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Yao, Shenglai; stner, Viktoria; Menezes, Prashanth W; Panda, Chakadola; Mebs, Stefan; Zolnhofer, Eva M; Miehlich, Matthias E; Szilvási, Tibor; Nanjundan, Ashok Kumar; Haumann, Michael; Meyer, Karsten; Grützmacher, Hansjörg; Driess, Matthias
Chemical science, 2018, Letnik: 9, Številka: 45Journal Article
In large-scale, hydrogen production from water-splitting represents the most promising solution for a clean, recyclable, and low-cost energy source. The realization of viable technological solutions requires suitable efficient electrochemical catalysts with low overpotentials and long-term stability for both hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) based on cheap and nontoxic materials. Herein, we present a unique molecular approach to monodispersed, ultra-small, and superiorly active iron phosphide (FeP) electrocatalysts for bifunctional OER, HER, and overall water-splitting. They result from transformation of a molecular iron phosphide precursor, containing a Fe2P3 core with mixed-valence FeIIFeIII sites bridged by an asymmetric cyclo-P(2+1)3− ligand. The as-synthesized FeP nanoparticles act as long-lasting electrocatalysts for OER and HER with low overpotential and high current densities that render them one of the best-performing electrocatalysts hitherto known. The fabricated alkaline electrolyzer delivered low cell voltage with durability over weeks, representing an attractive catalyst for large-scale water-splitting technologies.
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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in: SICRIS
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