We simulate the radiation belt electron flux enhancements during selected Geospace Environment Modeling (GEM) challenge events to quantitatively compare the major processes involved in relativistic electron acceleration under different conditions. Van Allen Probes observed significant electron flux enhancement during both the storm time of 17–18 March 2013 and non–storm time of 19–20 September 2013, but the distributions of plasma waves and energetic electrons for the two events were dramatically different. During 17–18 March 2013, the SYM‐H minimum reached −130 nT, intense chorus waves (peak Bw ~140 pT) occurred at 3.5 < L < 5.5, and several hundred keV to several MeV electron fluxes increased by ~2 orders of magnitude mostly at 3.5 < L < 5.5. During 19–20 September 2013, the SYM‐H remained higher than −30 nT, modestly intense chorus waves (peak Bw ~80 pT) occurred at L > 5.5, and electron fluxes at energies up to 3 MeV increased by a factor of ~5 at L > 5.5. The two electron flux enhancement events were simulated using the available wave distribution and diffusion coefficients from the GEM focus group Quantitative Assessment of Radiation Belt Modeling. By comparing the individual roles of local electron heating and radial transport, our simulation indicates that resonant interaction with chorus waves is the dominant process that accounts for the electron flux enhancement during the storm time event particularly near the flux peak locations, while radial diffusion by ultralow‐frequency waves plays a dominant role in the enhancement during the non–storm time event. Incorporation of both processes reasonably reproduces the observed location and magnitude of electron flux enhancement. Key Points Energetic electron fluxes are enhanced during storm and non–storm time events, but wave and electron structures are dramatically different Local heating by whistler mode chorus wave is the major contributor to the flux enhancement near the peak during 17–18 March 2013 Radial diffusion by ultralow‐frequency wave is the major contributor to the observed flux enhancement during 19–20 September 2013