We study the spectrum of elementary excitations of a dipolar Bose gas in a three-dimensional anisotropic trap across the superfluid-supersolid phase transition. Theoretically, we show that, when ...entering the supersolid phase, two distinct excitation branches appear, respectively associated with dominantly crystal and superfluid excitations. These results confirm infinite-system predictions, showing that finite-size effects play only a small qualitative role, and connect the two branches to the simultaneous occurrence of crystal and superfluid orders. Experimentally, we probe compressional excitations in an Er quantum gas across the phase diagram. While in the Bose-Einstein condensate regime the system exhibits an ordinary quadrupole oscillation, in the supersolid regime we observe a striking two-frequency response of the system, related to the two spontaneously broken symmetries.
We measure the excitation spectrum of a stable dipolar Bose-Einstein condensate over a wide momentum range via Bragg spectroscopy. We precisely control the relative strength ε_{dd} of the dipolar to ...the contact interactions and observe that the spectrum increasingly deviates from the linear phononic behavior for increasing ε_{dd}. Reaching the dipolar-dominated regime ε_{dd}>1, we observe the emergence of a roton minimum in the spectrum and its softening towards instability. We characterize how the excitation energy and the strength of the density-density correlations at the roton momentum vary with ε_{dd}. Our findings are in excellent agreement with numerical calculations based on mean-field Bogoliubov theory. When including beyond-mean-field corrections, in the form of a Lee-Huang-Yang potential, we observe a quantitative deviation from the experiment, questioning the validity of such a description in the roton regime.
Abstract
We present a solution for the ultraviolet – submillimetre (submm) interstellar radiation fields (ISRFs) of the Milky Way (MW), derived from modelling COBE, IRAS and Planck maps of the ...all-sky emission in the near-, mid-, far-infrared and submm. The analysis uses the axisymmetric radiative transfer model that we have previously implemented to model the panchromatic spectral energy distributions (SEDs) of star-forming galaxies in the nearby universe, but with a new methodology allowing for optimization of the radial and vertical geometry of stellar emissivity and dust opacity, as deduced from the highly resolved emission seen from the vantage point of the Sun. As such, this is the first self-consistent model of the broad-band continuum emission from the MW. In this paper, we present model predictions for the spatially integrated SED of the MW as seen from the Sun, showing good agreement with the data, and give a detailed description of the solutions for the distribution of ISRFs, as well as their physical origin, throughout the volume of the galaxy. We explore how the spatial and spectral distributions of our new predictions for the ISRF in the MW affects the amplitude and spectral distributions of the gamma rays produced via inverse Compton scattering for cosmic ray (CR) electrons situated at different positions in the galaxy, as well as the attenuation of the gamma rays due to interactions of the gamma-ray photons with photons of the ISRF. We also compare and contrast our solutions for the ISRF with those incorporated in the galprop package used for modelling the high-energy emission from CR in the MW.
Glutamatergic hyperactivity in the nucleus striatum, the main basal ganglia input, has been involved in the progression of Parkinson's disease (PD) and the onset of L-Dopa-induced dyskinesias (LIDs). ...Abnormalities in the spiny projection neurons excitability and firing, and in the overactivity of glutamate transmission found in animal models of PD, pointed to the synaptic dysfunctions as a primary target to counteract alterations before overt neurodegeneration, conferring a key role to striatal glutamatergic transmission in the early phases of the disease. The present paper provides an overview of the evidence that glutamatergic overactivity is a critical mechanism underlying different PD-associated striatal alterations in early and advanced symptomatic stages of the disease. These aberrant changes, under L-Dopa therapy, lead to a more complex synaptopathy that involves other neurotransmitter systems and persistent modifications to generate LIDs. The review discusses the main changes in glutamatergic functions found in PD preclinical models and clinical studies and an update of the current pharmacological strategies to modulate the glutamatergic systems at the pre- and postsynaptic levels will be provided.
•Glutamate-mediated excitatory signals play a key role in the basal ganglia circuitry.•Excessive glutamatergic transmission in the striatum is implicated in the progression of PD and in the emergence of LIDs.•DA levels reduction leads to alterations in firing activity patterns in tPD striatum of experimental models and patients.•Blunting excessive glutamate transmission is a therapeutic strategy to normalize neurotransmitter synaptic levels.
A supersolid is a counterintuitive phase of matter that combines the global phase coherence of a superfluid with a crystal-like self-modulation in space. Recently, such states have been ...experimentally realized using dipolar quantum gases. Here we investigate the response of a dipolar supersolid to an interaction quench that shatters the global phase coherence. We identify a parameter regime in which this out-of-equilibrium state rephases, indicating superfluid flow across the sample as well as an efficient dissipation mechanism. We find a crossover to a regime where the tendency to rephase gradually decreases until the system relaxes into an incoherent droplet array. Although a dipolar supersolid is, by its nature, ‘soft’, we capture the essential behaviour of the de- and rephasing process within a rigid Josephson junction array model. Yet, both experiment and simulation indicate that the interaction quench causes substantial collective mode excitations that connect to phonons in solids and affect the phase dynamics.A supersolid is a phase of matter featuring both crystalline order as a solid and global phase coherence as a superfluid. Now an experiment shows how this global phase coherence can be established across the system in a non-equilibrium process.
We realize a two-component dipolar Fermi gas with tunable interactions, using erbium atoms. Employing a lattice-protection technique, we selectively prepare deeply degenerate mixtures of the two ...lowest spin states and perform high-resolution Feshbach spectroscopy in an optical dipole trap. We identify a comparatively broad Feshbach resonance and map the interspin scattering length in its vicinity. The Fermi mixture shows a remarkable collisional stability in the strongly interacting regime, providing a first step towards studies of superfluid pairing, crossing from Cooper pairs to bound molecules, in presence of dipole-dipole interactions.
Amorphous alumina is highly transparent across the visible spectrum, making it a promising candidate for low-loss waveguiding at short wavelengths. However, previous alumina waveguide demonstrations ...in the visible region have focused on low- to moderate-confinement waveguides, where the diffuse mode reduces the design flexibility and integration density of photonic integrated circuits. Here, we have developed a high-quality etch mask and a highly selective BCl3 plasma etch, allowing etching of amorphous alumina waveguides up to 800 nm thick. Using this process, we have fabricated waveguides using an alumina film grown by atomic layer deposition (ALD) which are the lowest-loss high-confinement waveguides for blue light to date: we achieve single-mode propagation losses of 0.8 dB/cm at a propagation wavelength of 450 nm.
By combining theory and experiments, we demonstrate that dipolar quantum gases of bothEr166andDy164support a state with supersolid properties, where a spontaneous density modulation and a global ...phase coherence coexist. This paradoxical state occurs in a well-defined parameter range, separating the phases of a regular Bose-Einstein condensate and of an insulating droplet array, and is rooted in the roton mode softening, on the one side, and in the stabilization driven by quantum fluctuations, on the other side. Here, we identify the parameter regime for each of the three phases. In the experiment, we rely on a detailed analysis of the interference patterns resulting from the free expansion of the gas, quantifying both its density modulation and its global phase coherence. Reaching the phases via a slow interaction tuning, starting from a stable condensate, we observe thatEr166andDy164exhibit a striking difference in the lifetime of the supersolid properties, due to the different atom loss rates in the two systems. Indeed, while inEr166the supersolid behavior survives only a few tens of milliseconds, we observe coherent density modulations for more than 150 ms inDy164. Building on this long lifetime, we demonstrate an alternative path to reach the supersolid regime, relying solely on evaporative cooling starting from a thermal gas.
The diffusion of saturated and unsaturated hydrocarbons is of fundamental importance for many zeolite‐catalyzed processes. Transport of small alkenes in the confined zeolite pores can become ...hindered, resulting in a significant impact on the ultimate product selectivity and separation. Herein, intracrystalline light olefin/paraffin diffusion through the 8‐ring windows of zeolite SAPO‐34 is characterized by a complementary set of first‐principle molecular dynamics simulations, PFG‐NMR experiments, and pulse‐response temporal analysis of products measurements, yielding information at different length and time scales. Our results clearly show a promotional effect of the presence of Brønsted acid sites on the diffusion rate of ethene and propene, whereas transport of alkanes is found to be insensitive to the presence of acid sites. The enhanced diffusivity of unsaturated hydrocarbons is ascribed to the formation of favorable π–H interactions with acid protons, as confirmed by IR spectroscopy measurements. The acid site distribution is proven to be an important design parameter for optimizing product distributions and separations.
The influence of the acid site density on the diffusivities of alkanes and alkenes through the 8‐ring windows of SAPO‐34 was probed using a complementary set of ab initio MD simulations and experimental techniques (PFG‐NMR and TAP pulse‐response measurements). The presence of Brønsted acid sites was found to have a clear promotional effect on alkene diffusion but it does not influence alkane diffusion.
Abstract
Interpreting volcanic unrest is a highly challenging and non-unique problem at calderas, since large hydrothermal systems may either hide or amplify the dynamics of buried magma(s). Here we ...use the exceptional ground displacement and geochemical datasets from the actively degassing Campi Flegrei caldera (Southern Italy) to show that ambiguities disappear when the thermal evolution of the deep hydrothermal system is accurately tracked. By using temperatures from the CO
2
-CH
4
exchange of
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C and thermodynamic analysis of gas ascending in the crust, we demonstrate that after the last 1982–84 crisis the deep hydrothermal system evolved through supercritical conditions under the continuous isenthalpic inflow of hot CO
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-rich gases released from the deep (~8 km) magma reservoir of regional size. This resulted in the drying of the base of the hot hydrothermal system, no more buffered along the liquid-vapour equilibrium, and excludes any shallow arrival of new magma, whose abundant steam degassing due to decompression would have restored liquid-vapour equilibrium. The consequent CO
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-infiltration and progressive heating of the surrounding deforming rock volume cause the build-up of pore pressure in aquifers, and generate the striking temporal symmetry that characterizes the ongoing uplift and the post-1984 subsidence, both originated by the same but reversed deformation mechanism.