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Peer reviewed
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Sakai, K; Stoychev, S; Ouchi, T; Higuchi, I; Schöffler, M; Mazza, T; Fukuzawa, H; Nagaya, K; Yao, M; Tamenori, Y; Kuleff, A I; Saito, N; Ueda, K
Physical review letters, 01/2011, Volume: 106, Issue: 3Journal Article
We report the first observation of electron-transfer-mediated decay (ETMD) and interatomic Coulombic decay (ICD) from the triply charged states with an inner-valence vacancy, using the Ar dimer as an example. These ETMD and ICD processes, which lead to fragmentation of Ar(3+)-Ar into Ar(2+)-Ar(2+) and Ar(3+)-Ar+, respectively, are unambiguously identified by electron-ion-ion coincidence spectroscopy in which the kinetic energy of the ETMD or ICD electron and the kinetic energy release between the two fragment ions are measured in coincidence.
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