Thin, binder-less zeolite NaX laminates, with thicknesses ranging between 310 to 750 μm and widths exceeding 50 mm and biaxial tensile strength in excess of 3 MPa, were produced by pulsed current processing. The NaX laminates displayed a high CO adsorption capacity and high binary CO -over-N and CO -over-CH selectivity, suitable for CO capture from flue gas and upgrading of raw biogas. The thin laminates displayed a rapid CO uptake; NaX laminates with a thickness of 310 μm were saturated to 40% of their CO capacity within 24 seconds. The structured laminates of 310 μm thickness and 50 mm thickness would offer low pressure drop and efficient carbon capture performance in a laminate-based swing adsorption technology.