We introduce a new approach for the robust control of quantum dynamics of strongly interacting many-body systems. Our approach involves the design of periodic global control pulse sequences to ...engineer desired target Hamiltonians that are robust against disorder, unwanted interactions and pulse imperfections. It utilizes a matrix representation of the Hamiltonian engineering protocol based on time-domain transformations of the Pauli spin operator along the quantization axis. This representation allows us to derive a concise set of algebraic conditions on the sequence matrix to engineer robust target Hamiltonians, enabling the simple yet systematic design of pulse sequences. We show that this approach provides an efficient framework to (i) treat any secular many-body Hamiltonian and engineer it into a desired form, (ii) target dominant disorder and interaction characteristics of a given system, (iii) achieve robustness against imperfections, (iv) provide optimal sequence length within given constraints, and (v) substantially accelerate numerical searches of pulse sequences. Using this systematic approach, we develop novel sets of pulse sequences for the protection of quantum coherence, optimal quantum sensing and quantum simulation. Finally, we experimentally demonstrate the robust operation of these sequences in a system with the most general interaction form.
Understanding the coordination of cell division timing is one of the outstanding questions in the field of developmental biology. One active control parameter of the cell cycle duration is ...temperature, as it can accelerate or decelerate the rate of biochemical reactions. However, controlled experiments at the cellular-scale are challenging due to the limited availability of biocompatible temperature sensors as well as the lack of practical methods to systematically control local temperatures and cellular dynamics. Here, we demonstrate a method to probe and control the cell division timing in Caenorhabditis elegans embryos using a combination of local laser heating and nanoscale thermometry. Local infrared laser illumination produces a temperature gradient across the embryo, which is precisely measured by in-vivo nanoscale thermometry using quantum defects in nanodiamonds. These techniques enable selective, controlled acceleration of the cell divisions, even enabling an inversion of division order at the two cell stage. Our data suggest that the cell cycle timing asynchrony of the early embryonic development in C. elegans is determined independently by individual cells rather than via cell-to-cell communication. Our method can be used to control the development of multicellular organisms and to provide insights into the regulation of cell division timings as a consequence of local perturbations.
Quantum metrology makes use of coherent superpositions to detect weak signals. While in principle the sensitivity can be improved by increasing the density of sensing particles, in practice this ...improvement is severely hindered by interactions between them. Using a dense ensemble of interacting electronic spins in diamond, we demonstrate a novel approach to quantum metrology. It is based on a new method of robust quantum control, which allows us to simultaneously eliminate the undesired effects associated with spin-spin interactions, disorder and control imperfections, enabling a five-fold enhancement in coherence time compared to conventional control sequences. Combined with optimal initialization and readout protocols, this allows us to break the limit for AC magnetic field sensing imposed by interactions, opening a promising avenue for the development of solid-state ensemble magnetometers with unprecedented sensitivity.
The dynamic structure factor is a central quantity describing the physics of quantum many-body systems, capturing structure and collective excitations of a material. In condensed matter, it can be ...measured via inelastic neutron scattering, which is an energy-resolving probe for the density fluctuations. In ultracold atoms, a similar approach could so far not be applied due to the diluteness of the system. Here, we report on a direct, real-time and non-destructive measurement of the dynamic structure factor of a quantum gas exhibiting cavity-mediated long-range interactions. The technique relies on inelastic scattering of photons, stimulated by the enhanced vacuum field inside a high finesse optical cavity. We extract the density fluctuations, their energy and lifetime while the system undergoes a structural phase transition. We observe an occupation of the relevant quasi-particle mode on the level of a few excitations, and provide a theoretical description of this dissipative quantum many-body system.
We investigate thermalization dynamics of a driven dipolar many-body quantum system through the stability of discrete time crystalline order. Using periodic driving of electronic spin impurities in ...diamond, we realize different types of interactions between spins and demonstrate experimentally that the interplay of disorder, driving and interactions leads to several qualitatively distinct regimes of thermalization. For short driving periods, the observed dynamics are well described by an effective Hamiltonian which sensitively depends on interaction details. For long driving periods, the system becomes susceptible to energy exchange with the driving field and eventually enters a universal thermalizing regime, where the dynamics can be described by interaction-induced dephasing of individual spins. Our analysis reveals important differences between thermalization of long-range Ising and other dipolar spin models.
Insights into complex phenomena in quantum matter can be gained from simulation experiments with ultracold atoms, especially in cases where theoretical characterization is challenging. However these ...experiments are mostly limited to short-range collisional interactions. Recently observed perturbative effects of long-range interactions were too weak to reach novel quantum phases. Here we experimentally realize a bosonic lattice model with competing short- and infinite-range interactions, and observe the appearance of four distinct phases - a superfluid, a supersolid, a Mott insulator and a charge density wave. Our system is based on an atomic quantum gas trapped in an optical lattice inside a high finesse optical cavity. The strength of the short-ranged on-site interactions is controlled by means of the optical lattice depth. The infinite-range interaction potential is mediated by a vacuum mode of the cavity and is independently controlled by tuning the cavity resonance. When probing the phase transition between the Mott insulator and the charge density wave in real-time, we discovered a behaviour characteristic of a first order phase transition. Our measurements have accessed a regime for quantum simulation of many-body systems, where the physics is determined by the intricate competition between two different types of interactions and the zero point motion of the particles.
Statistical mechanics underlies our understanding of macroscopic quantum systems. It is based on the assumption that out-of-equilibrium systems rapidly approach their equilibrium states, forgetting ...any information about their microscopic initial conditions. This fundamental paradigm is challenged by disordered systems, in which a slowdown or even absence of thermalization is expected. We report the observation of critical thermalization in a three dimensional ensemble of \(\sim 10^6\) electronic spins coupled via dipolar interactions. By controlling the spin states of nitrogen vacancy color centers in diamond, we observe slow, sub-exponential relaxation dynamics and identify a regime of power-law decay with disorder-dependent exponents; this behavior is modified at late times owing to many-body interactions. These observations are quantitatively explained by a resonance counting theory that incorporates the effects of both disorder and interactions.
Understanding quantum dynamics away from equilibrium is an outstanding challenge in the modern physical sciences. It is well known that out-of-equilibrium systems can display a rich array of ...phenomena, ranging from self-organized synchronization to dynamical phase transitions. More recently, advances in the controlled manipulation of isolated many-body systems have enabled detailed studies of non-equilibrium phases in strongly interacting quantum matter. As a particularly striking example, the interplay of periodic driving, disorder, and strong interactions has recently been predicted to result in exotic "time-crystalline" phases, which spontaneously break the discrete time-translation symmetry of the underlying drive. Here, we report the experimental observation of such discrete time-crystalline order in a driven, disordered ensemble of \(\sim 10^6\) dipolar spin impurities in diamond at room-temperature. We observe long-lived temporal correlations at integer multiples of the fundamental driving period, experimentally identify the phase boundary and find that the temporal order is protected by strong interactions; this order is remarkably stable against perturbations, even in the presence of slow thermalization. Our work opens the door to exploring dynamical phases of matter and controlling interacting, disordered many-body systems.
We experimentally study the influence of dissipation on the driven Dicke quantum phase transition, realized by coupling external degrees of freedom of a Bose-Einstein condensate to the light field of ...a high-finesse optical cavity. The cavity provides a natural dissipation channel, which gives rise to vacuum-induced fluctuations and allows us to observe density fluctuations of the gas in real-time. We monitor the divergence of these fluctuations over two orders of magnitude while approaching the phase transition and observe a behavior which significantly deviates from that expected for a closed system. A correlation analysis of the fluctuations reveals the diverging time scale of the atomic dynamics and allows us to extract a damping rate for the external degree of freedom of the atoms. We find good agreement with our theoretical model including both dissipation via the cavity field and via the atomic field. Utilizing a dissipation channel to non-destructively gain information about a quantum many-body system provides a unique path to study the physics of driven-dissipative systems.
Photons are excellent information carriers but normally pass through each other without consequence. Engineered interactions between photons would enable applications from quantum information ...processing to simulation of condensed matter systems. Using an ensemble of cold atoms strongly coupled to an optical cavity, we demonstrate experimentally that the transmission of light through a medium may be controlled with few photons and even by the electromagnetic vacuum field. The vacuum induces a group delay of 25 ns on the input optical pulse, corresponding to a light velocity of 1600 m/s, and a transparency of 40% that increases to 80% when the resonator is filled with 10 photons. This strongly nonlinear effect provides prospects for advanced quantum devices such as photon-number-state filters.
