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Liu, Huijun; Zeng, Jiajie; Guo, Jingjing; Nie, Han; Zhao, Zujin; Tang, Ben Zhong
Angewandte Chemie International Edition, July 20, 2018, Letnik: 57, Številka: 30Journal Article
Non‐doped organic light‐emitting diodes (OLEDs) possess merits of higher stability and easier fabrication than doped devices. However, luminescent materials with high exciton use are generally unsuitable for non‐doped OLEDs because of severe emission quenching and exciton annihilation in neat films. Herein, we wish to report a novel molecular design of integrating aggregation‐induced delayed fluorescence (AIDF) moiety within host materials to explore efficient luminogens for non‐doped OLEDs. By grafting 4‐(phenoxazin‐10‐yl)benzoyl to common host materials, we develop a series of new luminescent materials with prominent AIDF property. Their neat films fluoresce strongly and can fully harvest both singlet and triplet excitons with suppressed exciton annihilation. Non‐doped OLEDs of these AIDF luminogens exhibit excellent luminance (ca. 100000 cd m−2), outstanding external quantum efficiencies (21.4–22.6 %), negligible efficiency roll‐off and improved operational stability. To the best of our knowledge, these are the most efficient non‐doped OLEDs reported so far. This convenient and versatile molecular design is of high significance for the advance of non‐doped OLEDs. Robust emitters, affording high‐performance non‐doped organic light‐emitting diodes with outstanding external quantum efficiencies (EQE) of up to 22.6 % and negligible efficiency roll‐off, have been obtained by molecularly integrating an aggregation‐induced delayed fluorescence (AIDF) luminogen into a host material.
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