An analysis of the Cloudnet data set collected at Leipzig, Germany, with special focus on mixed-phase layered clouds is presented. We derive liquid- and ice-water content together with vertical ...motions of ice particles falling through cloud base. The ice mass flux is calculated by combining measurements of ice-water content and particle Doppler velocity. The efficiency of heterogeneous ice formation and its impact on cloud lifetime is estimated for different cloud-top temperatures by relating the ice mass flux and the liquid-water content at cloud top. Cloud radar measurements of polarization and Doppler velocity indicate that ice crystals formed in mixed-phase cloud layers with a geometrical thickness of less than 350 m are mostly pristine when they fall out of the cloud.
We present particle optical properties of stratospheric smoke layers observed with multiwavelength polarization Raman lidar over Punta Arenas (53.2∘ S, 70.9∘ W), Chile, at the southernmost tip of ...South America in January 2020. The smoke originated from the record-breaking bushfires in Australia. The stratospheric aerosol optical thickness reached values up to 0.85 at 532 nm in mid-January 2020. The main goal of this rapid communication letter is to provide first stratospheric measurements of smoke extinction-to-backscatter ratios (lidar ratios) and particle linear depolarization ratios at 355 and 532 nm wavelengths. These aerosol parameters are important input parameters in the analysis of spaceborne CALIPSO and Aeolus lidar observations of the Australian smoke spreading over large parts of the Southern Hemisphere in January and February 2020 up to heights of around 30 km. Lidar and depolarization ratios, simultaneously measured at 355 and 532 nm, are of key importance regarding the homogenization of the overall Aeolus (355 nm wavelength) and CALIPSO (532 nm wavelength) lidar data sets documenting the spread of the smoke and the decay of the stratospheric perturbation, which will be observable over the entire year of 2020. We found typical values and spectral dependencies of the lidar ratio and linear depolarization ratio for aged stratospheric smoke. At 355 nm, the lidar ratio and depolarization ratio ranged from 53 to 97 sr (mean 71 sr) and 0.2 to 0.26 (mean 0.23), respectively. At 532 nm, the lidar ratios were higher (75–112 sr, mean 97 sr) and the depolarization ratios were lower with values of 0.14–0.22 (mean 0.18). The determined depolarization ratios for aged Australian smoke are in very good agreement with respective ones for aged Canadian smoke, observed with lidar in stratospheric smoke layers over central Europe in the summer of 2017. The much higher 532 nm lidar ratios, however, indicate stronger absorption by the Australian smoke particles.
For the first time, a closure study of the relationship between the ice-nucleating particle concentration (INP; INPC) and ice crystal number concentration (ICNC) in altocumulus and cirrus layers, ...solely based on ground-based active remote sensing, is presented. Such aerosol–cloud closure experiments are required (a) to better understand aerosol–cloud interaction in the case of mixed-phase clouds, (b) to explore to what extent heterogeneous ice nucleation can contribute to cirrus formation, which is usually controlled by homogeneous freezing, and (c) to check the usefulness of available INPC parameterization schemes, applied to lidar profiles of aerosol optical and microphysical properties up to the tropopause level. The INPC–ICNC closure studies were conducted in Cyprus (Limassol and Nicosia) during a 6-week field campaign in March–April 2015 and during the 17-month CyCARE (Cyprus Clouds Aerosol and Rain Experiment) campaign. The focus was on altocumulus and cirrus layers which developed in pronounced Saharan dust layers at heights from 5 to 11 km. As a highlight, a long-lasting cirrus event was studied which was linked to the development of a very strong dust-infused baroclinic storm (DIBS) over Algeria. The DIBS was associated with strong convective cloud development and lifted large amounts of Saharan dust into the upper troposphere, where the dust influenced the evolution of an unusually large anvil cirrus shield and the subsequent transformation into an cirrus uncinus cloud system extending from the eastern Mediterranean to central Asia, and thus over more than 3500 km. Cloud top temperatures of the three discussed closure study cases ranged from −20 to −57 ∘C. The INPC was estimated from polarization/Raman lidar observations in combination with published INPC parameterization schemes, whereas the ICNC was retrieved from combined Doppler lidar, aerosol lidar, and cloud radar observations of the terminal velocity of falling ice crystals, radar reflectivity, and lidar backscatter in combination with the modeling of backscattering at the 532 and 8.5 mm wavelengths. A good-to-acceptable agreement between INPC (observed before and after the occurrence of the cloud layer under investigation) and ICNC values was found in the discussed three proof-of-concept closure experiments. In these case studies, INPC and ICNC values matched within an order of magnitude (i.e., within the uncertainty ranges of the INPC and ICNC estimates), and they ranged from 0.1 to 10 L−1 in the altocumulus layers and 1 to 50 L−1 in the cirrus layers observed between 8 and 11 km height. The successful closure experiments corroborate the important role of heterogeneous ice nucleation in atmospheric ice formation processes when mineral dust is present. The observed long-lasting cirrus event could be fully explained by the presence of dust, i.e., without the need for homogeneous ice nucleation processes.
The Mediterranean region is a unique area characterized by a large spectrum of atmospheric phenomena, some of which have a high impact on many aspects of human activities, safety and wellbeing. The ...area is long considered as a hot spot of such atmospheric phenomena deserving multidisciplinary scientific attention. The scientific research that has been carried out on these high impact atmospheric processes that occur in the Mediterranean area is indeed widespread and the available international literature is very extensive. The paper touches initially the temperature and precipitation regimes, followed by a discussion of floods and droughts. The exciting cyclogenetic patterns of explosive cyclones and medicanes are presented in separate sections. The lightning activity and the presence of dust and other pollutants are also presented herein. The atmospheric chemistry of the region which is increasingly becoming of utmost importance for the area under study is distinctly discussed. Attempts to modify the weather (the precipitation, in particular) are outlined too. The effects of climatic change on various atmospheric processes are considered throughout this paper, in addition to a dedicated section on temperature and precipitation.
•Past and future trends of temperature and precipitation in the Mediterranean are presented.•Droughts, floods, lightning and weather modification practices in the Mediterranean area are discussed.•Mediterranean explosive cyclogenesis and medicanes are presented.•Aspects of Mediterranean atmospheric chemistry, dust and air pollution are exposed.•Challenges in Mediterranean climate projections are debated.
The HD(CP)2 Observational Prototype Experiment (HOPE) was performed as a major 2-month field experiment in Jülich, Germany, in April and May 2013, followed by a smaller campaign in Melpitz, Germany, ...in September 2013. HOPE has been designed to provide an observational dataset for a critical evaluation of the new German community atmospheric icosahedral non-hydrostatic (ICON) model at the scale of the model simulations and further to provide information on land-surface–atmospheric boundary layer exchange, cloud and precipitation processes, as well as sub-grid variability and microphysical properties that are subject to parameterizations. HOPE focuses on the onset of clouds and precipitation in the convective atmospheric boundary layer. This paper summarizes the instrument set-ups, the intensive observation periods, and example results from both campaigns. HOPE-Jülich instrumentation included a radio sounding station, 4 Doppler lidars, 4 Raman lidars (3 of them provide temperature, 3 of them water vapour, and all of them particle backscatter data), 1 water vapour differential absorption lidar, 3 cloud radars, 5 microwave radiometers, 3 rain radars, 6 sky imagers, 99 pyranometers, and 5 sun photometers operated at different sites, some of them in synergy. The HOPE-Melpitz campaign combined ground-based remote sensing of aerosols and clouds with helicopter- and balloon-based in situ observations in the atmospheric column and at the surface. HOPE provided an unprecedented collection of atmospheric dynamical, thermodynamical, and micro- and macrophysical properties of aerosols, clouds, and precipitation with high spatial and temporal resolution within a cube of approximately 10 × 10 × 10 km3. HOPE data will significantly contribute to our understanding of boundary layer dynamics and the formation of clouds and precipitation. The datasets have been made available through a dedicated data portal. First applications of HOPE data for model evaluation have shown a general agreement between observed and modelled boundary layer height, turbulence characteristics, and cloud coverage, but they also point to significant differences that deserve further investigations from both the observational and the modelling perspective.
We present a practical method to continuously calibrate Raman lidar
observations of water vapor mixing ratio profiles. The water vapor profile
measured with the multiwavelength polarization Raman ...lidar
PollyXT is calibrated by means of co-located AErosol
RObotic NETwork (AERONET) sun photometer observations and Global Data
Assimilation System (GDAS) temperature and pressure profiles. This method is
applied to lidar observations conducted during the Cyprus Cloud Aerosol and
Rain Experiment (CyCARE) in Limassol, Cyprus. We use the GDAS temperature and
pressure profiles to retrieve the water vapor density. In the next step, the
precipitable water vapor from the lidar observations is used for the
calibration of the lidar measurements with the sun photometer measurements.
The retrieved calibrated water vapor mixing ratio from the lidar measurements
has a relative uncertainty of 11 % in which the error is mainly caused by
the error of the sun photometer measurements. During CyCARE, nine measurement
cases with cloud-free and stable meteorological conditions are selected to
calculate the precipitable water vapor from the lidar and the sun photometer
observations. The ratio of these two precipitable water vapor values yields
the water vapor calibration constant. The calibration constant for the
PollyXT Raman lidar is
6.56 g kg−1 ± 0.72 g kg−1 (with a statistical uncertainty
of 0.08 g kg−1 and an instrumental uncertainty of 0.72 g kg−1).
To check the quality of the water vapor calibration, the water vapor mixing
ratio profiles from the simultaneous nighttime observations with Raman lidar
and Vaisala radiosonde sounding are compared. The correlation of the water
vapor mixing ratios from these two instruments is determined by using all of
the 19 simultaneous nighttime measurements during CyCARE. Excellent agreement
with the slope of 1.01 and the R2 of 0.99 is found. One example is
presented to demonstrate the full potential of a well-calibrated Raman lidar.
The relative humidity profiles from lidar, GDAS (simulation) and radiosonde
are compared, too. It is found that the combination of water vapor mixing
ratio and GDAS temperature profiles allow us to derive relative humidity
profiles with the relative uncertainty of 10–20 %.
Abstract
The relationship between vertical air velocity at cloud base and primary ice formation has been measured for shallow mixed-phase cloud layers (thickness <380 m) by means of ground-based ...cloud radar and Doppler lidar. For layers with a cloud-top temperature below −12 °C, an increase of vertical-velocity standard deviation from 0.1 to 1.0 m s
−1
leads to an increase in the mass flux of ice water by two orders of magnitude. The cloud layers under study were selected in such a way that secondary ice-formation processes played a minor role, and primary ice formation was the dominant source of ice formation. Phenomenological parameterizations of the ice mass and the ice mass flux as functions of standard deviation of vertical air velocity are given.
On 22nd August 2018, the European Space Agency (ESA) launched the first direct detection Doppler wind lidar into space. Operating at 355 nm and acquiring signals with a dual channel receiver, it ...allows wind observations in clear air and particle-laden regions of the atmosphere. Furthermore, particle optical properties can be obtained using the High Spectral Resolution Technique Lidar (HSRL) technique. Measuring with 87 km horizontal and 0.25-2 km vertical resolution between ground and up to 30 km in the stratosphere, the global coverage of Aeolus observations shall fill gaps in the global observing system and thus help improving numerical weather prediction. Within this contribution, first results from the German initiative for experimental Aeolus validation are presented and discussed. Ground-based wind and aerosol measurements from tropospheric radar wind profilers, Doppler wind lidars, radiosondes, aerosol lidars and cloud radars are utilized for that purpose.
Canadian wildfire smoke was detected in the troposphere and lower stratosphere over Europe in August and September 2017. Lidar measurements from various stations of the European Aerosol Research ...Lidar Network (EARLINET) observed the stratospheric smoke layer. Triple-wavelength (355, 532, and 1064 nm) lidar measurements of the depolarization and the lidar ratio are reported from Leipzig, Germany. The particle linear depolarization ratio of the wildfire smoke in the stratosphere had an exceptional strong wavelength dependence reaching from 0.22 at 355 nm, to 0.18 at 532 nm, and 0.04 at 1064 nm. The lidar ratio increased with wavelength from 40±16 sr at 355 nm, to 66±12 sr at 532 nm, and 92±27 sr at 1064 nm. The development of the stratospheric smoke plume over several months was studied by long-term lidar measurements in Cyprus. The stratospheric smoke layers increased in altitude up to 24 km height.
The development of fast and reliable finite element (FE) simulation codes has increased the relevance of FE simulations in predicting the outcomes of additive manufacturing (AM) processes and in the ...post-processing of additively manufactured components. The accuracy of FE simulations relies heavily on the quality of inputs such as material data, physical properties, numerical settings, and simulation methods. We review models used for simulating AM processes and the post-processing of AM components based on macro-scale continuum FE simulations. Particular attention is given to phase transformation and microstructure-based models because they determine the properties of AM components along manufacturing process chains and their subsequent performance. However, it's noted that FE simulations of AM components usually only consider the post-processing of AM components rather than complete process chains that include both AM and post-processing. A process chain simulation framework is proposed to model the entire manufacturing chain of AM parts.