Ionic transport in metal/oxide heterostructures offers a highly effective means to tailor material properties via modification of the interfacial characteristics. However, direct observation of ionic ...motion under buried interfaces and demonstration of its correlation with physical properties has been challenging. Using the strong oxygen affinity of gadolinium, we design a model system of GdxFe1-x/NiCoO bilayer films, where the oxygen migration is observed and manifested in a controlled positive exchange bias over a relatively small cooling field range. The exchange bias characteristics are shown to be the result of an interfacial layer of elemental nickel and cobalt, a few nanometres in thickness, whose moments are larger than expected from uncompensated NiCoO moments. This interface layer is attributed to a redox-driven oxygen migration from NiCoO to the gadolinium, during growth or soon after. These results demonstrate an effective path to tailoring the interfacial characteristics and interlayer exchange coupling in metal/oxide heterostructures.
Static and dynamic magnetic solitons play a critical role in applied nanomagnetism. Magnetic droplets, a type of non-topological dissipative soliton, can be nucleated and sustained in nanocontact ...spin-torque oscillators with perpendicular magnetic anisotropy free layers. Here, we perform a detailed experimental determination of the full droplet nucleation boundary in the current-field plane for a wide range of nanocontact sizes and demonstrate its excellent agreement with an analytical expression originating from a stability analysis. Our results reconcile recent contradicting reports of the field dependence of the droplet nucleation. Furthermore, our analytical model both highlights the relation between the fixed layer material and the droplet nucleation current magnitude, and provides an accurate method to experimentally determine the spin transfer torque asymmetry of each device.
To develop a full understanding of interactions in nanomagnet arrays is a persistent challenge, critically impacting their technological acceptance. This paper reports the experimental, numerical and ...analytical investigation of interactions in arrays of Co nanoellipses using the first-order reversal curve (FORC) technique. A mean-field analysis has revealed the physical mechanisms giving rise to all of the observed features: a shift of the non-interacting FORC-ridge at the low-HC end off the local coercivity HC axis; a stretch of the FORC-ridge at the high-HC end without shifting it off the HC axis; and a formation of a tilted edge connected to the ridge at the low-HC end. Changing from flat to Gaussian coercivity distribution produces a negative feature, bends the ridge, and broadens the edge. Finally, nearest neighbor interactions segment the FORC-ridge. These results demonstrate that the FORC approach provides a comprehensive framework to qualitatively and quantitatively decode interactions in nanomagnet arrays.
The first order reversal curve (FORC) method is a magnetometry based technique used to capture nanoscale magnetic phase separation and interactions with macroscopic measurements using minor ...hysteresis loop analysis. This makes the FORC technique a powerful tool in the analysis of complex systems which cannot be effectively probed using localized techniques. However, recovering quantitative details about the identified phases which can be compared to traditionally measured metrics remains an enigmatic challenge. We demonstrate a technique to reconstruct phase-resolved magnetic hysteresis loops by selectively integrating the measured FORC distribution. From these minor loops, the traditional metrics-including the coercivity and saturation field, and the remanent and saturation magnetization-can be determined. In order to perform this analysis, special consideration must be paid to the accurate quantitative management of the so-called reversible features. This technique is demonstrated on three representative materials systems, high anisotropy FeCuPt thin-films, Fe nanodots, and SmCo/Fe exchange spring magnet films, and shows excellent agreement with the direct measured major loop, as well as the phase separated loops.
It has been argued that if multiple spin wave modes are competing for the same centrally located energy source, as in a nanocontact spin torque oscillator, that only one mode should survive in the ...steady state. Here, the experimental conditions necessary for mode coexistence are explored. Mode coexistence is facilitated by the local field asymmetries induced by the spatially inhomogeneous Oersted field, which leads to a physical separation of the modes, and is further promoted by spin wave localization at reduced applied field angles. Finally, both simulation and experiment reveal a low frequency signal consistent with the intermodulation of two coexistent modes.
Light polarization rotators and nonreciprocal optical isolators are essential building blocks in photonics technology. These macroscopic passive devices are commonly based on magneto-optical Faraday ...and Kerr polarization rotation. Magnetoplasmonics, the combination of magnetism and plasmonics, is a promising route to bring these devices to the nanoscale. We introduce design rules for highly tunable active magnetoplasmonic elements in which we can tailor the amplitude and sign of the Kerr response over a broad spectral range.
Memory Effect in Magnetic Nanowire Arrays Kou, Xiaoming; Fan, Xin; Dumas, Randy K. ...
Advanced materials (Weinheim),
03/2011, Letnik:
23, Številka:
11
Journal Article
Recenzirano
Odprti dostop
A memory effect has been demonstrated in magnetic nanowire arrays. The magnetic nanowire array has the ability to record the maximum magnetic field that the array has been exposed to after the field ...has been turned off. The origin of the memory effect is the strong magnetic dipole interaction among the nanowires. Switching field distributions among nanowires has been studied with a first‐order reversal curve technique to elucidate the discrepancy between the experimental result and the theoretical explanation. Based on the memory effect, a novel and extremely low cost EMP detection scheme is proposed.
Spin-torque oscillators (STOs) are devices that allow for the excitation of a variety of magnetodynamical modes at the nanoscale. Depending on both external conditions and intrinsic magnetic ...properties, STOs can exhibit regimes of mode hopping and even mode coexistence. Whereas mode hopping has been extensively studied in STOs patterned as nanopillars, coexistence has been only recently observed for localized modes in nanocontact STOs (NC-STOs), where the current is confined to flow through a NC fabricated on an extended pseudo spin valve. By means of electrical characterization and a multimode STO theory, we investigate the physical origin of the mode-coupling mechanisms favoring coexistence. Two coupling mechanisms are identified: (i) magnon-mediated scattering and (ii) intermode interactions. These mechanisms can be physically disentangled by fabricating devices where the NCs have an elliptical cross section. The generation power and linewidth from such devices are found to be in good qualitative agreement with the theoretical predictions, as well as provide evidence of the dominant mode-coupling mechanisms.
Magnetic dissipative droplets are localized, strongly nonlinear dynamical modes excited in nanocontact spin valves with perpendicular magnetic anisotropy. These modes find potential application in ...nanoscale structures for magnetic storage and computation, but dissipative droplet studies have so far been limited to extended thin films. Here, numerical and asymptotic analyses are used to demonstrate the existence and properties of novel solitons in confined structures. As a nanowire's width is decreased with a nanocontact of fixed size at its center, the observed modes undergo transitions from a fully localized two-dimensional droplet into a two-dimensional droplet edge mode and then a pulsating one-dimensional droplet. These solitons are interpreted as dissipative versions of classical, conservative solitons, allowing for an analytical description of the modes and the mechanisms of bifurcation. The presented results open up new possibilities for the study of low-dimensional solitons and droplet applications in nanostructures.
Plasmon rulers are an emerging concept in which the strong near-field coupling of plasmon nanoantenna elements is employed to obtain structural information at the nanoscale. Here, we combine ...nanoplasmonics and nanomagnetism to conceptualize a magnetoplasmonic dimer nanoantenna that would be able to report nanoscale distances while optimizing its own spatial orientation. The latter constitutes an active operation in which a dynamically optimized optical response per measured unit length allows for the measurement of small and large nanoscale distances with about 2 orders of magnitude higher precision than current state-of-the-art plasmon rulers. We further propose a concept to optically measure the nanoscale response to the controlled application of force with a magnetic field.
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