The modeled robustness of the aridity response to climate change has already been well established: global drylands are expanding as increases in potential evapotranspiration outpace precipitation ...increases. This work considers three questions not previously addressed: (1) in which aridity zones are aridity trends expected to first emerge? (2) To what extent are future populations expected to experience changes in aridity? (3) For which locations and populations is aridity change determined by changes in precipitation versus temperature? Using a multi-model ensemble of general circulation models (GCMs) from the CMIP5 archives, together with population statistics from United Nations databases we find the following: (1) drier regions are projected to dry earlier, more severely and to a greater extent than humid regions. (2) By the end of the century, up to 700 million more people are projected to live in arid regions, with half of humankind living in regions experiencing drying of at least 5% and 3 billion experiencing 25% drying under a high emissions scenario. The largest populations to experience extreme drying are in Africa and Asia. According to GCMs, aridity increases have already begun to emerge in Northern Africa. Populations in sub-Saharan Africa appear to be the most vulnerable considering current water scarcity levels there. And (3) precipitation change is projected to drive the most severe drying in arid regions, contributing to the earliest emerging signals of aridity change and driving the differential drying across aridity zones. A comparison of aridity data derived from observations with model ensemble data suggests that increased aridity is already emerging in the driest regions. In sum, widespread aridity trends across a warming state imply that most of humanity will live in a more arid world.
This book examines the discourse on ‘primitive thinking’ in early 20th century Germany. It explores texts from the social sciences, writings on art and language and – most centrally – literary works ...by Robert Musil, Walter Benjamin, Gottfried Benn and Robert Müller, focusing on three figures of alterity prominent in European primitivism: indigenous cultures, children, and the mentally ill.
Simulation of polar ozone depletion: An update Solomon, Susan; Kinnison, Doug; Bandoro, Justin ...
Journal of geophysical research. Atmospheres,
16 August 2015, Letnik:
120, Številka:
15
Journal Article
Recenzirano
Odprti dostop
We evaluate polar ozone depletion chemistry using the specified dynamics version of the Whole Atmosphere Community Climate Model for the year 2011. We find that total ozone depletion in both ...hemispheres is dependent on cold temperatures (below 192 K) and associated heterogeneous chemistry on polar stratospheric cloud particles. Reactions limited to warmer temperatures above 192 K, or on binary liquid aerosols, yield little modeled polar ozone depletion in either hemisphere. An imposed factor of three enhancement in stratospheric sulfate increases ozone loss by up to 20 Dobson unit (DU) in the Antarctic and 15 DU in the Arctic in this model. Such enhanced sulfate loads are similar to those observed following recent relatively small volcanic eruptions since 2005 and imply impacts on the search for polar ozone recovery. Ozone losses are strongly sensitive to temperature, with a test case cooler by 2 K producing as much as 30 DU additional ozone loss in the Antarctic and 40 DU in the Arctic. A new finding of this paper is the use of the temporal behavior and variability of ClONO2 and HCl as indicators of the efficacy of heterogeneous chemistry. Transport of ClONO2 from the southern subpolar regions near 55–65°S to higher latitudes near 65–75°S provides a flux of NOx from more sunlit latitudes to the edge of the vortex and is important for ozone loss in this model. Comparisons between modeled and observed total column and profile ozone perturbations, ClONO2 abundances, and the rate of change of HCl bolster confidence in these conclusions.
Key Points
Ozone loss chemistry strongly depends on polar stratospheric clouds and temperatures below 192 K
ClONO2 and HCl seasonal changes and variability are key indicators of chemistry
Transport of ClONO2 from the edge of the vortex to higher latitudes affects ozone loss
The severity of damaging human-induced climate change depends not only on the magnitude of the change but also on the potential for irreversibility. This paper shows that the climate change that ...takes place due to increases in carbon dioxide concentration is largely irreversible for 1,000 years after emissions stop. Following cessation of emissions, removal of atmospheric carbon dioxide decreases radiative forcing, but is largely compensated by slower loss of heat to the ocean, so that atmospheric temperatures do not drop significantly for at least 1,000 years. Among illustrative irreversible impacts that should be expected if atmospheric carbon dioxide concentrations increase from current levels near 385 parts per million by volume (ppmv) to a peak of 450-600 ppmv over the coming century are irreversible dry-season rainfall reductions in several regions comparable to those of the "dust bowl" era and inexorable sea level rise. Thermal expansion of the warming ocean provides a conservative lower limit to irreversible global average sea level rise of at least 0.4-1.0 m if 21st century CO₂ concentrations exceed 600 ppmv and 0.6-1.9 m for peak CO₂ concentrations exceeding almost equal to1,000 ppmv. Additional contributions from glaciers and ice sheet contributions to future sea level rise are uncertain but may equal or exceed several meters over the next millennium or longer.
The response of the Southern Ocean to a repeating seasonal cycle of ozone loss is studied in two coupled climate models and is found to comprise both fast and slow processes. The fast response is ...similar to the interannual signature of the southern annular mode (SAM) on sea surface temperature (SST), onto which the ozone hole forcing projects in the summer. It comprises enhanced northward Ekman drift, inducing negative summertime SST anomalies around Antarctica, earlier sea ice freeze-up the following winter, and northward expansion of the sea ice edge year-round. The enhanced northward Ekman drift, however, results in upwelling of warm waters from below the mixed layer in the region of seasonal sea ice. With sustained bursts of westerly winds induced by ozone hole depletion, this warming from below eventually dominates over the cooling from anomalous Ekman drift. The resulting slow time-scale response (years to decades) leads to warming of SSTs around Antarctica and ultimately a reduction in sea ice cover year-round. This two-time-scale behavior—rapid cooling followed by slow but persistent warming—is found in the two coupled models analyzed: one with an idealized geometry and the other with a complex global climate model with realistic geometry. Processes that control the time scale of the transition from cooling to warming and their uncertainties are described. Finally the implications of these results are discussed for rationalizing previous studies of the effect of the ozone hole on SST and sea ice extent.
Celotno besedilo
Dostopno za:
BFBNIB, DOBA, IZUM, KILJ, NUK, PILJ, PNG, SAZU, SIK, UILJ, UKNU, UL, UM, UPUK
Stratospheric ozone depletion through catalytic chemistry involving man‐made chlorofluorocarbons is an area of focus in the study of geophysics and one of the global environmental issues of the ...twentieth century. This review presents a brief history of the science of ozone depletion and describes a conceptual framework to explain the key processes involved, with a focus on chemistry. Observations that may be considered as evidence (fingerprints) of ozone depletion due to chlorofluorocarbons are explored, and the related gas phase and surface chemistry is described. Observations of ozone and of chlorine‐related trace gases near 40 km provide evidence that gas phase chemistry has indeed currently depleted about 10% of the stratospheric ozone there as predicted, and the vertical and horizontal structures of this depletion are fingerprints for that process. More striking changes are observed each austral spring in Antarctica, where about half of the total ozone column is depleted each September, forming the Antarctic ozone hole. Measurements of large amounts of ClO, a key ozone destruction catalyst, are among the fingerprints showing that human releases of chlorofluorocarbons are the primary cause of this change. Enhanced ozone depletion in the Antarctic and Arctic regions is linked to heterogeneous chlorine chemistry that occurs on the surfaces of polar stratospheric clouds at cold temperatures. Observations also show that some of the same heterogeneous chemistry occurs on the surfaces of particles present at midlatitudes as well, and the abundances of these particles are enhanced following explosive volcanic eruptions. The partitioning of chlorine between active forms that destroy ozone and inert reservoirs that sequester it is a central part of the framework for our understanding of the 40‐km ozone decline, the Antarctic ozone hole, the recent Arctic ozone losses in particularly cold years, and the observation of record midlatitude ozone depletion after the major eruption of Mount Pinatubo in the early 1990s. As human use of chlorofluorocarbons continues to decrease, these changes throughout the ozone layer are expected to gradually reverse during the twenty‐first century.
Industrial chlorofluorocarbons that cause ozone depletion have been phased out under the Montreal Protocol. A chemically driven increase in polar ozone (or "healing") is expected in response to this ...historic agreement. Observations and model calculations together indicate that healing of the Antarctic ozone layer has now begun to occur during the month of September. Fingerprints of September healing since 2000 include (i) increases in ozone column amounts, (ii) changes in the vertical profile of ozone concentration, and (iii) decreases in the areal extent of the ozone hole. Along with chemistry, dynamical and temperature changes have contributed to the healing but could represent feedbacks to chemistry. Volcanic eruptions have episodically interfered with healing, particularly during 2015, when a record October ozone hole occurred after the Calbuco eruption.
The Montreal Protocol has begun to heal the Antarctic ozone hole and avoided more global warming than any other treaty. Still, recent research shows that new unexpected emissions of several ...chlorofluorocarbons, carbon tetrachloride, and hydrofluorocarbons, are undermining the Protocol’s success. It is time for policymakers to plug the holes in the ozone hole treaty.
Chlorofluorocarbons (CFCs) are harmful ozone depleting substances and greenhouse gases. CFC production was phased-out under the Montreal Protocol, however recent studies suggest new and unexpected ...emissions of CFC-11. Quantifying CFC emissions requires accurate estimates of both atmospheric lifetimes and ongoing emissions from old equipment (i.e. 'banks'). In a Bayesian framework we simultaneously infer lifetimes, banks and emissions of CFC-11, 12 and 113 using available constraints. We find lifetimes of all three gases are likely shorter than currently recommended values, suggesting that best estimates of inferred emissions are larger than recent evaluations. Our analysis indicates that bank emissions are decreasing faster than total emissions, and we estimate new, unexpected emissions during 2014-2016 were 23.2, 18.3, and 7.8 Gg/yr for CFC-11, 12 and 113, respectively. While recent studies have focused on unexpected CFC-11 emissions, our results call for further investigation of potential sources of emissions of CFC-12 and CFC-113, along with CFC-11.
Virtually all metrics of Atlantic tropical cyclone activity show substantial increases over the past two decades. It is argued here that cooling near the tropical tropopause and the associated ...decrease in tropical cyclone outflow temperature contributed to the observed increase in tropical cyclone potential intensity over this period. Quantitative uncertainties in the magnitude of the cooling are important, but a broad range of observations supports some cooling. Downscalings of the output of atmospheric general circulation models (AGCMs) that are driven by observed sea surface temperatures and sea ice cover produce little if any increase in Atlantic tropical cyclone metrics over the past two decades, even though observed variability before roughly 1970 is well simulated by some of the models. Part of this shortcoming is traced to the failure of the AGCMs examined to reproduce the observed cooling of the lower stratosphere and tropical tropopause layer (TTL) over the past few decades. The authors caution against using sea surface temperature or proxies based on it to make projections of tropical cyclone activity as there can be significant contributions from other variables such as the outflow temperature. The proposed mechanisms of TTL cooling (e.g., ozone depletion and stratospheric circulation changes) are reviewed, and the need for improved representations of these processes in global models in order to improve projections of future tropical cyclone activity is emphasized.
Celotno besedilo
Dostopno za:
BFBNIB, DOBA, IZUM, KILJ, NUK, PILJ, PNG, SAZU, SIK, UILJ, UKNU, UL, UM, UPUK