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Liu, Xun-Gao; Tao, Chen-Lei; Yu, Huang-Qin; Chen, Bin; Liu, Zhen; Zhu, Gen-Ping; Zhao, Zujin; Shen, Liang; Tang, Ben Zhong
Journal of materials chemistry. C, Materials for optical and electronic devices, 2018, Letnik: 6, Številka: 12Journal Article
In this work, we synthesized a dicarboxyl-substituted tetraphenylethene (TPE) ligand, 4,4′-(1,2-diphenylethene-1,2-diyl)dibenzoic acid (H 2 BCTPE), with a prominent aggregation-induced emission (AIE) feature. A two-fold interpenetrated luminescent metal–organic framework (LMOF) Zn 4 O(BCTPE) 3 ( 1 ) with Zn 4 O(CO 2 ) 6 nodes is prepared using the trans -isomer of H 2 BCTPE as a ligand, which shows a typical behavior of microporous materials and a high fluorescence quantum yield of 64.5%. The solvent free 1 is thermally stable, water stable and highly emissive. The suspension of solvent-free 1 in water exhibits high quenching efficiencies and low detection limits towards nitro-containing explosives ( e.g. nitrobenzene, 4-nitrophenol, 2,4,6-trinitrophenol), and nitro-containing antibiotics ( e.g. metronidazole and nitrofurazone). The solvent-free 1 can be a promising alternative to efficiently detect nitro-containing explosives and antibiotics under aqueous conditions.
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