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Liu, Yun; Mao, Yanyan; Tang, Xiaoxiao; Xu, Yin; Li, Chengcheng; Li, Feng
Chinese journal of catalysis, October 2017, 2017-10-00, Letnik: 38, Številka: 10Journal Article
A novel plasmonic photo-Fenton catalyst of Ag/AgCl/Fe-S was synthesized by ion exchange and photoreduction methods. The obtained catalyst was characterized by X-ray diffraction, X-ray photoelectron spectroscopy, scanning electron microscope imaging, and Brunauer-Emmett-Teller measurements. Moreover, the photocatalytic activity of Ag/AgCl/Fe-S was investigated for its degradation activity towards bisphenol A (BPA) as target pollutant under visible light irradiation. The effects of H2O2 concentration, pH value, illumination intensity, and catalyst dosage on BPA degradation were examined. Our results indicated that the Ag/AgCl material was successfully loaded onto Fe-sepiolite and showed a high photocatalytic activity under illumination by visible light. Furthermore, active species capture experiments were performed to explore the photocatalytic mechanism of the Ag/AgCl/Fe-S in this heterogeneous photo-Fenton process, where the major active species included hydroxyl radicals (•OH) and holes (h+). In a heterogeneous photo-Fenton system •OH radicals and holes are the major active species contributing to the high photocatalytic activity of Ag/AgCl/Fe-S catalyst.
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Leto | Faktor vpliva | Izdaja | Kategorija | Razvrstitev | ||||
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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in: SICRIS
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