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Skorobogatov, S A; Nikitin, S E; Shaykhutdinov, K A; Balaev, A D; Terentjev, K Yu; Ehlers, G; Sala, G; Pomjakushina, E V; Conder, K; Podlesnyak, A
Physical review. B, 01/2020, Letnik: 101, Številka: 1Journal Article
We investigate the magnetic dynamics of the orthorhombic perovskite TmFeO3 at low temperatures, below the spin reorientation transition at TSR≈80 K, by means of time-of-flight neutron spectroscopy. We find that the magnetic excitation spectrum combines two emergent collective modes associated with different magnetic sublattices. The Fe subsystem orders below TN∼632 K into a canted antiferromagnetic structure and exhibits sharp, high-energy magnon excitations. We describe them using linear spin-wave theory, and reveal a pronounced anisotropy between in- and out-of-plane exchange interactions, which was mainly neglected in previous reports on the spin dynamics in orthoferrites. At lower energies, we find two crystalline electrical field (CEF) excitations of Tm3+ ions at energies of ∼2 and 5 meV. In contrast to the sister compound YbFeO3, where the Yb3+ ions form quasi-one-dimensional chains along the c axis, the Tm excitations show dispersion along both directions in the (0KL) scattering plane. Analysis of the neutron scattering polarization factor reveals a longitudinal polarization of the 2 meV excitation. To evaluate the effect of the CEF on the Tm3+ ions, we perform point-charge model calculations, and their results quantitatively capture the main features of Tm single-ion physics, such as energies, intensities, and polarization of the CEF transitions, and the type of magnetic anisotropy.
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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