We report on several features in the energy spectrum from an ultralow-noise germanium detector operated deep underground. By implementing a new technique able to reject surface events, a number of ...cosmogenic peaks can be observed for the first time. We discuss an irreducible excess of bulklike events below 3 keV in ionization energy. These could be caused by unknown backgrounds, but also dark matter interactions consistent with DAMA/LIBRA. It is not yet possible to determine their origin. Improved constraints are placed on a cosmological origin for the DAMA/LIBRA effect.
Fifteen months of cumulative CoGeNT data are examined for indications of an annual modulation, a predicted signature of weakly interacting massive particle (WIMP) interactions. Presently available ...data support the presence of a modulated component of unknown origin, with parameters prima facie compatible with a galactic halo composed of light-mass WIMPs. Unoptimized estimators yield a statistical significance for a modulation of ∼2.8σ, limited by the short exposure.
Pacific Northwest National Laboratory has recently opened a shallow underground laboratory intended for measurement of low-concentration levels of radioactive isotopes in samples collected from the ...environment. The development of a low-background liquid scintillation counter is currently underway to further augment the measurement capabilities within this underground laboratory. Liquid scintillation counting is especially useful for measuring charged particle (e.g., β and α) emitting isotopes with no (or very weak) gamma-ray yields. The combination of high-efficiency detection of charged particle emission in a liquid scintillation cocktail coupled with the low-background environment of an appropriately designed shield located in a clean underground laboratory provides the opportunity for increased-sensitivity measurements of a range of isotopes. To take advantage of the 35m-water-equivalent overburden of the underground laboratory, a series of simulations have evaluated the scintillation counter's shield design requirements to assess the possible background rate achievable. This report presents the design and background evaluation for a shallow underground, low background liquid scintillation counter design for sample measurements.
•Graded-shielding can produce an ultra-low-background liquid scintillation counter.•Location in a shallow underground cleanroom further enhances background reduction.•A novel light collection design and selected low background materials are utilized.•The background is predicted to be 10–100 times below typical commercial systems.•Simulations tentatively predict a background rate of order 10 counts per day.
A new ultra-low-background proportional counter was recently developed with an internal volume of 100cm3 and has been characterized at pressures from 1–10atm with P-10 (90% Ar, 10% methane) gas. This ...design, along with a counting system providing event digitization and passive and active shielding, has been developed to complement a new shallow underground laboratory (30m water-equivalent). Backgrounds and low-level reference materials have been measured, and system sensitivity for 37Ar has been calculated.
•A new PNNL shallow underground laboratory is operational.•A low-background gas proportional counting system for argon has been prepared.•First background data has been collected relevant to an Ar-37 signature.•First calibration measurements of a low-level standard have been made.•Detector response to Ar-37 has been calculated and Ar-37 sensitivity projected.
The Ultra-Low Background Liquid Scintillation Counter developed by Pacific Northwest National Laboratory will expand the application of liquid scintillation counting by enabling lower detection ...limits and smaller sample volumes. By reducing the overall count rate of the background environment approximately 2 orders of magnitude below that of commercially available systems, backgrounds on the order of tens of counts per day over an energy range of ~3–3600keV can be realized. Initial test results of the ULB LSC show promising results for ultra-low background detection with liquid scintillation counting.
•Observed background is within a factor of 2 of the predictions from simulation.•Background achieved is 2 orders of magnitude below commercially available systems.•Backgrounds are in tens of counts per day over an energy range of ~3– 3600keV.•Initial results show promise for ultra-low background detection with the ULB LSC.
Pacific Northwest National Laboratory reports on the detection of 39Ar at the location of an underground nuclear explosion on the Nevada Nuclear Security Site. The presence of 39Ar was not ...anticipated at the outset of the experimental campaign but results from this work demonstrated that it is present, along with 37Ar and 85Kr in the subsurface at the site of an underground nuclear explosion. Our analysis showed that by using state-of-the-art technology optimized for radioargon measurements, it was difficult to distinguish 39Ar from the fission product 85Kr. Proportional counters are currently used for high-sensitivity measurement of 37Ar and 39Ar. Physical and chemical separation processes are used to separate argon from air or soil gas, yielding pure argon with contaminant gases reduced to the parts-per-million level or below. However, even with purification at these levels, the beta decay signature of 85Kr can be mistaken for that of 39Ar, and the presence of either isotope increases the measurement background level for the measurement of 37Ar. Measured values for the 39Ar measured at the site ranged from 36,000 milli- Becquerel/standard-cubic-meter-of-air (mBq/SCM) for shallow bore holes to 997,000 mBq/SCM from the rubble chimney from the underground nuclear explosion.
•We report on the detection of 39Ar at the location of an underground nuclear explosion on the Nevada Nuclear Security Site.•Argon-39 was detected, along with 37Ar and 85Kr in the subsurface at the Barnwell underground nuclear explosion.•These isotopes are produced through fission (85Kr) through the 40Ca(n, alpha) 37Ar reaction or 39K(n, p) 39Ar reaction.•Measured values for the 39Ar ranged from 36,000 (mBq/SCM) for shallow bore holes to 997,000 mBq/SCM from the rubble chimney.•Argon-39 and 85Kr, could interfere with gas sampling and detection equipment used in an on-site inspection.
This paper describes the generation of 39Ar, via reactor irradiation of potassium carbonate, followed by quantitative analysis (length-compensated proportional counting) to yield two calibration ...standards that are respectively 50 and 3 times atmospheric background levels. Measurements were performed in Pacific Northwest National Laboratory's shallow underground counting laboratory studying the effect of gas density on beta-transport; these results are compared with simulation. The total expanded uncertainty of the specific activity for the ~50× 39Ar in P10 standard is 3.6% (k=2).
•39Ar is generated via reactor irradiation of potassium carbonate.•Low-level standards are produced to assist in ground water age-dating studies.•Quantification using length compensated proportional counting is performed.•Wall- and threshold-effects are studied and discussed in terms of uncertainty.
The measurement of 37Ar has been proposed as a method of detecting underground nuclear testing. The isotope 37Ar is generated by neutron activation of calcium by the reaction, 40Ca(n, a)37Ar, and, as ...a noble gas, is able to migrate more freely underground. Pacific Northwest National Laboratory has developed a high throughput 37Ar collection and measurement system using modified Ultra-Low Background Proportional Counters (ULBPCs). This system is capable of collecting, purifying, and measuring radioactivity in argon from either atmospheric or soil gas samples. This process is automated, with minimal operator intervention. This paper describes quantification of 37Ar and how we account for varying background conditions. An example is provided in which 39Ar has been shown to be a significant background in some sample sets, created by process 39K(n,p)39Ar during an underground nuclear explosion that would also create 37Ar. To account for the large background of 39Ar, we fit the data with a constant plus exponential background model with Gaussian signal model and use the results of a constrained fit to calculate 37Ar activity. We discuss the methods used to purify and count samples. We discuss the impact of increased 39Ar backgrounds on the measurement of 37Ar.
As the world faces a challenging future in maintaining the commercial availability of radioactive isotopes for medical use, new methods of medical isotope production are being pursued. Many of these ...are small in size and could effectively operate continuously. With the potential for much shorter retention times, a new suite of isotopes may soon be found in the environment. The authors estimate that many more aerosols containing low-level isotopes of gas/volatile origin could be detectable at short range and times, and a few at longer ranges and times as compared to those released in more common nuclear reactor operations.
•New Medical Isotope production (MIP) facilities are coming online.•Modeled novel and classical medical isotope production techniques.•MDA values have been calculated for a multidimensional gamma-spectrometer.•New MIP methods may result in the environmental detection of additional isotopes.
Over the past several years, the Pacific Northwest National Laboratory (PNNL) has developed an ultra-low-background proportional counter (ULBPC) technology. The resulting detector is the product of ...an effort to produce a low-background, physically robust gas proportional counter for applications like radon emanation measurements, groundwater tritium, and
37
Ar. In order to fully take advantage of the inherent low-background properties designed into the ULBPC, a comparably low-background dedicated counting system is required. An ultra-low-background counting system (ULBCS) was recently built in the new shallow underground laboratory at PNNL. With a design depth of 30 m water-equivalent, the shallow underground laboratory provides approximately 100× fewer fast neutrons and 6× fewer muons than a surface location. The ULBCS itself provides additional shielding in the form of active anti-cosmic veto (via 2-in-thick plastic scintillator paddles) and passive borated poly (1 in.), lead (6 in.), and copper (~3 in.) shielding. This work will provide details on PNNL’s new shallow underground laboratory, examine the motivation for the design of the counting system, and provide results from the characterization of the ULBCS, including initial detector background.
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