncertainty in extracting the neutrino mass scale12.The difference between the β-decay rate predicted for free neutrons and that measured in real nuclei is explained by first-principles calculations to arise from strong correlations and the weak-force coupling between nucleons.
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