The acceleration of ions from ultrathin foils has been investigated by using 250 TW, subpicosecond laser pulses, focused to intensities of up to 3 × 10(20) W cm(-2). The ion spectra show the ...appearance of narrow-band features for protons and carbon ions peaked at higher energies (in the 5-10 MeV/nucleon range) and with significantly higher flux than previously reported. The spectral features and their scaling with laser and target parameters provide evidence of a multispecies scenario of radiation pressure acceleration in the light sail mode, as confirmed by analytical estimates and 2D particle-in-cell simulations. The scaling indicates that monoenergetic peaks with more than 100 MeV/nucleon are obtainable with moderate improvements of the target and laser characteristics, which are within reach of ongoing technical developments.
Abstract
Palladium promotion and deposition on
monoclinic
zirconia are effective strategies to boost the performance of bulk In
2
O
3
in CO
2
-to-methanol and could unlock superior reactivity if well ...integrated into a single catalytic system. However, harnessing synergic effects of the individual components is crucial and very challenging as it requires precise control over their assembly. Herein, we present ternary Pd-In
2
O
3
-ZrO
2
catalysts prepared by flame spray pyrolysis (FSP) with remarkable methanol productivity and improved metal utilization, surpassing their binary counterparts. Unlike established impregnation and co-precipitation methods, FSP produces materials combining low-nuclearity palladium species associated with In
2
O
3
monolayers highly dispersed on the ZrO
2
carrier, whose surface partially transforms from a
tetragonal
into a
monoclinic-
like structure upon reaction. A pioneering protocol developed to quantify oxygen vacancies using in situ electron paramagnetic resonance spectroscopy reveals their enhanced generation because of this unique catalyst architecture, thereby rationalizing its high and sustained methanol productivity.
Abstract
Helical coil accelerators are a recent development in laser-driven ion production, acting on the intrinsically wide divergence and broadband energy spectrum of laser-accelerated protons to ...deliver ultra-low divergence and quasi-monoenergetic beams. The modularity of helical coil accelerators also provides the attractive prospective of multi-staging. Here we show, on a proof-of-principle basis, a two-stage configuration which allows optical tuning of the energy of the selected proton beamlet. Experimental data, corroborated by particle tracing simulations, highlights the importance of controlling precisely the beam injection. Efficient post-acceleration of the protons with an energy gain up to ∼16 MeV (∼8 MeV per stage, at an average rate of ∼1 GeV m
−1
) was achieved at an optimal time delay, which allows synchronisation of the selected protons with the accelerating longitudinal electric fields to be maintained through both stages.
Highly anisotropic, beam-like neutron emission with peak flux of the order of 109 n/sr was obtained from light nuclei reactions in a pitcher-catcher scenario, by employing MeV ions driven by a ...sub-petawatt laser. The spatial profile of the neutron beam, fully captured for the first time by employing a CR39 nuclear track detector, shows a FWHM divergence angle of ∼ 70 ° , with a peak flux nearly an order of magnitude higher than the isotropic component elsewhere. The observed beamed flux of neutrons is highly favourable for a wide range of applications, and indeed for further transport and moderation to thermal energies. A systematic study employing various combinations of pitcher-catcher materials indicates the dominant reactions being d(p, n+p)1H and d(d,n)3He. Albeit insufficient cross-section data are available for modelling, the observed anisotropy in the neutrons' spatial and spectral profiles is most likely related to the directionality and high energy of the projectile ions.
We report on the temporally and spatially resolved detection of the precursory stages that lead to the formation of an unmagnetized, supercritical collisionless shock in a laser-driven laboratory ...experiment. The measured evolution of the electrostatic potential associated with the shock unveils the transition from a current free double layer into a symmetric shock structure, stabilized by ion reflection at the shock front. Supported by a matching particle-in-cell simulation and theoretical considerations, we suggest that this process is analogous to ion reflection at supercritical collisionless shocks in supernova remnants.
The shaping of astrophysical outflows into bright, dense, and collimated jets due to magnetic pressure is here investigated using laboratory experiments. Here we look at the impact on jet collimation ...of a misalignment between the outflow, as it stems from the source, and the magnetic field. For small misalignments, a magnetic nozzle forms and redirects the outflow in a collimated jet. For growing misalignments, this nozzle becomes increasingly asymmetric, disrupting jet formation. Our results thus suggest outflow/magnetic field misalignment to be a plausible key process regulating jet collimation in a variety of objects from our Sun's outflows to extragalatic jets. Furthermore, they provide a possible interpretation for the observed structuring of astrophysical jets. Jet modulation could be interpreted as the signature of changes over time in the outflow/ambient field angle, and the change in the direction of the jet could be the signature of changes in the direction of the ambient field.
We present a study on laser-driven proton acceleration from a hydrogen cluster target. Aiming for the optimisation of the proton source, we performed a detailed parametric scan of the interaction ...conditions by varying different laser and the target parameters. While the underlying process of a Coulomb-explosion delivers moderate energies, in the range of 100 s of keV, the use of hydrogen as target material comes with the benefit of a debris-free, single-species proton acceleration scheme, enabling high repetition-rate experiments, which are very robust against shot-to-shot fluctuations.
Abstract
We study the laser-driven acceleration of electrons from overdense hydrogen clusters to energies of up to 13 MeV in laser forward direction and several hundreds of keV in an outer ...ring-structure. The use of cryogenic hydrogen allows for high repetition-rate operation and examination of the influence of source parameters like temperature and gas flow. The outer ring-structure of accelerated electrons, originating from the interaction, that is robust against the change of laser and target parameters can be observed for low electron densities of ca 3 × 10
16
cm
−3
. For higher electron densities, an additional central spot of electrons in the laser forward direction can be observed. Utilizing 3D particle-in-cell simulations, it is revealed that both electron populations mainly stem from ponderomotive scattering.
The dynamics of magnetic fields with an amplitude of several tens of megagauss, generated at both sides of a solid target irradiated with a high-intensity (~10(19) W/cm(2)) picosecond laser pulse, ...has been spatially and temporally resolved using a proton imaging technique. The amplitude of the magnetic fields is sufficiently large to have a constraining effect on the radial expansion of the plasma sheath at the target surfaces. These results, supported by numerical simulations and simple analytical modeling, may have implications for ion acceleration driven by the plasma sheath at the rear side of the target as well as for the laboratory study of self-collimated high-energy plasma jets.
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