Changes to the El Niño/Southern Oscillation (ENSO) and its atmospheric teleconnections under climate change are investigated using simulations conducted for the Coupled Model Intercomparison Project ...(CMIP5). The overall response to CO2increases is determined using 27 models, and the ENSO amplitude change based on the multi‐model mean is indistinguishable from zero. However, changes between ensembles run with a given model are sometimes significant: for four of the eleven models having ensemble sizes larger than three, the 21st century change to ENSO amplitude is statistically significant. In these four models, changes to SST and wind stress do not differ substantially from those in the models with no ENSO response, indicating that mean changes are not predictive of the ENSO sensitivity to climate change. Also, ocean vertical stratification is less (more) sensitive to CO2in models where ENSO strengthens (weakens), likely due to a regulation of the subsurface temperature structure by ENSO‐related poleward heat transport. Atmospheric teleconnections also show differences between models where ENSO amplitude does and does not respond to climate change; in the former case El Niño/La Niña‐related sea level pressure anomalies strengthen with CO2, and in the latter they weaken and shift polewards and eastwards. These results illustrate the need for large ensembles to isolate significant ENSO climate change responses, and for future work on diagnosing the dynamical causes of inter‐model teleconnection differences.
Key Points
ENSO amplitude is insignificant in the majority of IPCC‐class models
ENSO amplitude change is not due to mean state or seasonal cycle changes
The teleconnection response is sensitive to the ENSO amplitude change
On interannual to decadal time scales, the climate mode with many of the strongest societal impacts is the El Niño–Southern Oscillation (ENSO). However, quantifying ENSO's changes in a warming ...climate remains a formidable challenge, due to both the noise arising from internal variability and the complexity of air‐sea feedbacks in the tropical Pacific Ocean. In this work, we use large (≥30‐member) ensembles of climate simulations to show that anthropogenic climate change can produce systematic increases in ENSO teleconnection strength over many land regions, driving increased interannual variability in regional temperature extremes and wildfire frequency. As the spatial character of this intensification exhibits strong land‐ocean contrasts, a causal role for land‐atmosphere feedbacks is suggested. The identified increase in variance occurs in multiple model ensembles, independent of changes in sea surface temperature variance. This suggests that in addition to changes in the overall likelihoods of heat and wildfire extremes, the variability in these events may also be a robust feature of future climate.
Plain Language Summary
Changes in climate variability strongly affect the overall impacts of climate change. In this work, increases in the intensity of heat waves and wildfire driven by El Niño/La Niña in a business‐as‐usual climate scenario are identified in recently produced climate simulations spanning the 20th and 21st centuries. The intensification in temperature extremes occurs mainly over land regions and independently of changes in eastern Pacific sea surface temperature variability. It is argued that land atmosphere feedbacks are likely to play a key role in the simulated amplification, with relevance to impacts such as heat waves and wildfire frequency.
Key Points
Intensity increases in temperature and wildfire extremes driven by ENSO in a warming climate are identified in climate model large ensembles
The intensification occurs mainly over land regions and is influenced by precipitation
Land‐atmosphere feedbacks are likely to play a key role in the projected amplification
Ozone holds a certain fascination in atmospheric science. It is ubiquitous in the atmosphere, central to tropospheric oxidation chemistry, yet harmful to human and ecosystem health as well as being ...an important greenhouse gas. It is not emitted into the atmosphere but is a byproduct of the very oxidation chemistry it largely initiates. Much effort is focused on the reduction of surface levels of ozone owing to its health and vegetation impacts, but recent efforts to achieve reductions in exposure at a country scale have proved difficult to achieve owing to increases in background ozone at the zonal hemispheric scale. There is also a growing realisation that the role of ozone as a short-lived climate pollutant could be important in integrated air quality climate change mitigation. This review examines current understanding of the processes regulating tropospheric ozone at global to local scales from both measurements and models. It takes the view that knowledge across the scales is important for dealing with air quality and climate change in a synergistic manner. The review shows that there remain a number of clear challenges for ozone such as explaining surface trends, incorporating new chemical understanding, ozone-climate coupling, and a better assessment of impacts. There is a clear and present need to treat ozone across the range of scales, a transboundary issue, but with an emphasis on the hemispheric scales. New observational opportunities are offered both by satellites and small sensors that bridge the scales.
A chronology of global air quality Fowler, David; Brimblecombe, Peter; Burrows, John ...
Philosophical transactions of the Royal Society of London. Series A: Mathematical, physical, and engineering sciences,
10/2020, Letnik:
378, Številka:
2183
Journal Article
Recenzirano
Odprti dostop
Air pollution has been recognized as a threat to human health since the time of Hippocrates,
ca
400 BC. Successive written accounts of air pollution occur in different countries through the following ...two millennia until measurements, from the eighteenth century onwards, show the growing scale of poor air quality in urban centres and close to industry, and the chemical characteristics of the gases and particulate matter. The industrial revolution accelerated both the magnitude of emissions of the primary pollutants and the geographical spread of contributing countries as highly polluted cities became the defining issue, culminating with the great smog of London in 1952. Europe and North America dominated emissions and suffered the majority of adverse effects until the latter decades of the twentieth century, by which time the transboundary issues of acid rain, forest decline and ground-level ozone became the main environmental and political air quality issues. As controls on emissions of sulfur and nitrogen oxides (SO
2
and NO
x
) began to take effect in Europe and North America, emissions in East and South Asia grew strongly and dominated global emissions by the early years of the twenty-first century. The effects of air quality on human health had also returned to the top of the priorities by 2000 as new epidemiological evidence emerged. By this time, extensive networks of surface measurements and satellite remote sensing provided global measurements of both primary and secondary pollutants. Global emissions of SO
2
and NO
x
peaked, respectively, in
ca
1990 and 2018 and have since declined to 2020 as a result of widespread emission controls. By contrast, with a lack of actions to abate ammonia, global emissions have continued to grow.
This article is part of a discussion meeting issue ‘Air quality, past present and future’.
Abstract
The LIGO/Virgo gravitational-wave observatories have detected at least 50 double black hole (BH) coalescences. This sample is large enough to have allowed several recent studies to draw ...conclusions about the implied branching ratios between isolated binaries versus dense stellar clusters as the origin of double BHs. It has also led to the exciting suggestion that the population is highly likely to contain primordial BHs. Here we demonstrate that such conclusions cannot yet be robust because of the large current uncertainties in several key aspects of binary stellar evolution. These include the development and survival of a common envelope, the mass and angular-momentum loss during binary interactions, mixing in stellar interiors, pair-instability mass loss, and supernova outbursts. Using standard tools such as the rapid population synthesis codes
StarTrack
and
COMPAS
and the detailed stellar evolution code
MESA
, we examine as a case study the possible future evolution of Melnick 34, the most massive known binary star system (with initial component masses of 144
M
⊙
and 131
M
⊙
). We show that, despite its fairly well-known orbital architecture, various assumptions regarding stellar and binary physics predict a wide variety of outcomes: from a close BH–BH binary (which would lead to a potentially detectable coalescence), through a wide BH–BH binary (which might be seen in microlensing observations), or a Thorne–Żytkow object, to a complete disruption of both objects by a pair-instability supernova. Thus, because the future of massive binaries is inherently uncertain, sound predictions about the properties of BH–BH systems formed in the isolated binary evolution scenario are highly challenging at this time. Consequently, it is premature to draw conclusions about the formation channel branching ratios that involve isolated binary evolution for the LIGO/Virgo BH–BH merger population.
The role of anthropogenic aerosols in future projections (up to 2100) of summertime precipitation and precipitation extremes over the Asian monsoon region is investigated, by comparing two sets of ...the Community Earth System Model (CESM1) large ensemble simulations under the Representative Concentration Pathway 8.5 scenario (RCP8.5) and the corresponding scenario with aerosol fixed at 2005 levels (RCP8.5_FixA). The model is verified to be performing well in capturing present-day (1986–2005) climate and precipitation extremes. Our results suggest that the Asian monsoon region would become progressively warmer and wetter in the future under RCP8.5, while precipitation extremes will be significantly aggravated due to anthropogenic aerosol mitigation, particularly over East Asia. Specifically, aerosol reductions are found to shift the distribution of precipitation mean and extremes to larger values. For example, aerosol reductions would result in an increased likelihood of extreme precipitation (e.g. the maximum consecutive 5-day precipitation amount) and related disasters. Sensitivities of changes in precipitation mean and extremes to local warming from aerosol reductions are much larger than that from greenhouse gas increases. This is particularly important over East Asia in accordance with larger magnitudes of aerosol reductions compared to South Asia. Finally, by investigating the response of the climate system to aerosol changes, our findings demonstrate that aerosol induced precipitation changes would be dominated by aerosol–radiation–cloud forcing over northern East Asia and aerosol forcing induced large-scale circulation anomalies over southern East and South Asia.
We analyse historical (1850–2014) atmospheric hydroxyl
(OH) and methane lifetime data from Coupled Model Intercomparison Project
Phase 6 (CMIP6)/Aerosols and Chemistry Model Intercomparison Project
...(AerChemMIP) simulations. Tropospheric OH changed little from 1850 up to
around 1980, then increased by around 9 % up to 2014, with an associated
reduction in methane lifetime. The model-derived OH trends from 1980 to 2005
are broadly consistent with trends estimated by several studies that infer
OH from inversions of methyl chloroform and associated measurements; most
inversion studies indicate decreases in OH since 2005. However, the model
results fall within observational uncertainty ranges. The upward trend in
modelled OH since 1980 was mainly driven by changes in anthropogenic
near-term climate forcer emissions (increases in anthropogenic nitrogen
oxides and decreases in CO). Increases in halocarbon emissions since 1950
have made a small contribution to the increase in OH, whilst increases in
aerosol-related emissions have slightly reduced OH. Halocarbon emissions
have dramatically reduced the stratospheric methane lifetime by about
15 %–40 %; most previous studies assumed a fixed stratospheric lifetime.
Whilst the main driver of atmospheric methane increases since 1850 is
emissions of methane itself, increased ozone precursor emissions have
significantly modulated (in general reduced) methane trends. Halocarbon and
aerosol emissions are found to have relatively small contributions to
methane trends. These experiments do not isolate the effects of climate
change on OH and methane evolution; however, we calculate residual terms that
are due to the combined effects of climate change and non-linear
interactions between drivers. These residual terms indicate that non-linear
interactions are important and differ between the two methodologies we use
for quantifying OH and methane drivers. All these factors need to be
considered in order to fully explain OH and methane trends since 1850; these
factors will also be important for future trends.
We use a state-of-the-art regional chemistry transport model (WRF-Chem v4.2.1) to simulate particulate air pollution over northern India during September–November 2016. This period includes a severe ...air pollution episode marked by exceedingly high levels of hourly PM2.5 (particulate matter having an aerodynamic diameter ≤ 2.5 µm) during 30 October to 7 November, particularly over the wider Indo-Gangetic Plain (IGP). We provide a comprehensive evaluation of simulated seasonal meteorology (nudged by ERA5 reanalysis products) and aerosol chemistry (PM2.5 and its black carbon (BC) component) using a range of ground-based, satellite and reanalysis products, with a focus on the November 2016 haze episode. We find the daily and diurnal features in simulated surface temperature show the best agreement followed by relative humidity, with the largest discrepancies being an overestimate of night-time wind speeds (up to 1.5 m s−1) confirmed by both ground and radiosonde observations. Upper-air meteorology comparisons with radiosonde observations show excellent model skill in reproducing the vertical temperature gradient (r>0.9). We evaluate modelled PM2.5 at 20 observation sites across the IGP including eight in Delhi and compare simulated aerosol optical depth (AOD) with data from four AERONET sites. We also compare our model aerosol results with MERRA-2 reanalysis aerosol fields and MODIS satellite AOD. We find that the model captures many features of the observed aerosol distributions but tends to overestimate PM2.5 during September (by a factor of 2) due to too much dust, and underestimate peak PM2.5 during the severe episode. Delhi experiences some of the highest daily mean PM2.5 concentrations within the study region, with dominant components nitrate (∼25 %), dust (∼25 %), secondary organic aerosols (∼20 %) and ammonium (∼10 %). Modelled PM2.5 and BC spatially correlate well with MERRA-2 products across the whole domain. High AOD at 550nm across the IGP is also well predicted by the model relative to MODIS satellite (r≥0.8) and ground-based AERONET observations (r≥0.7), except during September. Overall, the model realistically captures the seasonal and spatial variations of meteorology and ambient pollution over northern India. However, the observed underestimations in pollutant concentrations likely come from a combination of underestimated emissions, too much night-time dispersion, and some missing or poorly represented aerosol chemistry processes. Nevertheless, we find the model is sufficiently accurate to be a useful tool for exploring the sources and processes that control PM2.5 levels during severe pollution episodes.