Recently launched multichannel geostationary Earth orbit (GEO) satellite
sensors, such as the Geostationary Ocean Color Imager (GOCI) and the Advanced
Himawari Imager (AHI), provide aerosol products ...over East Asia with high
accuracy, which enables the monitoring of rapid diurnal variations and the
transboundary transport of aerosols. Most aerosol studies to date have used
low Earth orbit (LEO) satellite sensors, such as the Moderate Resolution
Imaging Spectroradiometer (MODIS) and the Multi-angle Imaging
Spectroradiometer (MISR), with a maximum of one or two overpass daylight
times per day from midlatitudes to low latitudes. Thus, the demand for new GEO
observations with high temporal resolution and improved accuracy has been
significant. In this study the latest versions of aerosol optical depth
(AOD) products from three LEO sensors – MODIS (Dark Target, Deep Blue, and
MAIAC), MISR, and the Visible/Infrared Imager Radiometer Suite
(VIIRS), along with two GEO sensors (GOCI and AHI), are validated,
compared, and integrated for a period during the Korea–United States Air
Quality Study (KORUS-AQ) field campaign from 1 May to 12 June 2016 over East
Asia. The AOD products analyzed here generally have high accuracy with high
R (0.84–0.93) and low RMSE (0.12–0.17), but their error characteristics differ
according to the use of several different surface-reflectance estimation
methods. High-accuracy near-real-time GOCI and AHI measurements facilitate
the detection of rapid AOD changes, such as smoke aerosol transport from
Russia to Japan on 18–21 May 2016, heavy pollution transport from China to
the Korean Peninsula on 25 May 2016, and local emission transport from the Seoul
Metropolitan Area to the Yellow Sea in South Korea on 5 June 2016. These
high-temporal-resolution GEO measurements result in more representative
daily AOD values and make a greater contribution to a combined daily AOD
product assembled by median value selection with a 0.5∘×0.5∘ grid resolution. The combined AOD is spatially continuous and has
a greater number of pixels with high accuracy (fraction within expected
error range of 0.61) than individual products. This study characterizes
aerosol measurements from LEO and GEO satellites currently in operation over
East Asia, and the results presented here can be used to evaluate satellite
measurement bias and air quality models.
Since the first International Cooperative for Aerosol Prediction (ICAP) multi‐model ensemble (MME) study, the number of ICAP global operational aerosol models has increased from five to nine. An ...update of the current ICAP status is provided, along with an evaluation of the performance of ICAP‐MME over 2012–2017, with a focus on June 2016–May 2017. Evaluated with ground‐based Aerosol Robotic Network (AERONET) aerosol optical depth (AOD) and data assimilation quality MODerate‐resolution Imaging Spectroradiometer (MODIS) retrieval products, the ICAP‐MME AOD consensus remains the overall top‐scoring and most consistent performer among all models in terms of root‐mean‐square error (RMSE), bias and correlation for total, fine‐ and coarse‐mode AODs as well as dust AOD; this is similar to the first ICAP‐MME study. Further, over the years, the performance of ICAP‐MME is relatively stable and reliable compared to more variability in the individual models. The extent to which the AOD forecast error of ICAP‐MME can be predicted is also examined. Leading predictors are found to be the consensus mean and spread. Regression models of absolute forecast errors were built for AOD forecasts of different lengths for potential applications. ICAP‐MME performance in terms of modal AOD RMSEs of the 21 regionally representative sites over 2012–2017 suggests a general tendency for model improvements in fine‐mode AOD, especially over Asia. No significant improvement in coarse‐mode AOD is found overall for this time period.
International Cooperative for Aerosol Predictions (ICAP) model 550 nm total AOD RMSE of the 72 h forecast versus corresponding mean AODs for AERONET sites listed in Table 2. Large black dots are ICAP multi‐model ensemble consensus means. Individual models are in small coloured dots. Validation of fine‐ and coarse‐modal AODs and dust AOD is also available in Figure 2.
While stand alone satellite and model aerosol products see wide utilization, there is a significant need in numerous atmospheric and climate applications for a fused product on a regular grid. ...Aerosol data assimilation is an operational reality at numerous centers, and like meteorological reanalyses, aerosol reanalyses will see significant use in the near future. Here we present a standardized 2003–2013 global 1 × 1° and 6-hourly modal aerosol optical thickness (AOT) reanalysis product. This data set can be applied to basic and applied Earth system science studies of significant aerosol events, aerosol impacts on numerical weather prediction, and electro-optical propagation and sensor performance, among other uses. This paper describes the science of how to develop and score an aerosol reanalysis product. This reanalysis utilizes a modified Navy Aerosol Analysis and Prediction System (NAAPS) at its core and assimilates quality controlled retrievals of AOT from the Moderate Resolution Imaging Spectroradiometer (MODIS) on Terra and Aqua and the Multi-angle Imaging SpectroRadiometer (MISR) on Terra. The aerosol source functions, including dust and smoke, were regionally tuned to obtain the best match between the model fine- and coarse-mode AOTs and the Aerosol Robotic Network (AERONET) AOTs. Other model processes, including deposition, were tuned to minimize the AOT difference between the model and satellite AOT. Aerosol wet deposition in the tropics is driven with satellite-retrieved precipitation, rather than the model field. The final reanalyzed fine- and coarse-mode AOT at 550 nm is shown to have good agreement with AERONET observations, with global mean root mean square error around 0.1 for both fine- and coarse-mode AOTs. This paper includes a discussion of issues particular to aerosol reanalyses that make them distinct from standard meteorological reanalyses, considerations for extending such a reanalysis outside of the NASA A-Train era, and examples of how the aerosol reanalysis can be applied or fused with other model or remote sensing products. Finally, the reanalysis is evaluated in comparison with other available studies of aerosol trends, and the implications of this comparison are discussed.
Intense heating by wildfires can generate deep, smoke-infused thunderstorms, known as pyrocumulonimbus (pyroCb), which can release a large quantity of smoke particles above jet aircraft cruising ...altitudes. Injections of pyroCb smoke into the lower stratosphere have gained increasing attention over the past 15 years due to the rapid proliferation of satellite remote sensing tools. Impacts from volcanic eruptions and other troposphere-to-stratosphere exchange processes on stratospheric radiative and chemical equilibrium are well recognized and monitored. However, the role of pyroCb smoke in the climate system has yet to be acknowledged. Here, we show that the mass of smoke aerosol particles injected into the lower stratosphere from five near-simultaneous intense pyroCbs occurring in western North America on 12 August 2017 was comparable to that of a moderate volcanic eruption, and an order of magnitude larger than previous benchmarks for extreme pyroCb activity. The resulting stratospheric plume encircled the Northern Hemisphere over several months. By characterizing this event, we conclude that pyroCb activity, considered as either large singular events, or a full fire season inventory, significantly perturb the lower stratosphere in a manner comparable with infrequent volcanic intrusions.
In a companion paper (Xian et al., 2022, part 1 of the study), we present an Arctic aerosol optical depth (AOD) climatology and trend analysis for 2003-2019 spring and summertime periods derived from ...a combination of aerosol reanalyses, remote-sensing retrievals, and ground observations. Continued from the previous discussion and as the second part of the study, we report the statistics and trends of Arctic AOD extreme events using the U.S. Navy Aerosol Analysis and Prediction System ReAnalysis version 1 (NAAPS-RA v1), the sun photometer data from the AErosol RObotic NETwork (AERONET) sites, and the oceanic Maritime Aerosol Network (MAN) measurements. Here, extreme AOD events are defined as events with AOD exceeding the 95th percentile (denoted "AOD.sub.95 ") of AOD distributions for given locations using 6-hourly or daily AOD data. While AERONET and MAN data estimate the Arctic median 550 nm AOD value to be 0.07, the 95th percentile value is 0.24. Such extreme events are dominated by fine-mode aerosol particles, largely attributable to biomass burning (BB) smoke events for the North American Arctic, the Asian Arctic, and most areas of the Arctic Ocean. However, extreme AOD events for the lower European Arctic are more attributable to anthropogenic and biogenic fine particles. The extreme-event occurrence dominance of sea salt is largely limited to the North Atlantic and Norwegian Sea. The extreme AOD amplitudes of anthropogenic and biogenic fine-mode and sea salt AOD are, however, significantly lower than those regions where extreme smoke AOD is dominant. Even for sites distant from BB source regions, BB smoke is the principal driver of AOD variation above the AOD.sub.95 threshold.
Abstract
The Black Summer fire season of 2019–2020 in southeastern Australia contributed to an intense ‘super outbreak’ of fire-induced and smoke-infused thunderstorms, known as pyrocumulonimbus ...(pyroCb). More than half of the 38 observed pyroCbs injected smoke particles directly into the stratosphere, producing two of the three largest smoke plumes observed at such altitudes to date. Over the course of 3 months, these plumes encircled a large swath of the Southern Hemisphere while continuing to rise, in a manner consistent with existing nuclear winter theory. We connect cause and effect of this event by quantifying the fire characteristics, fuel consumption, and meteorology contributing to the pyroCb spatiotemporal evolution. Emphasis is placed on the unusually long duration of sustained pyroCb activity and anomalous persistence during nighttime hours. The ensuing stratospheric smoke plumes are compared with plumes injected by significant volcanic eruptions over the last decade. As the second record-setting stratospheric pyroCb event in the last 4 years, the Australian super outbreak offers new clues on the potential scale and intensity of this increasingly extreme fire-weather phenomenon in a warming climate.
Southeast Asia (SEA) hosts one of the most complex aerosol systems in the world, with convoluted meteorological scales, sharp geographic and socioeconomic features, high biological productivity, ...mixtures of a wide range of atmospheric pollutants, and likely a significant susceptibility to global climate change. This physical complexity of SEA is coupled with one of the world's most challenging environments for both in situ and remote sensing observation. The 7-Southeast Asian Studies (7SEAS) program was formed to facilitate interdisciplinary research into the integrated SEA aerosol environment via grass roots style collaboration. In support of the early 7SEAS program and the affiliated Southeast Asia Composition, Cloud, Climate Coupling Regional Study (SEAC4RS), this review was created to outline the network of connections linking aerosol particles in SEA with meteorology, climate and the total earth system. In this review, we focus on and repeatedly link back to our primary data source: satellite aerosol remote sensing and associated observability issues. We begin with a brief rationale for the program, outlining key aerosol impacts and, comparing their magnitudes to the relative uncertainty of observations. We then discuss aspects of SEA's physical, socio-economic and biological geography relevant to meteorology and observability issues associated with clouds and precipitation. We show that not only does SEA pose significant observability challenges for aerosol particles, but for clouds and precipitation as well. With the fundamentals of the environment outlined, we explore SEA's most studied aerosol issue: biomass burning. We summarize research on bulk aerosol properties for SEA, including a short synopsis of recent AERONET observations. We describe long range transport patterns. Finally, considerable attention is paid to satellite aerosol observability issues, with a face value comparison of common aerosol products in the region including passive and active aerosol products as well as fluxes. We show that satellite data products diverge greatly due to a host of known artifacts. These artifacts have important implications for how research is conducted, and care must be taken when using satellite products to study aerosol problems. The paper ends with a discussion of how the community can approach this complex and important environment.
► The complex relationships between Southeast Asia’s geographic, meteorological and aerosol systems are reviewed. ► There are few aerosol measurements in Southeast Asia, and those that do exist suggest significant regional variability. ► Southeast Asia hosts one of the world’s most challenging aerosol observing environments. ► Satellite derived products for clouds, precipitation, fire and aerosol diverge significantly in Southeast Asia. ► If used properly, satellite products can provide significant insight into the regional aerosol environment.
Abstract
The first observationally based conceptual model for intense pyrocumulonimbus (pyroCb) development is described by applying reanalyzed meteorological model output to an inventory of 26 ...intense pyroCb events from June to August 2013 and a control inventory of intense fire activity without pyroCb. Results are based on 88 intense wildfires observed within the western United States and Canada. While surface-based fire weather indices are a useful indicator of intense fire activity, they are not a skillful predictor of intense pyroCb. Development occurs when a layer of increased moisture content and instability is advected over a dry, deep, and unstable mixed layer, typically along the leading edge of an approaching disturbance or under the influence of a monsoonal anticyclone. Upper-tropospheric dynamics are conducive to rising motion and vertical convective development. Mid- and upper-tropospheric conditions therefore resemble those that produce traditional dry thunderstorms. The specific quantity of midlevel moisture and instability required is shown to be strongly dependent on the surface elevation of the contributing fire. Increased thermal buoyancy from large and intense wildfires can serve as a potential trigger, implying that pyroCb occasionally develop in the absence of traditional meteorological triggering mechanisms. This conceptual model suggests that meteorological conditions favorable for pyroCb are observed regularly in western North America. PyroCb and ensuing stratospheric smoke injection are therefore likely to be significant and endemic features of summer climate. Results from this study provide a major step toward improved detection, monitoring, and prediction of pyroCb, which will ultimately enable improved understanding of the role of this phenomenon in the climate system.
We present an Arctic aerosol optical depth (AOD) climatology and trend analysis for 2003-2019 spring and summertime periods derived from a combination of multi-agency aerosol reanalyses, ...remote-sensing retrievals, and ground observations. This includes the U.S. Navy Aerosol Analysis and Prediction System ReAnalysis version 1 (NAAPS-RA v1), the NASA Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), and the Copernicus Atmosphere Monitoring Service ReAnalysis (CAMSRA). Spaceborne remote-sensing retrievals of AOD are considered from the Moderate Resolution Imaging Spectroradiometer (MODIS), the Multi-angle Imaging SpectroRadiometer (MISR), and the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). Ground-based data include sun photometer data from AErosol RObotic NETwork (AERONET) sites and oceanic Maritime Aerosol Network (MAN) measurements. Aerosol reanalysis AODs and spaceborne retrievals show consistent climatological spatial patterns and trends for both spring and summer seasons over the lower Arctic (60-70.sup." N). Consistent AOD trends are also found for the high Arctic (north of 70.sup." N) from reanalyses. The aerosol reanalyses yield more consistent AOD results than climate models, can be verified well with AERONET, and corroborate complementary climatological and trend analysis. Speciated AODs are more variable than total AOD among the three reanalyses and a little more so for March-May (MAM) than for June-August (JJA). Black carbon (BC) AOD in the Arctic comes predominantly from biomass burning (BB) sources in both MAM and JJA, and BB overwhelms anthropogenic sources in JJA for the study period.
An accurate estimation of biomass burning emissions is partially limited by the lack of knowledge of fire burning phase (smoldering vs. flaming). In recent years, several fire detection products have ...been developed to provide information of fire radiative power (FRP), location, size, and temperature of fire pixels, but no information regarding fire burning phase is retrieved. The Day-Night band (DNB) aboard Visible Infrared Imaging Radiometer Suite (VIIRS) is sensitive to visible light from flaming fires in nighttime scenes. In contrast, VIIRS 4 μm moderate resolution band #13 (M13), though capable of detecting fires at all phases, has no direct sensitivity for discerning fire phase. However, the hybrid usage of VIIRS DNB and M-bands data is hampered by their different scanning technology and spatial resolution. In this study, we present a novel method to rapidly and accurately resample DNB pixel radiances to the footprint of M-band pixels, accounting for onboard detector aggregation schemes and bowtie effect removals. The visible energy fraction (VEF) is subsequently introduced as an indicator of fire burning phase. VEF is calculated as the ratio of visible light power (VLP) to FRP for each fire pixel retrieved from the VIIRS 750 m active fire product. A global distribution of VEF values is quantitatively obtained, showing smaller VEF values in regions with mostly smoldering wildfires, such as peatland fires in Indonesia, larger VEF values in regions with flaming wildfires over grasslands and savannas in the sub-Sahelian region, and the largest VEF values associated with gas flaring in the Middle East. Mean VEF for different land cover types or regions is highly correlated with modified combustion efficiency (MCE). These results, together with a case study of the 2018 California Camp Fire, show that the VEF has the potential to be an indicator of fire combustion phase for each fire pixel, appropriate for estimating emission factors at the satellite pixel level.
•Novel approach to resample VIIRS′ Day-Night-Band radiances to its M-band footprint.•Visible energy fraction (VEF) concept is mathematically defined for nighttime fires.•VEF is more effective than fire radiative power to describe fire phase.•VEF is a strong indicator of the modified combustion efficiency (MCE) of fires.•VEF is computed globally and captures MCE global variation for different biomes.