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Shen, L; Jellyman, E; Forgan, E M; Blackburn, E; Laver, M; Canévet, E; Schefer, J; He, Z; Itoh, M
Physical review. B, 08/2017, Letnik: 96, Številka: 5Journal Article
We have explored the magnetism in the nongeometrically frustrated spin-chain system γ−CoV2O6 which possesses a complex magnetic exchange network. Our neutron diffraction patterns at low temperatures (T≤TN=6.6 K) are best described by a model in which two magnetic phases coexist in a volume ratio 65(1) : 35(1), with each phase consisting of a single spin modulation. This model fits previous studies and our observations better than the model proposed by Lenertz et al. J. Phys. Chem. C 118, 13981 (2014), which consisted of one phase with two spin modulations. By decreasing the temperature from TN, the minority phase of our model undergoes an incommensurate-commensurate lock-in transition at T*=5.6 K. Based on these results, we propose that phase separation is an alternative approach for degeneracy-lifting in frustrated magnets.
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