High Mobility Ambipolar Diketopyrrolopyrrole-Based Conjugated Polymer Synthesized Via Direct Arylation Polycondensation

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High Mobility Ambipolar Diketopyrrolopyrrole-Based Conjugated Polymer Synthesized Via Direct Arylation Polycondensation

Gao, Yao; Zhang, Xiaojie; Tian, Hongkun; Zhang, Jidong; Yan, Donghang; Geng, Yanhou; Wang, Fosong

Advanced materials (Weinheim), 11/2015, Volume: 27, Issue: 42

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A diketopyrrolopyrrole‐based conjugated polymer, PDPP‐4FTVT, which exhibits ambipolar transport behavior in air with hole and electron mobilities up to 3.40 and 5.86 cm2 V−1 s−1, respectively, is synthesized via direct arylation polycondensation. Incorporation of F‐atoms in β‐positions of thiophene rings dramatically improves the efficiency of direct arylation polycondensation.

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