The rapid development of the computational methods based on density functional theory, on the one hand, and of time-, energy-, and momentum-resolved spectroscopy, on the other hand, allows today an ...unprecedently detailed insight into the processes governing hot-electron relaxation dynamics, and, in particular, into the role of the electron-phonon coupling. Instead of focusing on the development of a particular method, theoretical or experimental, this review aims to treat the progress in the understanding of the electron-phonon coupling which can be gained from both, on the basis of recently obtained results. We start by defining several regimes of hot electron relaxation via electron-phonon coupling, with respect to the electron excitation energy. We distinguish between energy and momentum relaxation of hot electrons, and summarize, for several semiconductors of the IV and III-V groups, the orders of magnitude of different relaxation times in different regimes, on the basis of known experimental and numerical data. Momentum relaxation times of hot electrons become very short around 1 eV above the bottom of the conduction band, and such ultrafast relaxation mechanisms are measurable only in the most recent pump-probe experiments. Then, we give an overview of the recent progress in the experimental techniques allowing to obtain detailed information on the hot-electron relaxation dynamics, with the main focus on time-, energy-, and momentum-resolved photoemission experiments. The particularities of the experimental approach developed by one of us, which allows to capture time-, energy-, and momentum-resolved hot-electron distributions, as well as to measure momentum relaxation times of the order of 10 fs, are discussed. We further discuss the main advances in the calculation of the electron-phonon scattering times from first principles over the past ten years, in semiconducting materials. Ab initio techniques and efficient interpolation methods provide the possibility to calculate electron-phonon scattering times with high precision at reasonable numerical cost. We highlight the methods of analysis of the obtained numerical results, which allow to give insight into the details of the electron-phonon scattering mechanisms. Finally, we discuss the concept of hot electron ensemble which has been proposed recently to describe the hot-electron relaxation dynamics in GaAs, the applicability of this concept to other materials, and its limitations. We also mention some open problems.
We discuss the ultrafast evolution of the surface electronic structure of the topological insulator Bi2Te3 following a femtosecond laser excitation. Using time and angle-resolved photoelectron ...spectroscopy, we provide a direct real-time visualization of the transient carrier population of both the surface states and the bulk conduction band. We find that the thermalization of the surface states is initially determined by interband scattering from the bulk conduction band, lasting for about 0.5 ps; subsequently, few picoseconds are necessary for the Dirac cone nonequilibrium electrons to recover a Fermi-Dirac distribution, while their relaxation extends over more than 10 ps. The surface sensitivity of our measurements makes it possible to estimate the range of the bulk-surface interband scattering channel, indicating that the process is effective over a distance of 5 nm or less. This establishes a correlation between the nanoscale thickness of the bulk charge reservoir and the evolution of the ultrafast carrier dynamics in the surface Dirac cone.
The task of digitalizing meandering complex spaces in 3D is a challenging one even with the most advanced instrumentation like lightweight terrestrial laser scanner or portable/wearable Mobile ...Mapping Systems (MMSs). The complexity and extension of architectonic spaces such as staircases, corridors and passages are such that the acquisition time using static devices becomes prohibitive and the accuracy using mobile devices gets affected by drift error leading to warped models or requiring abundant control measurements. This paper presents a photogrammetric portable fisheye multicamera solution for the 3D survey of complex areas that aims at being both handy and fast in the acquisition as well as more reliable ad accurate than common MMSs. The paper showcases a stress test conducted on five complex reconstruction trajectories selected from the meandering connection passages of Milan’s Cathedral. The tests are constructed as worst-case scenario to evaluate the accuracy and drift error amount of the proposed system in open-ended unconstrained paths. The results, though still suffering from moderate drift error, highlights the potential of the solution, especially in retaining the overall shape and orthogonality of the architectonic elements acquired.
The research illustrated in this article aimed at identifying a good standard methodology to survey very narrow spaces during 3D investigation of Cultural Heritage. It is an important topic in ...today’s era of BIM modelling applied to Cultural Heritage. Spaces like staircases, corridors and passages are very common in the architectural or archaeological fields, and obtaining a 3D-oriented survey of those areas can be a very complex task when completeness of the model and high precision are requested. Photogrammetry appears to be the most promising solution in terms of versatility and manoeuvrability also considering the quality of the required data. Fisheye lenses were studied and tested in depth because of their significant advantage in the field of view if compared with rectilinear lenses. This advantage alone can be crucial to reduce the total amount of photos and, as a consequence, to obtain manageable data, to simplify the survey phase and to significantly reduce the elaboration time. In order to overcome the main issue that arise when using fisheye lenses, which is the lack of rules that can be employed to design the survey, a general mathematical formulation to precisely estimate the GSD (Ground Sampling Distance) for every optical projection is presented here. A complete survey of a real complex case study was performed in order to test and stress the proposed methodology, and to handle a fisheye-based survey from beginning to end: the photogrammetric survey of the Minguzzi Staircase. It is a complex service spiral-staircase located in the Duomo di Milano with a total height of 25 meters and characterized by a narrow walkable space about 70 centimetres wide.
Obtaining insight into microscopic cooperative effects is a fascinating topic in condensed matter research because, through self-coordination and collectivity, they can lead to instabilities with ...macroscopic impacts like phase transitions. We used femtosecond time- and angle-resolved photoelectron spectroscopy (trARPES) to optically pump and probe TbTe3, an excellent model system with which to study these effects. We drove a transient charge density wave melting, excited collective vibrations in TbTe3, and observed them through their time-, frequency-, and momentum-dependent influence on the electronic structure. We were able to identify the role of the observed collective vibration in the transition and to document the transition in real time. The information that we demonstrate as being accessible with trARPES will greatly enhance the understanding of all materials exhibiting collective phenomena.
The paper presents the case study of the complete 3D survey of the area of the Fort of Pietole in Borgo Virgilio using the Leica Pegasus Backpack wearable Mobile Mapping System (MMS). Surveying the ...site is challenging because of its complex topology on the one hand (with notably narrow passages) and because of the presence of vegetation on the other. The framework within which this research takes place is the Fort of Pietole survey project that aims at the extraction of the Digital Terrain Model (DTM) of the area and the georeferencing of the fort defensive structures. The requirement of the project is the 3D reconstruction of the whole area at an accuracy that stands between a big scale environmental survey and a small-scale architectonic survey (1 : 500). The project is the opportunity to discuss the state of the art of wearable MMS, and to test the versatility and accuracy outcomes of the Pegasus Backpack under varying and challenging condition (indoor-outdoor, even-uneven pavement, satellite covered-denied areas) with the ambitious goal to use only the backpack MMS to record all the data from the DTM to the indoor narrow structures.
The study of photoexcited strongly correlated materials is attracting growing interest since their rich phase diagram often translates into an equally rich out-of-equilibrium behaviour. With ...femtosecond optical pulses, electronic and lattice degrees of freedom can be transiently decoupled, giving the opportunity of stabilizing new states inaccessible by quasi-adiabatic pathways. Here we show that the prototype Mott-Hubbard material V
O
presents a transient non-thermal phase developing immediately after ultrafast photoexcitation and lasting few picoseconds. For both the insulating and the metallic phase, the formation of the transient configuration is triggered by the excitation of electrons into the bonding a
orbital, and is then stabilized by a lattice distortion characterized by a hardening of the A
coherent phonon, in stark contrast with the softening observed upon heating. Our results show the importance of selective electron-lattice interplay for the ultrafast control of material parameters, and are relevant for the optical manipulation of strongly correlated systems.
The advent of mobile mapping systems (MMSs) and computer vision algorithms has enriched a wide range of navigation and mapping tasks such as localisation, 3D motion estimation and 3D mapping. This ...study focuses on Visual Simultaneous Localisation and Mapping (V-SLAM) in the context of two in-houses MMSs: Ant3D, a patented five-fisheye multi-camera rig and GeoRizon, a high-resolution stereo fisheye rig. The aim is to leverage V-SLAM to enhance the systems performance in near-real-time and non-real-time 3D reconstruction applications. The research investigates both Monocular and Stereo V-SLAM applied to both MMSs and tackles the challenge of combining the V-SLAM estimated trajectory of one or a pair of cameras with known multi-camera relative orientation. We propose a state-of-the-art code that serves as a flexible and extensible platform for MMSs image acquisition and processing, along with an adapted version of the well-established ORB-SLAM3.0. Evaluation is performed in a cultural heritage challenging setup: the Minguzzi spiral staircase in the Duomo di Milano Cathedral. Performed tests highlight that introducing V-SLAM trajectories as well as pre-calibrated interior orientation and multi-camera constraints improve speed, applicability and accuracy of 3D surveys.
Photogrammetric applications nowadays envisage the use of more and more low-cost cameras such as those equipped on commercial UAV platforms. Typically, these low-grade cameras suffer from extreme ...radial distortion and strong vignetting among other defects. This, initiated a trend among the low-cost cameras’ manufacturers to try to hide the camera defects by applying software pre-corrections to the images. These Built-In Correction Profiles gets applied to both the JPG files, directly in-camera, and usually to the raw files as well, through the opcode functions of the DNG standard. In this paper we rise this issue that is still under-reported in the literature and further assess the accuracy implication of applying or discarding the Built-In Correction Profile in the scenario of UAV mapping. We tested the commercial UAV DJI Phantom 4 Pro v2 in a calibration environment and a field test to compare the performance of pre-corrected versus uncorrected images. In our tests, processing the original uncorrected images led to improved IO calibration and reduced bowing effect in the field test.
Multi-camera devices are increasingly popular in various metrological applications, including cultural heritage digitalisation, where these devices are adopted as low-cost alternatives to more ...traditional methods or mobile mapping systems. They can be of two types: panoramic and non-panoramic configurations, with the former usually more compact and ready-made off-the-shelves and the latter usually custom-developed for metrological applications. In the paper, we compare the accuracy and reliability performance of two types of multi-camera: the spherical camera INSTA 360 Pro2 and the custom multi-camera rig Ant3D. The case study is a challenging spiral staircase environment, typical in many cultural heritage survey projects. The processed image datasets were evaluated in the most common constrain scenario (GCPs at both ends of the staircase) and the worst-case scenario (open-ended path, GCPs at the start). The datasets were processed with precalibrated IO and various degrees of multi-camera constraints up to precalibrated relative orientations. The results highlight that the nominal scale 1:50 can be achieved, e.g. an accuracy of <2 cm plus complete and precise point clouds and mesh results.
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