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Liu, J Y; J Yu; Ning, J L; Yi, H M; Miao, L; Min, L J; Zhao, Y F; Ning, W; Lopez, K A; Zhu, Y L; Pillsbury, T; Zhang, Y B; Wang, Y; J Hu; Cao, H B; Balakirev, F; Weickert, F; Jaime, M; Lai, Y; Yang, Kun; Sun, J W; Alem, N; Gopalan, V; Chang, C Z; Samarth, N; Liu, C X; Mcdonald, R D; Mao, Z Q
arXiv.org, 11/2020Paper
Spin-valley locking in the band structure of monolayers of MoS\(_2\) and other group-VI dichalcogenides has attracted enormous interest, since it offers potential for valleytronic and optoelectronic applications. Such an exotic electronic state has sparsely been seen in bulk materials. Here, we report spin-valley locking in a bulk Dirac semimetal BaMnSb\(_2\). We find valley and spin are inherently coupled for both valence and conduction bands in this material. This is revealed by comprehensive studies using first principle calculations, tight-binding and effective model analyses, angle-resolved photoemission spectroscopy and quantum transport measurements. Moreover, this material also exhibits a stacked quantum Hall effect. The spin-valley degeneracy extracted from the plateau height of quantized Hall resistivity is close to 2. This result, together with the observed Landau level spin splitting, further confirms the spin-valley locking picture. In the extreme quantum limit, we have also observed a two-dimensional chiral metal at the side surface, which represents a novel topological quantum liquid. These findings establish BaMnSb\(_2\) as a rare platform for exploring coupled spin and valley physics in bulk single crystals and accessing 3D interacting topological states.
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