In this work, we study the topological properties and magnon Hall effect of a three-dimensional ferromagnet in the ABC stacking honeycomb lattice, motivated by the recent inelastic neutron scattering ...study of CrI3. We show that the magnon band structure and Chern numbers of the magnon branches are significantly affected by the interlayer coupling Jc, which moreover has a qualitatively different effect in the ABC stacking compared to the AA stacking adopted by other authors. The nontrivial Chern number of the lowest magnon band is stabilized by the next-nearest-neighbor Dzyaloshinskii-Moriya interaction in each honeycomb layer, resulting in the hopping term similar to that in the electronic Haldane model for graphene. However, we also find several gapless Weyl points, separating the nonequivalent Chern insulating phases, tuned by the ratio of the interlayer coupling Jc and the third-neighbor Heisenberg interaction J3. We further show that the topological character of magnon bands results in nonzero thermal Hall conductivity, whose sign and magnitude depend on Jc and the intralayer couplings. Since the interlayer coupling strength Jc can be easily tuned by applying pressure to the quasi-2D material such as CrI3, this provides a potential route to tuning the magnon thermal Hall effect in an experiment.
We use neutron resonance spin echo and Larmor diffraction to study the effect of uniaxial pressure on the tetragonal-to-orthorhombic structural (T sub(s)) and antiferromagnetic (AF) phase transitions ...in iron pnictides BaFe sub(2-x) Ni sub(x) As sub(2)(x=0,0.03,0.12),SrFe sub(1.97) Ni sub(0.03) As sub(2), and BaFe sub(2)(As sub(0.7) P sub(0.3)) sub(2). In antiferromagnetically ordered BaFe sub(2-x) Ni sub(x) As sub(2) and SrFe sub(1.97) Ni sub(0.03) As sub(2) with T sub(N) and T sub(s)(T sub(N)T sub(s)), a uniaxial pressure necessary to detwin the sample also increases T sub(N), smears out the structural transition, and induces an orthorhombic lattice distortion at all temperatures. By comparing temperature and doping dependence of the pressure induced lattice parameter changes with the elastoresistance and nematic susceptibility obtained from transport and ultrasonic measurements, we conclude that the in-plane resistivity anisotropy found in the paramagnetic state of electron underdoped iron pnictides depends sensitively on the nature of the magnetic phase transition and a strong coupling between the uniaxial pressure induced lattice distortion and electronic nematic susceptibility.
The origin of magnetism in metals has been traditionally discussed in two diametrically opposite limits: itinerant and local moments. Surprisingly, there are very few known examples of materials that ...are close to the itinerant limit, and their properties are not universally understood. In the case of the two such examples discovered several decades ago, the itinerant ferromagnets ZrZn2 and Sc3In, the understanding of their magnetic ground states draws on the existence of 3d electrons subject to strong spin fluctuations. Similarly, in Cr, an elemental itinerant antiferromagnet with a spin density wave ground state, its 3d electron character has been deemed crucial to it being magnetic. Here, we report evidence for an itinerant antiferromagnetic metal with no magnetic constituents: TiAu. Antiferromagnetic order occurs below a Néel temperature of 36 K, about an order of magnitude smaller than in Cr, rendering the spin fluctuations in TiAu more important at low temperatures. This itinerant antiferromagnet challenges the currently limited understanding of weak itinerant antiferromagnetism, while providing insights into the effects of spin fluctuations in itinerant-electron systems.
We report measurements of the diffusion of atomic hydrogen in single crystalline VO2 micro/nanobeams by direct exposure to atomic hydrogen, without catalyst. The atomic hydrogen is generated by a hot ...filament, and the doping process takes place at moderate temperature (373 K). Undoped VO2 has a metal-to-insulator phase transition at ∼340 K between a high-temperature, rutile, metallic phase and a low-temperature, monoclinic, insulating phase with a resistance exhibiting a semiconductor-like temperature dependence. Atomic hydrogenation results in stabilization of the metallic phase of VO2 micro/nanobeams down to 2 K, the lowest point we could reach in our measurement setup. Optical characterization shows that hydrogen atoms prefer to diffuse along the c axis of rutile (a axis of monoclinic) VO2, along the oxygen “channels”. Based on observing the movement of the hydrogen diffusion front in single crystalline VO2 beams, we estimate the diffusion constant for hydrogen along the c axis of the rutile phase to be 6.7 × 10–10 cm2/s at approximately 373 K, exceeding the value in isostructural TiO2 by ∼38×. Moreover, we find that the diffusion constant along the c axis of the rutile phase exceeds that along the equivalent a axis of the monoclinic phase by at least 3 orders of magnitude. This remarkable change in kinetics must originate from the distortion of the “channels” when the unit cell doubles along this direction upon cooling into the monoclinic structure. Ab initio calculation results are in good agreement with the experimental trends in the relative kinetics of the two phases. This raises the possibility of a switchable membrane for hydrogen transport.
The Ni1+/Ni2+ states of nickelates have the identical (3d(9)/3d(8)) electronic configuration as Cu2+/Cu3+ in the high temperature superconducting cuprates, and are expected to show interesting ...properties. An intriguing question is whether mimicking the electronic and structural features of cuprates would also result in superconductivity in nickelates. Here we report experimental evidence for a bulklike magnetic transition in La4Ni3O8 at 105 K. Density functional theory calculations relate the transition to a spin density wave nesting instability of the Fermi surface.
Here we provide the first clear evidence of Fermi-liquid breakdown in an intermediate valence system. We employ high precision magnetization measurements of the valence fluctuating superconductor ...β-YbAlB4 to probe the quantum critical free energy down to temperatures far below the characteristic energy scale of the valence fluctuations. The observed T/B scaling in the magnetization over three decades not only indicates unconventional quantum criticality, but places an upper bound on the critical magnetic field |Bc| < 0.2 mT, a value comparable with the Earth's magnetic field and six orders of magnitude smaller than the valence fluctuation scale. This tiny value of the upper bound on Bc, well inside the superconducting dome, raises the fascinating possibility that valence fluctuating β-YbAlB4 is intrinsically quantum critical, without tuning the magnetic field, pressure, or composition: the first known example of such a phenomenon in a metal.