The Arctic region is known to be very sensitive to climate change. Clouds and in particular mixed-phase clouds (MPCs) remain one of the greatest sources of uncertainties in the modelling of the ...Arctic response to climate change due to an inaccurate representation of their variability and their quantification. In this study, we present a characterisation of the vertical, spatial and seasonal variability of Arctic clouds and MPCs over the entire Arctic region based on satellite active remote sensing observations. MPC properties in the region of the Svalbard archipelago (78° N, 15° E) are also investigated. The occurrence frequency of clouds and MPCs are determined from CALIPSO/CLOUDSAT measurements processed with the DARDAR retrieval algorithm, which allow for a reliable cloud thermodynamic phase classification (warm liquid, supercooled liquid, ice, mixing of ice and supercooled liquid). Significant differences are observed between MPC properties over the entire Arctic region and over the Svalbard region. Results show that MPCs are encountered all year long, with a minimum occurrence of 30% in winter and 50% during the rest of the year on average over the entire Arctic. Over the Svalbard region, MPC occurrence is more constant with time with larger values (55%) compared to the average observed in the Arctic. MPCs are especially located at low altitudes, below 3000 m, where their frequency of occurrence reaches 90%, particularly during winter, spring and autumn. Moreover, results highlight that MPCs are statistically more frequent above open sea than land or sea ice. The temporal and spatial distribution of MPCs over the Svalbard region seems to be linked to the supply of moister air and warmer water from the North Atlantic Ocean, which contribute to the initiation of the liquid water phase. Over the whole Arctic, and particularly in western regions, the increase of MPC occurrence from spring to autumn could be connected to the sea ice melting. During this period, the open water transports some of the warm water from the North Atlantic Ocean to the rest of the Arctic region. This facilitates the vertical transfer of moisture and thus the persistence of the liquid phase. Particular attention is also paid to the measurement uncertainties and how they could affect our conclusions.
We compare the cloud detection and cloud phase determination of three independent climatologies based on Cloud‐Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) to airborne in ...situ measurements. Our analysis of the cloud detection shows that the differences between the satellite and in situ measurements mainly arise from three factors. First, averaging CALIPSO Level l data along track before cloud detection increases the estimate of high‐ and low‐level cloud fractions. Second, the vertical averaging of Level 1 data before cloud detection tends to artificially increase the cloud vertical extent. Third, the differences in classification of fully attenuated pixels among the CALIPSO climatologies lead to differences in the low‐level Arctic cloud fractions. In another section, we compare the cloudy pixels detected by colocated in situ and satellite observations to study the cloud phase determination. At midlatitudes, retrievals of homogeneous high ice clouds by CALIPSO data sets are very robust (more than 94.6% of agreement with in situ). In the Arctic, where the cloud phase vertical variability is larger within a 480 m pixel, all climatologies show disagreements with the in situ measurements and CALIPSO‐General Circulation Models‐Oriented Cloud Product (GOCCP) report significant undefined‐phase clouds, which likely correspond to mixed‐phase clouds. In all CALIPSO products, the phase determination is dominated by the cloud top phase. Finally, we use global statistics to demonstrate that main differences between the CALIPSO cloud phase products stem from the cloud detection (horizontal averaging, fully attenuated pixels) rather than the cloud phase determination procedures.
Key Points
Comparison of the cloud and cloud phase of three CALIPSO climatologies with in situ measurements
Cloud detection differences due to vertical/horizontal averaging and fully attenuated pixels
Very high agreement for midlatitude ice clouds, more disagreement with the mixed‐phase clouds
There is growing evidence that marine microorganisms may influence cloud cover over the ocean through their impact on sea spray and trace gas emissions, further forming cloud droplets or ice ...crystals. However, evidence of a robust causal relationship based on observations is still pending. In this study, we use 4 years of multi‐instrument satellite data to segregate low‐level clouds into ice‐containing and liquid‐water clouds to obtain clear relationships between cloud types and ocean biological tracers, especially with nanophytoplankton cell abundances. Results suggest that microorganisms may be involved in compensating effects on cloud properties, increasing the frequency of occurrence of warm‐liquid clouds, and decreasing the occurrence of ice‐containing clouds in most regions during springtime. The relationships observed in most regions do not apply to the South Pacific Ocean in the 40°S–50°S latitude band. These results shed light on overlooked potential compensating effects of ocean microorganisms on cloud cover.
Plain Language Summary
Climate is governed by interactions between the ocean and the atmosphere. While physical interactions such as exchanges of heat and water vapor are fairly well understood, the role of biology, that is, the living marine microorganisms, on atmospheric processes, is a lot more complex. For instance, marine microorganisms may influence the number and the chemical composition of sea sprays and also emit trace gasses that will form tiny particles. Sea sprays and newly formed particles can then serve as nuclei on which cloud droplets or ice crystals form, therefore influencing cloud properties and climate. These chains of processes are theoretical, and there are few clear linkages between ocean biology and cloud properties derived from observational data. This study uses new satellite retrievals to establish relationships between cloud phase occurrence (ice, warm‐liquid, mixed‐phase or supercooled‐liquid clouds) and the biological activity of the ocean in different regions of the southern ocean. For a given month, locations of higher abundance of phytoplankton corresponds to a higher warm‐liquid cloud cover but lower ice cloud cover. These results suggest compensating effects of marine microorganisms on cloud lifetime via their potential to impact the formation of particles able to become water droplets or ice crystals.
Key Points
Nanophytoplankton biomass shows more relations to cloud occurrences than Chlorophyll‐a or Particulate Organic Carbon concentrations
Higher nanophytoplankon abundance is positively linked to warm‐liquid cloud frequency of occurrence in spring in most regions of 40°S–60°S
Higher nanophytoplankton abundance is linked to a decrease in the ice‐containing cloud frequency of occurrence in most regions
•Heterogeneous cirrus clouds are generated.•Lidar signals are simulated using a Monte-Carlo code.•Effects on CALIOP lidar measured data are evaluated.•Importance of horizontal photon transport is ...underscored.
The goal of this work is to evaluate the effects of cirrus heterogeneity on characteristics that are directly measured by the CALIOP/CALIPSO lidar, i.e. attenuated backscatter coefficient and depolarization ratio. This assessment was done using the 3D Monte Carlo simulator of Polarized Lidar signals (3DMcPOLID) together with the high-resolution 3D cloud fields-generator 3DCLOUD_V2. The evaluation is based on random sampling and on comparison between mean profiles of 3D clouds and of plane-parallel equivalent 1D clouds.
Mean profiles of the apparent attenuated backscatter as well as of the integrated apparent backscatter are statistically equal when a cirrus cloud field is probed with the 325 m resolution. To the contrary, the difference between profiles is statistically significant in the case of the 1 km resolution. Profiles of the volume depolarization ratio are statistically different for both cases of the horizontal resolution. The total bias of CALIOP/CALIPSO lidar data is mainly due to the plane parallel bias and multiple scattering, i.e., horizontal photon transport.
The aim of this paper is to present the Monte Carlo code McRALI that
provides simulations under multiple-scattering regimes of polarized high-spectral-resolution (HSR) lidar and Doppler radar ...observations for
a three-dimensional (3D) cloudy atmosphere. The effects of nonuniform beam
filling (NUBF) on HSR lidar and Doppler radar signals related to the
EarthCARE mission are investigated with the help of an academic 3D
box cloud characterized by a single isolated jump in cloud optical depth,
assuming vertically constant wind velocity. Regarding Doppler radar signals,
it is confirmed that NUBF induces a severe bias in velocity estimates. The
correlation of the NUBF bias of Doppler velocity with the horizontal
gradient of reflectivity shows a correlation coefficient value around 0.15 m s−1 (dBZ km-1)-1, close to that given in the scientific
literature. Regarding HSR lidar signals, we confirm that multiple-scattering
processes are not negligible. We show that NUBF effects on molecular,
particulate, and total attenuated backscatter are mainly due to unresolved
variability of cloud inside the receiver field of view and, to a lesser
extent, to the horizontal photon transport. This finding gives some insight
into the reliability of lidar signal modeling using independent column
approximation (ICA).
During the CIRCLE-2 experiment carried out over Western Europe in May 2007, combined in situ and remote sensing observations allowed to describe microphysical and optical properties near-top of an ...overshooting convective cloud (11 080 m/−58 °C). The airborne measurements were performed with the DLR Falcon aircraft specially equipped with a unique set of instruments for the extensive in situ cloud measurements of microphysical and optical properties (Polar Nephelometer, FSSP-300, Cloud Particle Imager and PMS 2-D-C) and nadir looking remote sensing observations (DLR WALES Lidar). Quasi-simultaneous space observations from MSG/SEVIRI, CALIPSO/CALIOP-WFC-IIR and CloudSat/CPR combined with airborne RASTA radar reflectivity from the French Falcon aircraft flying above the DLR Falcon depict very well convective cells which overshoot by up to 600 m the tropopause level. Unusual high values of the concentration of small ice particles, extinction, ice water content (up to 70 cm−3, 30 km−1 and 0.5 g m−3, respectively) are experienced. The mean effective diameter and the maximum particle size are 43 μm and about 300 μm, respectively. This very dense cloud causes a strong attenuation of the WALES and CALIOP lidar returns. The SEVIRI retrieved parameters confirm the occurrence of small ice crystals at the top of the convective cell. Smooth and featureless phase functions with asymmetry factors of 0.776 indicate fairly uniform optical properties. Due to small ice crystals the power-law relationship between ice water content (IWC) and radar reflectivity appears to be very different from those usually found in cirrus and anvil clouds. For a given equivalent reflectivity factor, IWCs are significantly larger for the overshooting cell than for the cirrus. Assuming the same prevalent microphysical properties over the depth of the overshooting cell, RASTA reflectivity profiles scaled into ice water content show that retrieved IWC up to 1 g m−3 may be observed near the cloud top. Extrapolating the relationship for stronger convective clouds with similar ice particles, IWC up to 5 g m−3 could be experienced with reflectivity factors no larger than about 20 dBZ. This means that for similar situations, indication of rather weak radar echo does not necessarily warn the occurrence of high ice water content carried by small ice crystals. All along the cloud penetration the shape of the ice crystals is dominated by chain-like aggregates of frozen droplets. Our results confirm previous observations that the chains of ice crystals are found in a continental deep convective systems which are known generally to generate intense electric fields causing efficient ice particle aggregation processes. Vigorous updrafts could lift supercooled droplets which are frozen extremely rapidly by homogeneous nucleation near the −37 °C level, producing therefore high concentrations of very small ice particles at upper altitudes. They are sufficient to deplete the water vapour and suppress further nucleation as confirmed by humidity measurements. These observations address scientific issues related to the microphysical properties and structure of deep convective clouds and confirm that particles smaller than 50 μm may control the radiative properties in convective-related clouds. These unusual observations may also provide some possible insights regarding engineering issues related to the failure of jet engines commonly used on commercial aircraft during flights through areas of high ice water content. However, large uncertainties of the measured and derived parameters limit our observations.
In this paper, we describe in situ observations of mid-latitude cirrus cloud band carried out on 16 May 2007 during the CIRCLE-2 experiment. The Polar Nephelometer and the Cloud Particle Imager (CPI) ...instruments with PMS FSSP-300 and 2D-C probes were used for the description of the optical and microphysical cloud properties. Two selected cloud regions are compared and discussed in detail. Significant differences in optical properties are evidenced in terms of 22° halo occurrences even though prevalent planar-plate ice crystals are observed in both cloud regions. Featureless scattering phase functions are measured in the first cloud region located near the trailing edge of the cirrus-band at about 11 800 m/−57 °C. In contrast, well pronounced 22° halo peaks are observed with predominant similar-shaped ice crystals near the cirrus-band leading edge at 7100 m/−27 °C. CPI ice crystal images with Polar Nephelometer observations are carefully analysed and interpreted from a theoretical light scattering model in order to explain occurrence and non-occurrence of the 22° halo feature. The results highlight that the halo peaks are inherent only in perfect plate ice crystals (or pristine crystals). On the basis of previous datasets in mid-latitude cirrus, it is found that simple pristine crystals are uncommon whereas particles with imperfect or complex shapes are prevalent. As a result, phase functions that are smooth and featureless best represent cirrus scattering properties.
Airborne measurements of spectral upwelling radiances (350–2200 nm) reflected by cirrus using the Spectral Modular Airborne Radiation measurement sysTem (SMART)‐Albedometer were made over land and ...water surfaces. Based on these data, cloud optical thickness τ and effective radius Reff of the observed cirrus were retrieved. By using different crystal shape assumptions (hexagonal plates, solid and hollow columns, rough aggregates, planar and spatial rosettes, ice spheres, and a mixture of particle habits) in the retrieval, the influence of crystal shape on the retrieved τ and Reff was evaluated. With relative differences of up to 70%, the influence of particle habit on τ is larger than on Reff (up to 20% differences). Retrieved τ values agreed with values derived from concurrent lidar measurements within the measurement uncertainties.