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Hameed, S; Pelc, D; Anderson, Z W; Klein, A; Spieker, R J; Yue, L; Das, B; Ramberger, J; Lukas, M; Liu, Y; Krogstad, M J; Osborn, R; Li, Y; Leighton, C; Fernandes, R M; Greven, M
Nature materials, 01/2022, Letnik: 21, Številka: 1Journal Article
The properties of quantum materials are commonly tuned using experimental variables such as pressure, magnetic field and doping. Here we explore a different approach using irreversible, plastic deformation of single crystals. We show that compressive plastic deformation induces low-dimensional superconductivity well above the superconducting transition temperature (T ) of undeformed SrTiO , with evidence of possible superconducting correlations at temperatures two orders of magnitude above the bulk T . The enhanced superconductivity is correlated with the appearance of self-organized dislocation structures, as revealed by diffuse neutron and X-ray scattering. We also observe deformation-induced signatures of quantum-critical ferroelectric fluctuations and inhomogeneous ferroelectric order using Raman scattering. Our results suggest that strain surrounding the self-organized dislocation structures induces local ferroelectricity and quantum-critical dynamics that strongly influence T , consistent with a theory of superconductivity enhanced by soft polar fluctuations. Our results demonstrate the potential of plastic deformation and dislocation engineering for the manipulation of electronic properties of quantum materials.
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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in: SICRIS
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