Studying the evaporation process and its link to the atmospheric circulation is central for a better understanding of the feedbacks between the surface water components and the atmosphere. In this ...study, we use 5 months of deuterium excess (d) measurements at the hourly to daily timescale from a cavity ring-down laser spectrometer to characterise the evaporation source of low-level continental water vapour at the long-term hydrometeorological monitoring site Rietholzbach in northeastern Switzerland. To reconstruct the phase change history of the air masses in which we measure the d signature and to diagnose its area of surface evaporation we apply a Lagrangian moisture source diagnostic. With the help of a correlation analysis we investigate the strength of the relation between d measurements and the moisture source conditions. Temporal episodes with a duration of a few days of strong anticorrelation between d and relative humidity as well as temperature are identified. The role of plant transpiration, the large-scale advection of remotely evaporated moisture, the local boundary layer dynamics at the measurement site and recent precipitation at the site of evaporation are discussed as reasons for the existence of these modes of strong anticorrelation between d and moisture source conditions. We show that the importance of continental moisture recycling and the contribution of plant transpiration to the continental evaporation flux may be deduced from the d–relative humidity relation at the seasonal timescale as well as for individual events. The methodology and uncertainties associated with these estimates of the transpiration fraction of evapotranspiration are presented and the proposed novel framework is applied to individual events from our data set. Over the whole analysis period (August to December 2011) a transpiration fraction of the evapotranspiration flux over the continental part of the moisture source region of 62% is found albeit with a large event-to-event variability (0% to 89%) for continental Europe. During days of strong local moisture recycling a higher overall transpiration fraction of 76% (varying between 65% and 86%) is found. These estimates are affected by uncertainties in the assumptions involved in our method as well as by parameter uncertainties. An average uncertainty of 11% results from the strong dependency of the transpiration estimates on the choice of the non-equilibrium fractionation factor. Other uncertainty sources like the influence of boundary layer dynamics are probably large but more difficult to quantify. Nevertheless, such Lagrangian estimates of the transpiration part of continental evaporation could potentially be useful for the verification of model estimates of this important land–atmosphere coupling parameter.
▶ Analysis of EB deficit in multi-site analysis with up to 26 sites. ▶ Relative EB deficit is larger for very unstable conditions than for less unstable conditions, because of reduced ...mechanically-induced turbulence for very unstable conditions, and not related with increased thermally-induced turbulence. ▶ Average absolute EB deficits are largest when relative EB deficits are smallest. ▶ Relative EB deficits are smallest for strong thermally-induced turbulence (TT) or strongly suppressed TT, but largest for intermediate conditions. ▶ For non-neutral atmospheric conditions the relative EB deficit is not given by the slope of the regression line of the absolute EB deficit as a function of net radiation. ▶ Storage terms are important for reducing relative EB deficit during nighttime and stable conditions, but otherwise not so important.
This paper presents a multi-site (>20) analysis of the relative and absolute energy balance (EB) closure at European FLUXNET sites, as a function of the stability parameter
ξ, the friction velocity
u
*, thermally-induced turbulence, and the time of the day. A focus of the analysis is the magnitude of EB deficits for very unstable conditions. A univariate analysis of the relative EB deficit as function of
ξ alone (both for individual sites and a synthesis for all sites), reveals that the relative EB deficit is larger for very unstable conditions (
ξ
<
−1.0) than for less unstable conditions (−0.02
>
ξ
≥
−1.0). A bivariate analysis of the relative EB deficit as function of both
ξ and
u
*, however, indicates that for situations with comparable
u
* the closure is better for very unstable conditions than for less unstable conditions. Our results suggest that the poorer closure for very unstable conditions identified from the univariate analysis is due to reduced
u
* under these conditions. In addition, we identify that the conditions characterized by smallest relative EB deficits (elevated overall turbulence, mostly during day time) correspond to cases with the largest absolute EB deficits. Thus, the total EB deficit at the sites is induced mostly under these conditions, which is particularly relevant for evapotranspiration estimates. Further, situations with the largest relative EB deficits are generally characterized by small absolute EB deficits. We also find that the relative EB deficit does generally not correspond to the regression line of absolute EB deficit with the net radiation because there is a (positive or negative) offset. This can be understood from theoretical considerations. Finally, we find that storage effects explain a considerable fraction of the large
relative (but small absolute) nocturnal EB deficits, and only a limited fraction of the overall relative and absolute EB deficits.
Heterogeneity in small‐scale subsurface flow processes does not necessarily lead to complex system behavior at larger scales. Here we use the simple dynamical systems approach recently proposed by ...Kirchner (WRR, 2009) to analyze, characterize, and simulate streamflow dynamics in the Swiss Rietholzbach catchment. The Rietholzbach data set used here provides 32 years of continuous and high‐quality observations, which include a soil moisture profile and unique observations of storage changes and evapotranspiration measured by a weighing lysimeter. Streamflow recession at the daily time scale shows a marked seasonal cycle and is fastest in summer due to the higher evapotranspiration losses. The discharge sensitivity function linking storage and discharge is nonlinear and slightly downward‐curving in double‐logarithmic space. Small diurnal discharge fluctuations prevent application of the approach at the hourly resolution for low‐discharge conditions. The vast majority of runoff peaks can be explained by storage variations, except peaks that follow events with extreme precipitation intensity (30–40 mm h−1). Storage change dynamics inferred from streamflow variations compare well to observations from the lysimeter and simulations with a land surface model but become very uncertain under dry conditions. Good results can be obtained when the discharge sensitivity function is calibrated on a monthly time scale to avoid the effect of the diurnal discharge fluctuations. Our analysis highlights the importance of evapotranspiration for catchment hydrology, as it is the main driver of changes in streamflow at Rietholzbach for 21% of the time.
Biogeochemical cycling of elements largely occurs in dissolved state, but many elements may also be bound to natural nanoparticles (NNP, 1–100 nm) and fine colloids (100–450 nm). We examined the ...hypothesis that the size and composition of stream water NNP and colloids vary systematically across Europe. To test this hypothesis, 96 stream water samples were simultaneously collected in 26 forested headwater catchments along two transects across Europe. Three size fractions (~1–20 nm, >20–60 nm, and >60 nm) of NNP and fine colloids were identified with Field Flow Fractionation coupled to inductively coupled plasma mass spectrometry and an organic carbon detector. The results showed that NNP and fine colloids constituted between 2 ± 5% (Si) and 53 ± 21% (Fe; mean ± SD) of total element concentrations, indicating a substantial contribution of particles to element transport in these European streams, especially for P and Fe. The particulate contents of Fe, Al, and organic C were correlated to their total element concentrations, but those of particulate Si, Mn, P, and Ca were not. The fine colloidal fractions >60 nm were dominated by clay minerals across all sites. The resulting element patterns of NNP <60 nm changed from North to South Europe from Fe‐ to Ca‐dominated particles, along with associated changes in acidity, forest type, and dominant lithology.
Key Points
Stream phosphorus is largely bound to natural nanoparticles and colloids
The chemical composition of colloids varies systematically from Northern to Southern European streams
Evapotranspiration amplifies European summer drought Teuling, Adriaan J; Van Loon, Anne F; Seneviratne, Sonia Isabelle ...
Geophysical research letters,
28 May 2013, Letnik:
40, Številka:
10
Journal Article, Web Resource
Recenzirano
Odprti dostop
Drought is typically associated with a lack of precipitation, whereas the contribution of evapotranspiration and runoff to drought evolution is not well understood. Here we use unique long‐term ...observations made in four headwater catchments in central and western Europe to reconstruct storage anomalies and study the drivers of storage anomaly evolution during drought. We provide observational evidence for the “drought‐paradox” in that region: a consistent and significant increase in evapotranspiration during drought episodes, which acts to amplify the storage anomalies. In contrast, decreases in runoff act to limit storage anomalies. Our findings stress the need for the correct representation of evapotranspiration and runoff processes in drought indices.
Key Points
Storage anomaly change drivers attributed to observed fluxesEvapotranspiration amplifies effect of negative precipitation anomaliesNegative runoff anomalies reduce storage anomalies
Accurate measurements of evapotranspiration are required for many meteorological, climatological, ecological, and hydrological research applications and developments. Here we examine and compare two ...well-established methods to determine evapotranspiration at the site level: lysimeter-based measurements (EL) and eddy covariance (EC) flux measurements (EEC). The analyses are based on parallel measurements carried out with these two methods at the research catchment Rietholzbach in northeastern Switzerland, and cover the time period of June 2009 to December 2015. The measurements are compared on various timescales, and with respect to a 40-year lysimeter-based evapotranspiration time series. Overall, the lysimeter and EC measurements agree well, especially on the annual timescale. On that timescale, the long-term lysimeter measurements also correspond well with catchment water-balance estimates of evapotranspiration. This highlights the representativeness of the site-level lysimeter and EC measurements for the entire catchment despite their comparatively small source areas and the heterogeneous land use and topography within the catchment. Furthermore, we identify that lack of reliable EC measurements using open-path gas analyzers during and following precipitation events (due to limitations of the measurement technique under these conditions) significantly contributes to an underestimation of EEC and to the overall energy balance gap at the site.
The Nordic region was subjected to severe drought in 2018 with a particularly long-lasting and large soil water deficit in Denmark, Southern Sweden and Estonia. Here, we analyse the impact of the ...drought on carbon and water fluxes in 11 forest ecosystems of different composition: spruce, pine, mixed and deciduous. We assess the impact of drought on fluxes by estimating the difference (anomaly) between year 2018 and a reference year without drought. Unexpectedly, the evaporation was only slightly reduced during 2018 compared to the reference year at two sites while it increased or was nearly unchanged at all other sites. This occurred under a 40 to 60% reduction in mean surface conductance and the concurrent increase in evaporative demand due to the warm and dry weather. The anomaly in the net ecosystem productivity (NEP) was 93% explained by a multilinear regression with the anomaly in heterotrophic respiration and the relative precipitation deficit as independent variables. Most of the variation (77%) was explained by the heterotrophic component. Six out of 11 forests reduced their annual NEP with more than 50 g C m
yr
during 2018 as compared to the reference year. The NEP anomaly ranged between -389 and +74 g C m
yr
with a median value of -59 g C m
yr
. This article is part of the theme issue 'Impacts of the 2018 severe drought and heatwave in Europe: from site to continental scale'.
The prealpine Rietholzbach research catchment provides long‐term continuous hydroclimatological measurements in northeastern Switzerland, including lysimeter evapotranspiration measurements since ...1976, and soil moisture measurements since 1994. We analyze here the monthly data record over 32 years (1976–2007), with a focus on the extreme 2003 European drought. In particular, we assess whether the well‐established hypothesis that the 2003 event was due to spring precipitation deficits is valid at the site. The Rietholzbach measurements are found to be internally consistent and representative for a larger region in Switzerland. Despite the scale discrepancy (3.14 m2 versus 3.31 km2), the lysimeter seepage and catchment‐wide streamflow show similar monthly dynamics. High correlations are further found with other streamflow measurements within the Thur river basin (1750 km2) and—for interannual anomalies—also in most of northern Switzerland. Analyses for 2003 confirm the occurrence of extreme heat and drought conditions at Rietholzbach. However, unlike findings from regional‐scale modeling studies, they reveal a late onset of the soil moisture deficit (from June onward), despite large precipitation deficits from mid‐February to mid‐April. These early spring deficits were mostly compensated for by decreased runoff during this period and excess precipitation in the preceding weeks to months (including in the 2002 fall). Our results show that evapotranspiration excess in June 2003 was the main driver initiating the 2003 summer drought conditions in Rietholzbach, contributing 60% of the June 2003 water storage deficit. Finally, long‐lasting drought effects on the lysimeter water storage due to rewetting inhibition were recorded until spring 2004.
Key Points
Unique hydroclimatological data set including multidecadal lysimeter record
Evapotranspiration as major and underestimated driver of 2003 European drought
Precipitation deficits in spring 2003 play a minor role for drought development
Multidrug efflux pumps are found in all major transporter families. Along with a lack of three-dimensional structure information, the mechanism of drug recognition, energy coupling with drug ...translocation and the catalytic cycle are so far not understood. In the present study, we present first data of a fluorescence-based assay to study the pH-gradient-mediated activity of the multidrug antiporter EmrE, by co-reconstitution with the light-driven proton pump bacteriorhodopsin. In addition to biochemical approaches, the emerging technique, solid-state NMR, can be used for the investigation of these transporters. A number of experiments based on MAS (magic angle sample spinning) NMR are available to provide data on protein structure and dynamics, drug binding and protein-lipid interactions. However, these experiments dictate a number of constraints with respect to sample preparation that will be discussed for proteins from the SMR (small multidrug resistance transporter) family. In addition, 2H-NMR is used to probe protein mobility of Lactococcus lactis ABC transporter, LmrA.
During the summer of 2018, a widespread drought developed over Northern and Central Europe. The increase in temperature and the reduction of soil moisture have influenced carbon dioxide (CO
2
) ...exchange between the atmosphere and terrestrial ecosystems in various ways, such as a reduction of photosynthesis, changes in ecosystem respiration, or allowing more frequent fires. In this study, we characterize the resulting perturbation of the atmospheric CO
2
seasonal cycles. 2018 has a good coverage of European regions affected by drought, allowing the investigation of how ecosystem flux anomalies impacted spatial CO
2
gradients between stations. This density of stations is unprecedented compared to previous drought events in 2003 and 2015, particularly thanks to the deployment of the Integrated Carbon Observation System (ICOS) network of atmospheric greenhouse gas monitoring stations in recent years. Seasonal CO
2
cycles from 48 European stations were available for 2017 and 2018. Earlier data were retrieved for comparison from international databases or national networks. Here, we show that the usual summer minimum in CO
2
due to the surface carbon uptake was reduced by 1.4 ppm in 2018 for the 10 stations located in the area most affected by the temperature anomaly, mostly in Northern Europe. Notwithstanding, the CO
2
transition phases before and after July were slower in 2018 compared to 2017, suggesting an extension of the growing season, with either continued CO
2
uptake by photosynthesis and/or a reduction in respiration driven by the depletion of substrate for respiration inherited from the previous months due to the drought. For stations with sufficiently long time series, the CO
2
anomaly observed in 2018 was compared to previous European droughts in 2003 and 2015. Considering the areas most affected by the temperature anomalies, we found a higher CO
2
anomaly in 2003 (+3 ppm averaged over 4 sites), and a smaller anomaly in 2015 (+1 ppm averaged over 11 sites) compared to 2018.
This article is part of the theme issue ‘Impacts of the 2018 severe drought and heatwave in Europe: from site to continental scale'.
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