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Galyamin, Dmitry; Torrero, Jorge; Rodríguez, Isabel; Kolb, Manuel J; Ferrer, Pilar; Pascual, Laura; Salam, Mohamed Abdel; Gianolio, Diego; Celorrio, Verónica; Mokhtar, Mohamed; Garcia Sanchez, Daniel; Gago, Aldo Saul; Friedrich, Kaspar Andreas; Peña, Miguel A; Alonso, José Antonio; Calle-Vallejo, Federico; Retuerto, María; Rojas, Sergio
Nature communications, 04/2023, Letnik: 14, Številka: 1Journal Article
Abstract The production of green hydrogen in water electrolyzers is limited by the oxygen evolution reaction (OER). State-of-the-art electrocatalysts are based on Ir. Ru electrocatalysts are a suitable alternative provided their performance is improved. Here we show that low-Ru-content pyrochlores (R 2 MnRuO 7 , R = Y, Tb and Dy) display high activity and durability for the OER in acidic media. Y 2 MnRuO 7 is the most stable catalyst, displaying 1.5 V at 10 mA cm −2 for 40 h, or 5000 cycles up to 1.7 V. Computational and experimental results show that the high performance is owed to Ru sites embedded in RuMnO x surface layers. A water electrolyser with Y 2 MnRuO 7 (with only 0.2 mg Ru cm −2 ) reaches 1 A cm −2 at 1.75 V, remaining stable at 200 mA cm −2 for more than 24 h. These results encourage further investigation on Ru catalysts in which a partial replacement of Ru by inexpensive cations can enhance the OER performance.
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