Abstract
Understanding the evolution of the nuclear charge radius is one of the long-standing challenges for nuclear theory. Recently, density functional theory calculations utilizing Fayans ...functionals have successfully reproduced the charge radii of a variety of exotic isotopes. However, difficulties in the isotope production have hindered testing these models in the immediate region of the nuclear chart below the heaviest self-conjugate doubly-magic nucleus
100
Sn, where the near-equal number of protons (
Z
) and neutrons (
N
) lead to enhanced neutron-proton pairing. Here, we present an optical excursion into this region by crossing the
N
= 50 magic neutron number in the silver isotopic chain with the measurement of the charge radius of
96
Ag (
N
= 49). The results provide a challenge for nuclear theory: calculations are unable to reproduce the pronounced discontinuity in the charge radii as one moves below
N
= 50. The technical advancements in this work open the
N
=
Z
region below
100
Sn for further optical studies, which will lead to more comprehensive input for nuclear theory development.
We report on a set of high-precision measurements of nuclear binding and excitation energies, as well as nuclear spins, magnetic dipole and electric quadrupole moments of neutron-rich silver ...isotopes, 113−123Ag. The measurements were performed using the JYFLTRAP mass spectrometer and the collinear laser spectroscopy beamline at the Ion Guide Isotope Separator On-Line (IGISOL) facility. For the first time, we can firmly establish the ordering of the long-lived Iπ=1/2−,7/2+ states in these isotopes, and pin down the inversion of these two levels at either A=121(N=74) or A=123(N=76). We compare these findings to calculations performed with density functional theory (DFT), from which we establish the crucial role that the spin-orbit strength and time-odd mean fields play in the simultaneous description of electromagnetic moments and nuclear binding.
In deep inelastic multinucleon transfer reactions of 48Ca + 248Cm we observed about 100 residual nuclei with proton numbers between Z=82 and Z=100. Among them, there are five new neutron-deficient ...isotopes: 216U, 219Np, 223Am, 229Am and 233Bk. As separator for the transfer products we used the velocity filter SHIP of GSI while the isotope identification was performed via the α decay chains of the nuclei. These first results reveal that multinucleon transfer reactions together with here applied fast and sensitive separation and detection techniques are promising for the synthesis of new isotopes in the region of heaviest nuclei.
Precision mass measurements of 104Y, 106Zr, 104,104m,109Nb, and 111,112Mo have been performed with the JYFLTRAP double Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line ...facility. The order of the long-lived states in 104Nb was unambiguously established. The trend in two-neutron separation energies around the N=66 neutron midshell appeared to be steeper with respect to the Atomic Mass Evaluation 2020 extrapolations for the 39Y and 40Zr isotopic chains and less steep for the 41Nb chain, indicating a possible gap opening around Z=40. The experimental results were compared to the BSkG2 model calculations performed with and without vibrational and rotational corrections. All of them predict two low-lying minima for 106Zr. While the unaltered BSkG2 model fails to predict the trend in two-neutron separation energies, selecting the more deformed minima in calculations and removing the vibrational correction, the calculations are more in line with experimental data. The same is also true for the 21+ excitation energies and differences in charge radii in the Zr isotopes. The results stress the importance of improved treatment of collective corrections in large-scale models and further development of beyond-mean-field techniques.
The impact of nuclear deformation can been seen in the systematics of nuclear charge radii, with radii generally expanding with increasing deformation. In this Letter, we present a detailed analysis ...of the precise relationship between nuclear quadrupole deformation and the nuclear size. Our approach combines the first measurements of the changes in the mean-square charge radii of well-deformed palladium isotopes between A=98 and A=118 with nuclear density functional calculations using Fayans functionals, specifically Fy(std) and Fy(Δr,HFB), and the UNEDF2 functional. The changes in mean-square charge radii are extracted from collinear laser spectroscopy measurements on the 4d^{9}5s ^{3}D_{3}→4d^{9}5p ^{3}P_{2} atomic transition. The analysis of the Fayans functional calculations reveals a clear link between a good reproduction of the charge radii for the neutron-rich Pd isotopes and the overestimated odd-even staggering: Both aspects can be attributed to the strength of the pairing correlations in the particular functional which we employ.
This letter reports on the first observation of an octupole band in the neutron-deficient (N=Z+2) nucleus 110Xe. The 110Xe nuclei were produced via the 54Fe(58Ni,2n) fusion-evaporation reaction. The ...emitted γ rays were detected using the jurogam 3γ-ray spectrometer, while the fusion-evaporation residues were separated with the MARA separator at the Accelerator Laboratory of the University of Jyväskylä, Finland. The experimental observation of the low-lying 3− and 5− states and inter-band E1 transitions between the ground-state band and the octupole band proves the importance of octupole correlations in this region. These new experimental data combined with theoretical calculations using the symmetry-conserving configuration-mixing method, based on a Gogny energy density functional, have been interpreted as an evidence of enhanced octupole correlations in neutron-deficient xenon isotopes.
The cosmological lithium problem (CLP) stems from the outstanding discrepancy between theoretical predictions and astronomical observations of primordial lithium abundances. For the radiogenic ...production of 7Li, 7Be plays a pivotal role in the Big Bang nucleosynthesis (BBN). Nevertheless, the data for neutron-induced 7Be destruction processes were still sparse, and especially lacked information on the contributions of transitions to the 7Li excited states. In this work, we have determined the 7Be\({(n,{p}_{0})}^{7}\)Li, 7Be\({(n,{p}_{1})}^{7}\)Li*, and 7Be\({(n,\alpha )}^{4}\)He reaction cross sections by means of the Trojan Horse method. The present and the previous data were analyzed together by a multichannel R-matrix fit, providing an improved uncertainty evaluation of the \((n,{p}_{0})\) channel and the first-ever quantification of the \((n,{p}_{1})\) contribution in the BBN-relevant energy range. We implemented the revised total reaction rate summing both the \((n,{p}_{0})\) and \((n,{p}_{1})\) contributions in a state-of-the-art BBN code PRIMAT. As a consequence, the present nuclear-physics data offers a reduction of the predicted 7Li abundance by about one-tenth, which would impose a stricter constraint on BBN and head us in the correct direction to the CLP solution.
γ emission probabilities from unbound states in 78,80Se, populated by a neutron-transfer reaction (d,p) on 77,79Se nuclei in inverse kinematics, were measured by directly detecting reaction residues. ...Assuming the spin distribution at the respective excitation energy of the unbound state, the cross-sections of the 79Se(n,γ)80Se reaction were evaluated using the γ emission probabilities. The surrogate-ratio method with the experimental γ emission probabilities of 78,80Se was also employed to deduce the cross-sections of 79Se(n,γ) reaction by incorporating the theoretical evaluations of the neutron-capture reaction on the isomeric state in 77Se. Our two cross-sections are in good agreement with existing nuclear data compilations for the neutron-capture reaction on 79Se. The presented method contributes to the body of existing knowledge by providing approaches for determining the neutron capture cross-sections of radioactive nuclei at various neutron energies.
The HPHT diamond Schottky diode was assembled as a Metal/Intrinsic/p-doped structure betavoltaic cell (BC) with a very thin (1 μm) drift layer and tested under 5–30 keV electron beam irradiation ...using a scanning electron microscope (SEM). The effect of the β-radiation energy and the backscattering of electrons on the energy conversion was studied. From the results obtained, it is shown that, the efficiency of the investigated BC increases from 1.01 to 3.75% with the decrease of β-particle energy from 30 to 5 keV due to an increase of the electron beam absorption in a thin drift layer. Maximum efficiency is achieved when the electron beam energy is close to the average β-decay energy of 3H. The BC maximum output power of the 1.6 μW was obtained at an electron beam energy of 15 keV, that matches the β-decay energy of 63Ni. The total BC conversion efficiency at 15 keV electron-beam energy is about 3%. The calculations indicated that a preferable β-source for the diamond based BCs with a thin (1 μm) drift layer is 63Ni.
•The total conversion efficiency (TCE) of the diamond cell with a thin drift layer increases while the beam energy decrease.•The most preferred beta source for the diamond Schottky diode with a thin drift layer is 63Ni.•The β-backscattered coefficient and the energy loss in the electrode significantly affects the TCE at low beam energies.•The lateral electron spread can lead to a significant loss of the output power and TCE at the edges of the drift layer.
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