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Hofer, Corinne J; Grass, Robert N; Schneider, Elia M; Hendriks, Lyndsey; Herzog, Antoine F; Zeltner, Martin; Günther, Detlef; Stark, Wendelin J
01/2018, Letnik: 9, Številka: 2Journal Article
Selective dealloying of metal nanoparticles results in rattle-type hollow carbon nanoshells enclosing platinum nanoparticles, which are able to perform size-selective catalysis. Selective functionalization of the outer graphene-like carbon surface prevents agglomeration and leads to well dispersible nanocatalysts in aqueous solutions. The synthesis starts with the production of nanoparticles with a cobalt-platinum-alloy core surrounded by graphene-like carbon via reducing flame spray synthesis. After surface functionalization, simultaneous pore formation in the shell-wall and dissolution of the cobalt results in platinum encapsulated in hollow carbon nanospheres. Catalytic oxidation of differently sized sugars (glucose and maltoheptaose) reveales size-selective catalytic properties of these platinum nanorattles. Surface-functionalized hollow carbon nanobubbles containing platinum in their interior perform size-selective catalysis.
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