New computing technologies inspired by the brain promise fundamentally different ways to process information with extreme energy efficiency and the ability to handle the avalanche of unstructured and ...noisy data that we are generating at an ever-increasing rate. To realize this promise requires a brave and coordinated plan to bring together disparate research communities and to provide them with the funding, focus and support needed. We have done this in the past with digital technologies; we are in the process of doing it with quantum technologies; can we now do it for brain-inspired computing?
A novel experimental method is presented to determine the optical efficiency and the loss channels of a luminescent solar concentrator (LSC). Despite strong promise, LSCs have not yet reached their ...full potential due to various mechanisms affecting the device's optical efficiency. Among those loss channels, escape cone and non-unity quantum yield losses are generally the most dominant. To further advance the field of LSCs, it is vital to understand the impact of each independently. So far, researchers have only characterized the total loss in LSCs. Here, an experimental method is proposed to separate the contribution from each individual loss channel. The experimental apparatus is the same as used for quantum yield measurements of fluorophores in solid samples. Therefore, the setup is commonly available to research groups already involved in LSC research. The accuracy of this method is demonstrated by comparing the experimental results with Monte-Carlo ray tracing. Our experimental method can have a strong impact on LSC research as it offers a means to unveil the loss channels of LSCs in addition to the optical efficiency.
•A novel method to characterize luminescent solar concentrators is proposed.•For the very first time the main loss channels can be distinguished.•The results are independent of excitation wavelength which simplifies measurements.•The experimental setup required is the same as used for quantum yield measurements.•Experimental results are validated by Monte-Carlo ray tracing.
Abstract
Artificial neural networks are notoriously power- and time-consuming when implemented on conventional von Neumann computing systems. Consequently, recent years have seen an emergence of ...research in machine learning hardware that strives to bring memory and computing closer together. A popular approach is to realise artificial neural networks in hardware by implementing their synaptic weights using memristive devices. However, various device- and system-level non-idealities usually prevent these physical implementations from achieving high inference accuracy. We suggest applying a well-known concept in computer science—committee machines—in the context of memristor-based neural networks. Using simulations and experimental data from three different types of memristive devices, we show that committee machines employing ensemble averaging can successfully increase inference accuracy in physically implemented neural networks that suffer from faulty devices, device-to-device variability, random telegraph noise and line resistance. Importantly, we demonstrate that the accuracy can be improved even without increasing the total number of memristors.
We describe the synthesis of charge-stabilised gold and silver nanoparticles by a modified Turkevich method and their interaction with a selection of cationic and anionic dyes. It was found that gold ...nanoparticles interact strongly with cationic dyes and in some cases enhanced absorption was observed by UV-visible spectroscopy. It is also shown that addition of cationic dyes to gold nanoparticles triggers aggregation of the nanoparticles into large, micrometre-scale clusters. Simultaneous fragmentation and agglomeration of the gold nanoparticles was observed at high concentrations of cationic dye in the solution. These effects were not observed when gold nanoparticles were mixed with anionic dyes, nor for silver nanoparticles with either cationic or anionic dyes.
We describe the synthesis of charge-stabilised gold and silver nanoparticles by a modified Turkevich method and their interaction with a selection of cationic and anionic dyes.
Resistive switching offers a promising route to universal electronic memory, potentially replacing current technologies that are approaching their fundamental limits. In many cases switching ...originates from the reversible formation and dissolution of nanometre-scale conductive filaments, which constrain the motion of electrons, leading to the quantisation of device conductance into multiples of the fundamental unit of conductance, G0. Such quantum effects appear when the constriction diameter approaches the Fermi wavelength of the electron in the medium - typically several nanometres. Here we find that the conductance of silicon-rich silica (SiOx) resistive switches is quantised in half-integer multiples of G0. In contrast to other resistive switching systems this quantisation is intrinsic to SiOx, and is not due to drift of metallic ions. Half-integer quantisation is explained in terms of the filament structure and formation mechanism, which allows us to distinguish between systems that exhibit integer and half-integer quantisation.
Rare-earth doped materials are of crucial importance to optoelectronics, and are widely deployed in fibre amplifiers and solid-state lasers. This article summarises the present state of the art in ...this rapidly growing field. Recent developments in the areas of rare-earth doped semiconductors and insulators are discussed and new classes of materials that open up new possibilities for extended functionality and greater optoelectronic integration are described. Nanostructured materials and wide bandgap semiconductors are of particular interest, though recent developments in more traditional material systems are highlighted. Emphasis is placed on erbium-doped materials, as these are of the greatest importance for telecommunications applications, but a range of other rare-earth ions are also discussed.
Microbial processes are known to mediate selenium (Se) oxidation–reduction reactions, strongly influencing Se speciation, bioavailability, and transport throughout the environment. While these ...processes have commonly been studied in anaerobic bacteria, the role that aerobic fungi play in Se redox reactions could be important for Se‐rich soil systems, dominated by microbial activity. We quantified fungal growth, aerobic Se(IV, VI) reduction, and Se immobilization and volatilization in the presence of six, metal‐tolerant Ascomycete fungi. We found that the removal of dissolved Se was dependent on the fungal species, Se form (i.e., selenite or selenate), and Se concentration. All six species grew and removed dissolved Se(IV) or Se(VI) from solution, with five species reducing both oxyanions to Se(0) biominerals, and all six species removing at least 15%–20% of the supplied Se via volatilization. Growth rates of all fungi, however, decreased with increasing Se(IV,VI) concentrations. All fungi removed 85%–93% of the dissolved Se(IV) within 10 d in the presence of 0.01 mm Se(IV), although only about 20%–30% Se(VI) was removed when grown with 0.01 mm Se(VI). Fungi‐produced biominerals were typically 50‐ to 300‐nm‐diameter amorphous or paracrystalline spherical Se(0) nanoparticles. Our results demonstrate that activity of common soil fungi can influence Se form and distribution, and these organisms may therefore play a role in detoxifying Se‐polluted environments.
Abstract
The inner ∼200 pc region of the Galaxy contains a 4 million M
⊙
supermassive black hole (SMBH), significant quantities of molecular gas, and star formation and cosmic-ray energy densities ...that are roughly two orders of magnitude higher than the corresponding levels in the Galactic disk. At a distance of only 8.2 kpc, the region presents astronomers with a unique opportunity to study a diverse range of energetic astrophysical phenomena, from stellar objects in extreme environments, to the SMBH and star-formation-driven feedback processes that are known to influence the evolution of galaxies as a whole. We present a new survey of the Galactic center conducted with the South African MeerKAT radio telescope. Radio imaging offers a view that is unaffected by the large quantities of dust that obscure the region at other wavelengths, and a scene of striking complexity is revealed. We produce total-intensity and spectral-index mosaics of the region from 20 pointings (144 hr on-target in total), covering 6.5 square degrees with an angular resolution of 4″ at a central frequency of 1.28 GHz. Many new features are revealed for the first time due to a combination of MeerKAT’s high sensitivity, exceptional
u
,
v
-plane coverage, and geographical vantage point. We highlight some initial survey results, including new supernova remnant candidates, many new nonthermal filament complexes, and enhanced views of the Radio Arc bubble, Sagittarius A, and Sagittarius B regions. This project is a South African Radio Astronomy Observatory public legacy survey, and the image products are made available with this article.