In this study we use the ERA-Interim reanalysis data set from the European Centre for Medium-Range Weather Forecasts (ECMWF) and a refined version of a previously developed Lagrangian methodology to ...compile a global 33 yr climatology of stratosphere–troposphere exchange (STE) from 1979 to 2011. Fluxes of mass and ozone are calculated across the tropopause, pressure surfaces in the troposphere, and the top of the planetary boundary layer (PBL). This climatology provides a state-of-the-art quantification of the geographical distribution of STE and the preferred transport pathways, as well as insight into the temporal evolution of STE during the last 33 yr. We confirm the distinct zonal and seasonal asymmetry found in previous studies using comparable methods. The subset of "deep STE", where stratospheric air reaches the PBL within 4 days or vice versa, shows especially strong geographical and seasonal variations. The global hotspots for deep STE are found along the west coast of North America and over the Tibetan Plateau, especially in boreal winter and spring. An analysis of the time series reveals significant positive trends of the net downward mass flux and of deep STE in both directions, which are particularly large over North America. The downward ozone flux across the tropopause is dominated by the seasonal cycle of ozone concentrations at the tropopause and peaks in summer, when the mass flux is nearly at its minimum. For the subset of deep STE events, the situation is reversed and the downward ozone flux into the PBL is dominated by the mass flux and peaks in early spring. Thus surface ozone concentration along the west coast of North America and around the Tibetan Plateau are likely to be influenced by deep stratospheric intrusions. We discuss the sensitivity of our results on the choice of the control surface representing the tropopause, the horizontal and vertical resolution of the trajectory starting grid, and the minimum residence time τ used to filter out transient STE trajectories.
The Himalayas and the Tibetan Plateau region (HTP), despite being a remote and sparsely populated area, is regularly exposed to polluted air masses with significant amounts of aerosols including ...black carbon. These dark, light-absorbing particles are known to exert a great melting potential on mountain cryospheric reservoirs through albedo reduction and radiative forcing. This study combines ground-based and satellite remote sensing data to identify a severe aerosol pollution episode observed simultaneously in central Tibet and on the southern side of the Himalayas during 13-19 March 2009 (pre-monsoon). Trajectory calculations based on the high-resolution numerical weather prediction model COSMO are used to locate the source regions and study the mechanisms of pollution transport in the complex topography of the HTP. We detail how polluted air masses from an atmospheric brown cloud (ABC) over South Asia reach the Tibetan Plateau within a few days. Lifting and advection of polluted air masses over the great mountain range is enabled by a combination of synoptic-scale and local meteorological processes. During the days prior to the event, winds over the Indo-Gangetic Plain (IGP) are generally weak at lower levels, allowing for accumulation of pollutants and thus the formation of ABCs. The subsequent passing of synoptic-scale troughs leads to southwesterly flow in the middle troposphere over northern and central India, carrying the polluted air masses across the Himalayas. As the IGP is known to be a hotspot of ABCs, the cross-Himalayan transport of polluted air masses may have serious implications for the cryosphere in the HTP and impact climate on regional to global scales. Since the current study focuses on one particularly strong pollution episode, quantifying the frequency and magnitude of similar events in a climatological study is required to assess the total impact.
It is well known that the storm tracks are a preferred region of stratosphere-troposphere exchange (STE), but a systematic and climatological investigation of the connection between cyclones and STE ...has not yet been performed. We use two ERA-Interim climatologies of STE and cyclones for the years 1979-2011 to quantify the amount of STE that occurs during the life cycle of North Atlantic cyclones. A Lagrangian method serves to identify individual STE events, and a sophisticated cyclone identification tool detects cyclones, their shape and size from the sea-level pressure (SLP) field and from geopotential height anomalies at 300-700 hPa. Combining the two data sets reveals that roughly 50-60 % of the total STE in the North Atlantic occurs in the vicinity of cyclones and that both downward and upward fluxes of mass across the tropopause (STT and TST, respectively) are more intense in deeper cyclones (lower minimum SLP) compared to less intense cyclones. In summer, STT and TST in the vicinity of cyclones are almost equal; in the other seasons, STT is larger by 25-60 %. Compared to climatology, cross-tropopause mass fluxes are enhanced by a factor of about 1.29 and 1.06 for STT and TST, respectively, when a cyclone is present. On average, STE is strongest during the mature phase of cyclones, i.e., in a 24 h time window around the time of maximum intensity. Systematic patterns of exchange locations relative to the cyclone centre are identified via composite analysis and shed light on the different characteristics of STT and TST. During cyclone intensification and in the mature stage, TST is mainly confined to the cyclone centre, whereas STT occurs mainly in a region further southwest. During the decay of the cyclones, both STT and TST are most frequent close to the cyclone centre, in a region with a fairly low tropopause.
We study the contribution of tropopause folds in the summertime pool of tropospheric ozone over the eastern Mediterranean and the Middle East (EMME) with the aid of the ECHAM5/MESSy Atmospheric ...Chemistry (EMAC) model. Tropopause fold events in EMAC simulations were identified with a 3-D labeling algorithm that detects folds at grid points where multiple crossings of the dynamical tropopause are computed. Subsequently the events featuring the largest horizontal and vertical extent were selected for further study. For the selection of these events we identified a significant contribution of the stratospheric ozone reservoir to the high concentrations of ozone in the middle and lower free troposphere over the EMME. A distinct increase of ozone is found over the EMME in the middle troposphere during summer as a result of the fold activity, shifting towards the southeast and decreasing altitude. We find that the interannual variability of near-surface ozone over the eastern Mediterranean (EM) during summer is related to that of both tropopause folds and ozone in the free troposphere.
Stratospheric intrusion (SI) events are a topic of ongoing research, especially because of their ability to change the oxidation capacity of the troposphere and their contribution to tropospheric ...ozone levels. In this work, a novel tool called STEFLUX (Stratosphere-to-Troposphere Exchange Flux) is presented, discussed, and used to provide a first long-term investigation of SI over two global hot-spot regions for climate change and air pollution: the southern Himalayas and the central Mediterranean Basin. The main purpose of STEFLUX is to obtain a fast-computing and reliable identification of the SI events occurring at a specific location and during a specified time window. It relies on a compiled stratosphere-to-troposphere exchange (STE) climatology, which makes use of the ERA-Interim reanalysis dataset from the ECMWF, as well as a refined version of a well-established Lagrangian methodology. STEFLUX results are compared to the SI observations (SIO) at two high-mountain WMO/GAW global stations in these climate hot spots, i.e., the Nepal Climate Observatory-Pyramid (NCO-P, 5079 m a.s.l.) and Mt. Cimone (2165 m a.s.l.), which are often affected by SI events. Compared to the observational datasets at the two specific measurement sites, STEFLUX is able to detect SI events on a regional scale. Furthermore, it has the advantage of retaining additional information concerning the pathway of stratospheric-affected air masses, such as the location of tropopause crossing and other meteorological parameters along the trajectories. However, STEFLUX neglects mixing and dilution that air masses undergo along their transport within the troposphere. Therefore, the regional-scale STEFLUX events cannot be expected to perfectly reproduce the point measurements at NCO-P and Mt. Cimone, which are also affected by small-scale (orographic) circulations. Still, the seasonal variability in SI events according to SIO and STEFLUX agrees fairly well. By exploiting the fact that the ERA-Interim reanalysis extends back to 1979, the long-term climatology of SI events at NCO-P and Mt. Cimone is also assessed in this work. The analysis of the 35-year record at both stations denies the existence of any significant trend in the SI frequency, except for winter seasons at NCO-P. Furthermore, for the first time, by using the STEFLUX outputs, we investigate the potential impact of specific climate factors (i.e. ENSO, QBO, and solar activity) on SI frequency variability over the Mediterranean Basin and the Himalayas.
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