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Jahan, Maryam; Bao, Qiaoliang; Loh, Kian Ping
Journal of the American Chemical Society, 04/2012, Letnik: 134, Številka: 15Journal Article
Pyridine-functionalized graphene (reduced graphene oxide) can be used as a building block in the assembly of metal organic framework (MOF). By reacting the pyridine-functionalized graphene with iron–porphyrin, a graphene–metalloporphyrin MOF with enhanced catalytic activity for oxygen reduction reactions (ORR) is synthesized. The structure and electrochemical property of the hybrid MOF are investigated as a function of the weight percentage of the functionalized graphene added to the iron–porphyrin framework. The results show that the addition of pyridine-functionalized graphene changes the crystallization process of iron–porphyrin in the MOF, increases its porosity, and enhances the electrochemical charge transfer rate of iron–porphyrin. The graphene–metalloporphyrin hybrid shows facile 4-electron ORR and can be used as a promising Pt-free cathode in alkaline Direct Methanol Fuel Cell.
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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in: SICRIS
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